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Fully integrated ultra-sensitive electronic nose based on organic field-effect transistors

Modern solid-state gas sensors approaching ppb-level limit of detection open new perspectives for process control, environmental monitoring and exhaled breath analysis. Organic field-effect transistors (OFETs) are especially promising for gas sensing due to their outstanding sensitivities, low cost...

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Autores principales: Anisimov, Daniil S., Chekusova, Victoria P., Trul, Askold A., Abramov, Anton A., Borshchev, Oleg V., Agina, Elena V., Ponomarenko, Sergey A.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8140082/
https://www.ncbi.nlm.nih.gov/pubmed/34021171
http://dx.doi.org/10.1038/s41598-021-88569-x
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author Anisimov, Daniil S.
Chekusova, Victoria P.
Trul, Askold A.
Abramov, Anton A.
Borshchev, Oleg V.
Agina, Elena V.
Ponomarenko, Sergey A.
author_facet Anisimov, Daniil S.
Chekusova, Victoria P.
Trul, Askold A.
Abramov, Anton A.
Borshchev, Oleg V.
Agina, Elena V.
Ponomarenko, Sergey A.
author_sort Anisimov, Daniil S.
collection PubMed
description Modern solid-state gas sensors approaching ppb-level limit of detection open new perspectives for process control, environmental monitoring and exhaled breath analysis. Organic field-effect transistors (OFETs) are especially promising for gas sensing due to their outstanding sensitivities, low cost and small power consumption. However, they suffer of poor selectivity, requiring development of cross-selective arrays to distinguish analytes, and environmental instability, especially in humid air. Here we present the first fully integrated OFET-based electronic nose with the whole sensor array located on a single substrate. It features down to 30 ppb limit of detection provided by monolayer thick active layers and operates in air with up to 95% relative humidity. By means of principal component analysis, it is able to discriminate toxic air pollutants and monitor meat product freshness. The approach presented paves the way for developing affordable air sensing networks for the Internet of Things.
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spelling pubmed-81400822021-05-25 Fully integrated ultra-sensitive electronic nose based on organic field-effect transistors Anisimov, Daniil S. Chekusova, Victoria P. Trul, Askold A. Abramov, Anton A. Borshchev, Oleg V. Agina, Elena V. Ponomarenko, Sergey A. Sci Rep Article Modern solid-state gas sensors approaching ppb-level limit of detection open new perspectives for process control, environmental monitoring and exhaled breath analysis. Organic field-effect transistors (OFETs) are especially promising for gas sensing due to their outstanding sensitivities, low cost and small power consumption. However, they suffer of poor selectivity, requiring development of cross-selective arrays to distinguish analytes, and environmental instability, especially in humid air. Here we present the first fully integrated OFET-based electronic nose with the whole sensor array located on a single substrate. It features down to 30 ppb limit of detection provided by monolayer thick active layers and operates in air with up to 95% relative humidity. By means of principal component analysis, it is able to discriminate toxic air pollutants and monitor meat product freshness. The approach presented paves the way for developing affordable air sensing networks for the Internet of Things. Nature Publishing Group UK 2021-05-21 /pmc/articles/PMC8140082/ /pubmed/34021171 http://dx.doi.org/10.1038/s41598-021-88569-x Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Anisimov, Daniil S.
Chekusova, Victoria P.
Trul, Askold A.
Abramov, Anton A.
Borshchev, Oleg V.
Agina, Elena V.
Ponomarenko, Sergey A.
Fully integrated ultra-sensitive electronic nose based on organic field-effect transistors
title Fully integrated ultra-sensitive electronic nose based on organic field-effect transistors
title_full Fully integrated ultra-sensitive electronic nose based on organic field-effect transistors
title_fullStr Fully integrated ultra-sensitive electronic nose based on organic field-effect transistors
title_full_unstemmed Fully integrated ultra-sensitive electronic nose based on organic field-effect transistors
title_short Fully integrated ultra-sensitive electronic nose based on organic field-effect transistors
title_sort fully integrated ultra-sensitive electronic nose based on organic field-effect transistors
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8140082/
https://www.ncbi.nlm.nih.gov/pubmed/34021171
http://dx.doi.org/10.1038/s41598-021-88569-x
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