Cargando…

Hot-carrier dynamics in InAs/AlAsSb multiple-quantum wells

A type-II InAs/AlAs[Formula: see text] Sb[Formula: see text] multiple-quantum well sample is investigated for the photoexcited carrier dynamics as a function of excitation photon energy and lattice temperature. Time-resolved measurements are performed using a near-infrared pump pulse, with photon en...

Descripción completa

Detalles Bibliográficos
Autores principales: Piyathilaka, Herath P., Sooriyagoda, Rishmali, Esmaielpour, Hamidreza, Whiteside, Vincent R., Mishima, Tetsuya D., Santos, Michael B., Sellers, Ian R., Bristow, Alan D.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8131607/
https://www.ncbi.nlm.nih.gov/pubmed/34006905
http://dx.doi.org/10.1038/s41598-021-89815-y
Descripción
Sumario:A type-II InAs/AlAs[Formula: see text] Sb[Formula: see text] multiple-quantum well sample is investigated for the photoexcited carrier dynamics as a function of excitation photon energy and lattice temperature. Time-resolved measurements are performed using a near-infrared pump pulse, with photon energies near to and above the band gap, probed with a terahertz probe pulse. The transient terahertz absorption is characterized by a multi-rise, multi-decay function that captures long-lived decay times and a metastable state for an excess-photon energy of [Formula: see text] meV. For sufficient excess-photon energy, excitation of the metastable state is followed by a transition to the long-lived states. Excitation dependence of the long-lived states map onto a nearly-direct band gap ([Formula: see text] ) density of states with an Urbach tail below [Formula: see text] . As temperature increases, the long-lived decay times increase [Formula: see text] , due to the increased phonon interaction of the unintentional defect states, and by phonon stabilization of the hot carriers [Formula: see text] . Additionally, Auger (and/or trap-assisted Auger) scattering above the onset of the plateau may also contribute to longer hot-carrier lifetimes. Meanwhile, the initial decay component shows strong dependence on excitation energy and temperature, reflecting the complicated initial transfer of energy between valence-band and defect states, indicating methods to further prolong hot carriers for technological applications.