Cargando…

Highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a MoO(3)/Au/MoO(3) electrode with encapsulation

Stretchable organic light-emitting diodes are ubiquitous in the rapidly developing wearable display technology. However, low efficiency and poor mechanical stability inhibit their commercial applications owing to the restrictions generated by strain. Here, we demonstrate the exceptional performance...

Descripción completa

Detalles Bibliográficos
Autores principales: Choi, Dae Keun, Kim, Dong Hyun, Lee, Chang Min, Hafeez, Hassan, Sarker, Subrata, Yang, Jun Su, Chae, Hyung Ju, Jeong, Geon-Woo, Choi, Dong Hyun, Kim, Tae Wook, Yoo, Seunghyup, Song, Jinouk, Ma, Boo Soo, Kim, Taek-Soo, Kim, Chul Hoon, Lee, Hyun Jae, Lee, Jae Woo, Kim, Donghyun, Bae, Tae-Sung, Yu, Seung Min, Kang, Yong-Cheol, Park, Juyun, Kim, Kyoung-Ho, Sujak, Muhammad, Song, Myungkwan, Kim, Chang-Su, Ryu, Seung Yoon
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8128878/
https://www.ncbi.nlm.nih.gov/pubmed/34001906
http://dx.doi.org/10.1038/s41467-021-23203-y
_version_ 1783694190012530688
author Choi, Dae Keun
Kim, Dong Hyun
Lee, Chang Min
Hafeez, Hassan
Sarker, Subrata
Yang, Jun Su
Chae, Hyung Ju
Jeong, Geon-Woo
Choi, Dong Hyun
Kim, Tae Wook
Yoo, Seunghyup
Song, Jinouk
Ma, Boo Soo
Kim, Taek-Soo
Kim, Chul Hoon
Lee, Hyun Jae
Lee, Jae Woo
Kim, Donghyun
Bae, Tae-Sung
Yu, Seung Min
Kang, Yong-Cheol
Park, Juyun
Kim, Kyoung-Ho
Sujak, Muhammad
Song, Myungkwan
Kim, Chang-Su
Ryu, Seung Yoon
author_facet Choi, Dae Keun
Kim, Dong Hyun
Lee, Chang Min
Hafeez, Hassan
Sarker, Subrata
Yang, Jun Su
Chae, Hyung Ju
Jeong, Geon-Woo
Choi, Dong Hyun
Kim, Tae Wook
Yoo, Seunghyup
Song, Jinouk
Ma, Boo Soo
Kim, Taek-Soo
Kim, Chul Hoon
Lee, Hyun Jae
Lee, Jae Woo
Kim, Donghyun
Bae, Tae-Sung
Yu, Seung Min
Kang, Yong-Cheol
Park, Juyun
Kim, Kyoung-Ho
Sujak, Muhammad
Song, Myungkwan
Kim, Chang-Su
Ryu, Seung Yoon
author_sort Choi, Dae Keun
collection PubMed
description Stretchable organic light-emitting diodes are ubiquitous in the rapidly developing wearable display technology. However, low efficiency and poor mechanical stability inhibit their commercial applications owing to the restrictions generated by strain. Here, we demonstrate the exceptional performance of a transparent (molybdenum-trioxide/gold/molybdenum-trioxide) electrode for buckled, twistable, and geometrically stretchable organic light-emitting diodes under 2-dimensional random area strain with invariant color coordinates. The devices are fabricated on a thin optical-adhesive/elastomer with a small mechanical bending strain and water-proofed by optical-adhesive encapsulation in a sandwiched structure. The heat dissipation mechanism of the thin optical-adhesive substrate, thin elastomer-based devices or silicon dioxide nanoparticles reduces triplet-triplet annihilation, providing consistent performance at high exciton density, compared with thick elastomer and a glass substrate. The performance is enhanced by the nanoparticles in the optical-adhesive for light out-coupling and improved heat dissipation. A high current efficiency of ~82.4 cd/A and an external quantum efficiency of ~22.3% are achieved with minimum efficiency roll-off.
format Online
Article
Text
id pubmed-8128878
institution National Center for Biotechnology Information
language English
publishDate 2021
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-81288782021-06-01 Highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a MoO(3)/Au/MoO(3) electrode with encapsulation Choi, Dae Keun Kim, Dong Hyun Lee, Chang Min Hafeez, Hassan Sarker, Subrata Yang, Jun Su Chae, Hyung Ju Jeong, Geon-Woo Choi, Dong Hyun Kim, Tae Wook Yoo, Seunghyup Song, Jinouk Ma, Boo Soo Kim, Taek-Soo Kim, Chul Hoon Lee, Hyun Jae Lee, Jae Woo Kim, Donghyun Bae, Tae-Sung Yu, Seung Min Kang, Yong-Cheol Park, Juyun Kim, Kyoung-Ho Sujak, Muhammad Song, Myungkwan Kim, Chang-Su Ryu, Seung Yoon Nat Commun Article Stretchable organic light-emitting diodes are ubiquitous in the rapidly developing wearable display technology. However, low efficiency and poor mechanical stability inhibit their commercial applications owing to the restrictions generated by strain. Here, we demonstrate the exceptional performance of a transparent (molybdenum-trioxide/gold/molybdenum-trioxide) electrode for buckled, twistable, and geometrically stretchable organic light-emitting diodes under 2-dimensional random area strain with invariant color coordinates. The devices are fabricated on a thin optical-adhesive/elastomer with a small mechanical bending strain and water-proofed by optical-adhesive encapsulation in a sandwiched structure. The heat dissipation mechanism of the thin optical-adhesive substrate, thin elastomer-based devices or silicon dioxide nanoparticles reduces triplet-triplet annihilation, providing consistent performance at high exciton density, compared with thick elastomer and a glass substrate. The performance is enhanced by the nanoparticles in the optical-adhesive for light out-coupling and improved heat dissipation. A high current efficiency of ~82.4 cd/A and an external quantum efficiency of ~22.3% are achieved with minimum efficiency roll-off. Nature Publishing Group UK 2021-05-17 /pmc/articles/PMC8128878/ /pubmed/34001906 http://dx.doi.org/10.1038/s41467-021-23203-y Text en © The Author(s) 2021, corrected publication 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Choi, Dae Keun
Kim, Dong Hyun
Lee, Chang Min
Hafeez, Hassan
Sarker, Subrata
Yang, Jun Su
Chae, Hyung Ju
Jeong, Geon-Woo
Choi, Dong Hyun
Kim, Tae Wook
Yoo, Seunghyup
Song, Jinouk
Ma, Boo Soo
Kim, Taek-Soo
Kim, Chul Hoon
Lee, Hyun Jae
Lee, Jae Woo
Kim, Donghyun
Bae, Tae-Sung
Yu, Seung Min
Kang, Yong-Cheol
Park, Juyun
Kim, Kyoung-Ho
Sujak, Muhammad
Song, Myungkwan
Kim, Chang-Su
Ryu, Seung Yoon
Highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a MoO(3)/Au/MoO(3) electrode with encapsulation
title Highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a MoO(3)/Au/MoO(3) electrode with encapsulation
title_full Highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a MoO(3)/Au/MoO(3) electrode with encapsulation
title_fullStr Highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a MoO(3)/Au/MoO(3) electrode with encapsulation
title_full_unstemmed Highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a MoO(3)/Au/MoO(3) electrode with encapsulation
title_short Highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a MoO(3)/Au/MoO(3) electrode with encapsulation
title_sort highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a moo(3)/au/moo(3) electrode with encapsulation
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8128878/
https://www.ncbi.nlm.nih.gov/pubmed/34001906
http://dx.doi.org/10.1038/s41467-021-23203-y
work_keys_str_mv AT choidaekeun highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT kimdonghyun highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT leechangmin highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT hafeezhassan highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT sarkersubrata highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT yangjunsu highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT chaehyungju highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT jeonggeonwoo highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT choidonghyun highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT kimtaewook highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT yooseunghyup highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT songjinouk highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT maboosoo highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT kimtaeksoo highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT kimchulhoon highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT leehyunjae highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT leejaewoo highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT kimdonghyun highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT baetaesung highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT yuseungmin highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT kangyongcheol highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT parkjuyun highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT kimkyoungho highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT sujakmuhammad highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT songmyungkwan highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT kimchangsu highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation
AT ryuseungyoon highlyefficientheatdissipatingstretchableorganiclightemittingdiodesbasedonamoo3aumoo3electrodewithencapsulation