Cargando…

Hot-carrier dynamics in InAs/AlAsSb multiple-quantum wells

A type-II InAs/AlAs[Formula: see text] Sb[Formula: see text] multiple-quantum well sample is investigated for the photoexcited carrier dynamics as a function of excitation photon energy and lattice temperature. Time-resolved measurements are performed using a near-infrared pump pulse, with photon en...

Descripción completa

Detalles Bibliográficos
Autores principales: Piyathilaka, Herath P., Sooriyagoda, Rishmali, Esmaielpour, Hamidreza, Whiteside, Vincent R., Mishima, Tetsuya D., Santos, Michael B., Sellers, Ian R., Bristow, Alan D.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8131607/
https://www.ncbi.nlm.nih.gov/pubmed/34006905
http://dx.doi.org/10.1038/s41598-021-89815-y
_version_ 1783694733923581952
author Piyathilaka, Herath P.
Sooriyagoda, Rishmali
Esmaielpour, Hamidreza
Whiteside, Vincent R.
Mishima, Tetsuya D.
Santos, Michael B.
Sellers, Ian R.
Bristow, Alan D.
author_facet Piyathilaka, Herath P.
Sooriyagoda, Rishmali
Esmaielpour, Hamidreza
Whiteside, Vincent R.
Mishima, Tetsuya D.
Santos, Michael B.
Sellers, Ian R.
Bristow, Alan D.
author_sort Piyathilaka, Herath P.
collection PubMed
description A type-II InAs/AlAs[Formula: see text] Sb[Formula: see text] multiple-quantum well sample is investigated for the photoexcited carrier dynamics as a function of excitation photon energy and lattice temperature. Time-resolved measurements are performed using a near-infrared pump pulse, with photon energies near to and above the band gap, probed with a terahertz probe pulse. The transient terahertz absorption is characterized by a multi-rise, multi-decay function that captures long-lived decay times and a metastable state for an excess-photon energy of [Formula: see text] meV. For sufficient excess-photon energy, excitation of the metastable state is followed by a transition to the long-lived states. Excitation dependence of the long-lived states map onto a nearly-direct band gap ([Formula: see text] ) density of states with an Urbach tail below [Formula: see text] . As temperature increases, the long-lived decay times increase [Formula: see text] , due to the increased phonon interaction of the unintentional defect states, and by phonon stabilization of the hot carriers [Formula: see text] . Additionally, Auger (and/or trap-assisted Auger) scattering above the onset of the plateau may also contribute to longer hot-carrier lifetimes. Meanwhile, the initial decay component shows strong dependence on excitation energy and temperature, reflecting the complicated initial transfer of energy between valence-band and defect states, indicating methods to further prolong hot carriers for technological applications.
format Online
Article
Text
id pubmed-8131607
institution National Center for Biotechnology Information
language English
publishDate 2021
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-81316072021-05-19 Hot-carrier dynamics in InAs/AlAsSb multiple-quantum wells Piyathilaka, Herath P. Sooriyagoda, Rishmali Esmaielpour, Hamidreza Whiteside, Vincent R. Mishima, Tetsuya D. Santos, Michael B. Sellers, Ian R. Bristow, Alan D. Sci Rep Article A type-II InAs/AlAs[Formula: see text] Sb[Formula: see text] multiple-quantum well sample is investigated for the photoexcited carrier dynamics as a function of excitation photon energy and lattice temperature. Time-resolved measurements are performed using a near-infrared pump pulse, with photon energies near to and above the band gap, probed with a terahertz probe pulse. The transient terahertz absorption is characterized by a multi-rise, multi-decay function that captures long-lived decay times and a metastable state for an excess-photon energy of [Formula: see text] meV. For sufficient excess-photon energy, excitation of the metastable state is followed by a transition to the long-lived states. Excitation dependence of the long-lived states map onto a nearly-direct band gap ([Formula: see text] ) density of states with an Urbach tail below [Formula: see text] . As temperature increases, the long-lived decay times increase [Formula: see text] , due to the increased phonon interaction of the unintentional defect states, and by phonon stabilization of the hot carriers [Formula: see text] . Additionally, Auger (and/or trap-assisted Auger) scattering above the onset of the plateau may also contribute to longer hot-carrier lifetimes. Meanwhile, the initial decay component shows strong dependence on excitation energy and temperature, reflecting the complicated initial transfer of energy between valence-band and defect states, indicating methods to further prolong hot carriers for technological applications. Nature Publishing Group UK 2021-05-18 /pmc/articles/PMC8131607/ /pubmed/34006905 http://dx.doi.org/10.1038/s41598-021-89815-y Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open AccessThis article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Piyathilaka, Herath P.
Sooriyagoda, Rishmali
Esmaielpour, Hamidreza
Whiteside, Vincent R.
Mishima, Tetsuya D.
Santos, Michael B.
Sellers, Ian R.
Bristow, Alan D.
Hot-carrier dynamics in InAs/AlAsSb multiple-quantum wells
title Hot-carrier dynamics in InAs/AlAsSb multiple-quantum wells
title_full Hot-carrier dynamics in InAs/AlAsSb multiple-quantum wells
title_fullStr Hot-carrier dynamics in InAs/AlAsSb multiple-quantum wells
title_full_unstemmed Hot-carrier dynamics in InAs/AlAsSb multiple-quantum wells
title_short Hot-carrier dynamics in InAs/AlAsSb multiple-quantum wells
title_sort hot-carrier dynamics in inas/alassb multiple-quantum wells
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8131607/
https://www.ncbi.nlm.nih.gov/pubmed/34006905
http://dx.doi.org/10.1038/s41598-021-89815-y
work_keys_str_mv AT piyathilakaherathp hotcarrierdynamicsininasalassbmultiplequantumwells
AT sooriyagodarishmali hotcarrierdynamicsininasalassbmultiplequantumwells
AT esmaielpourhamidreza hotcarrierdynamicsininasalassbmultiplequantumwells
AT whitesidevincentr hotcarrierdynamicsininasalassbmultiplequantumwells
AT mishimatetsuyad hotcarrierdynamicsininasalassbmultiplequantumwells
AT santosmichaelb hotcarrierdynamicsininasalassbmultiplequantumwells
AT sellersianr hotcarrierdynamicsininasalassbmultiplequantumwells
AT bristowaland hotcarrierdynamicsininasalassbmultiplequantumwells