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Highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a MoO(3)/Au/MoO(3) electrode with encapsulation
Stretchable organic light-emitting diodes are ubiquitous in the rapidly developing wearable display technology. However, low efficiency and poor mechanical stability inhibit their commercial applications owing to the restrictions generated by strain. Here, we demonstrate the exceptional performance...
Autores principales: | , , , , , , , , , , , , , , , , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2021
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8128878/ https://www.ncbi.nlm.nih.gov/pubmed/34001906 http://dx.doi.org/10.1038/s41467-021-23203-y |
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author | Choi, Dae Keun Kim, Dong Hyun Lee, Chang Min Hafeez, Hassan Sarker, Subrata Yang, Jun Su Chae, Hyung Ju Jeong, Geon-Woo Choi, Dong Hyun Kim, Tae Wook Yoo, Seunghyup Song, Jinouk Ma, Boo Soo Kim, Taek-Soo Kim, Chul Hoon Lee, Hyun Jae Lee, Jae Woo Kim, Donghyun Bae, Tae-Sung Yu, Seung Min Kang, Yong-Cheol Park, Juyun Kim, Kyoung-Ho Sujak, Muhammad Song, Myungkwan Kim, Chang-Su Ryu, Seung Yoon |
author_facet | Choi, Dae Keun Kim, Dong Hyun Lee, Chang Min Hafeez, Hassan Sarker, Subrata Yang, Jun Su Chae, Hyung Ju Jeong, Geon-Woo Choi, Dong Hyun Kim, Tae Wook Yoo, Seunghyup Song, Jinouk Ma, Boo Soo Kim, Taek-Soo Kim, Chul Hoon Lee, Hyun Jae Lee, Jae Woo Kim, Donghyun Bae, Tae-Sung Yu, Seung Min Kang, Yong-Cheol Park, Juyun Kim, Kyoung-Ho Sujak, Muhammad Song, Myungkwan Kim, Chang-Su Ryu, Seung Yoon |
author_sort | Choi, Dae Keun |
collection | PubMed |
description | Stretchable organic light-emitting diodes are ubiquitous in the rapidly developing wearable display technology. However, low efficiency and poor mechanical stability inhibit their commercial applications owing to the restrictions generated by strain. Here, we demonstrate the exceptional performance of a transparent (molybdenum-trioxide/gold/molybdenum-trioxide) electrode for buckled, twistable, and geometrically stretchable organic light-emitting diodes under 2-dimensional random area strain with invariant color coordinates. The devices are fabricated on a thin optical-adhesive/elastomer with a small mechanical bending strain and water-proofed by optical-adhesive encapsulation in a sandwiched structure. The heat dissipation mechanism of the thin optical-adhesive substrate, thin elastomer-based devices or silicon dioxide nanoparticles reduces triplet-triplet annihilation, providing consistent performance at high exciton density, compared with thick elastomer and a glass substrate. The performance is enhanced by the nanoparticles in the optical-adhesive for light out-coupling and improved heat dissipation. A high current efficiency of ~82.4 cd/A and an external quantum efficiency of ~22.3% are achieved with minimum efficiency roll-off. |
format | Online Article Text |
id | pubmed-8128878 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-81288782021-06-01 Highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a MoO(3)/Au/MoO(3) electrode with encapsulation Choi, Dae Keun Kim, Dong Hyun Lee, Chang Min Hafeez, Hassan Sarker, Subrata Yang, Jun Su Chae, Hyung Ju Jeong, Geon-Woo Choi, Dong Hyun Kim, Tae Wook Yoo, Seunghyup Song, Jinouk Ma, Boo Soo Kim, Taek-Soo Kim, Chul Hoon Lee, Hyun Jae Lee, Jae Woo Kim, Donghyun Bae, Tae-Sung Yu, Seung Min Kang, Yong-Cheol Park, Juyun Kim, Kyoung-Ho Sujak, Muhammad Song, Myungkwan Kim, Chang-Su Ryu, Seung Yoon Nat Commun Article Stretchable organic light-emitting diodes are ubiquitous in the rapidly developing wearable display technology. However, low efficiency and poor mechanical stability inhibit their commercial applications owing to the restrictions generated by strain. Here, we demonstrate the exceptional performance of a transparent (molybdenum-trioxide/gold/molybdenum-trioxide) electrode for buckled, twistable, and geometrically stretchable organic light-emitting diodes under 2-dimensional random area strain with invariant color coordinates. The devices are fabricated on a thin optical-adhesive/elastomer with a small mechanical bending strain and water-proofed by optical-adhesive encapsulation in a sandwiched structure. The heat dissipation mechanism of the thin optical-adhesive substrate, thin elastomer-based devices or silicon dioxide nanoparticles reduces triplet-triplet annihilation, providing consistent performance at high exciton density, compared with thick elastomer and a glass substrate. The performance is enhanced by the nanoparticles in the optical-adhesive for light out-coupling and improved heat dissipation. A high current efficiency of ~82.4 cd/A and an external quantum efficiency of ~22.3% are achieved with minimum efficiency roll-off. Nature Publishing Group UK 2021-05-17 /pmc/articles/PMC8128878/ /pubmed/34001906 http://dx.doi.org/10.1038/s41467-021-23203-y Text en © The Author(s) 2021, corrected publication 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Choi, Dae Keun Kim, Dong Hyun Lee, Chang Min Hafeez, Hassan Sarker, Subrata Yang, Jun Su Chae, Hyung Ju Jeong, Geon-Woo Choi, Dong Hyun Kim, Tae Wook Yoo, Seunghyup Song, Jinouk Ma, Boo Soo Kim, Taek-Soo Kim, Chul Hoon Lee, Hyun Jae Lee, Jae Woo Kim, Donghyun Bae, Tae-Sung Yu, Seung Min Kang, Yong-Cheol Park, Juyun Kim, Kyoung-Ho Sujak, Muhammad Song, Myungkwan Kim, Chang-Su Ryu, Seung Yoon Highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a MoO(3)/Au/MoO(3) electrode with encapsulation |
title | Highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a MoO(3)/Au/MoO(3) electrode with encapsulation |
title_full | Highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a MoO(3)/Au/MoO(3) electrode with encapsulation |
title_fullStr | Highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a MoO(3)/Au/MoO(3) electrode with encapsulation |
title_full_unstemmed | Highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a MoO(3)/Au/MoO(3) electrode with encapsulation |
title_short | Highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a MoO(3)/Au/MoO(3) electrode with encapsulation |
title_sort | highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a moo(3)/au/moo(3) electrode with encapsulation |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8128878/ https://www.ncbi.nlm.nih.gov/pubmed/34001906 http://dx.doi.org/10.1038/s41467-021-23203-y |
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