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Sub- and Supercritical Water Gasification of Rice Husk: Parametric Optimization Using the I-Optimality Criterion

[Image: see text] In this study, rice husk biomass was gasified under sub- and supercritical water conditions in an autoclave reactor. The effect of temperature (350–500 °C), residence time (30–120 min), and feed concentration (3–10 wt %) was experimentally studied using the response surface methodo...

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Autores principales: Bakari, Ramadhani, Kivevele, Thomas, Huang, Xiao, Jande, Yusufu A. C.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2021
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8154174/
https://www.ncbi.nlm.nih.gov/pubmed/34056398
http://dx.doi.org/10.1021/acsomega.0c06318
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author Bakari, Ramadhani
Kivevele, Thomas
Huang, Xiao
Jande, Yusufu A. C.
author_facet Bakari, Ramadhani
Kivevele, Thomas
Huang, Xiao
Jande, Yusufu A. C.
author_sort Bakari, Ramadhani
collection PubMed
description [Image: see text] In this study, rice husk biomass was gasified under sub- and supercritical water conditions in an autoclave reactor. The effect of temperature (350–500 °C), residence time (30–120 min), and feed concentration (3–10 wt %) was experimentally studied using the response surface methodology in relation to the yield of gasification products. The quadratic models have been suggested for both responses. Based on the models, the quantitative relationship between various operational conditions and the responses will reliably forecast the experimental outcomes. The findings revealed that higher temperatures, longer residence times, and lower feed concentrations favored high gas yields. The lowest tar yield obtained was 2.98 wt %, while the highest gasification efficiency and gas volume attained were 64.27% and 423 mL/g, respectively. The ANOVA test showed that the order of the effects of the factors on all responses except gravimetric tar yield follows temperature > feed concentration > residence time. The gravimetric tar yield followed a different trend: temperature > residence time > feed concentration. The results revealed that SCW gasification could provide an effective mechanism for transforming the energy content of RH into a substantial fuel product.
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spelling pubmed-81541742021-05-27 Sub- and Supercritical Water Gasification of Rice Husk: Parametric Optimization Using the I-Optimality Criterion Bakari, Ramadhani Kivevele, Thomas Huang, Xiao Jande, Yusufu A. C. ACS Omega [Image: see text] In this study, rice husk biomass was gasified under sub- and supercritical water conditions in an autoclave reactor. The effect of temperature (350–500 °C), residence time (30–120 min), and feed concentration (3–10 wt %) was experimentally studied using the response surface methodology in relation to the yield of gasification products. The quadratic models have been suggested for both responses. Based on the models, the quantitative relationship between various operational conditions and the responses will reliably forecast the experimental outcomes. The findings revealed that higher temperatures, longer residence times, and lower feed concentrations favored high gas yields. The lowest tar yield obtained was 2.98 wt %, while the highest gasification efficiency and gas volume attained were 64.27% and 423 mL/g, respectively. The ANOVA test showed that the order of the effects of the factors on all responses except gravimetric tar yield follows temperature > feed concentration > residence time. The gravimetric tar yield followed a different trend: temperature > residence time > feed concentration. The results revealed that SCW gasification could provide an effective mechanism for transforming the energy content of RH into a substantial fuel product. American Chemical Society 2021-05-04 /pmc/articles/PMC8154174/ /pubmed/34056398 http://dx.doi.org/10.1021/acsomega.0c06318 Text en © 2021 The Authors. Published by American Chemical Society Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Bakari, Ramadhani
Kivevele, Thomas
Huang, Xiao
Jande, Yusufu A. C.
Sub- and Supercritical Water Gasification of Rice Husk: Parametric Optimization Using the I-Optimality Criterion
title Sub- and Supercritical Water Gasification of Rice Husk: Parametric Optimization Using the I-Optimality Criterion
title_full Sub- and Supercritical Water Gasification of Rice Husk: Parametric Optimization Using the I-Optimality Criterion
title_fullStr Sub- and Supercritical Water Gasification of Rice Husk: Parametric Optimization Using the I-Optimality Criterion
title_full_unstemmed Sub- and Supercritical Water Gasification of Rice Husk: Parametric Optimization Using the I-Optimality Criterion
title_short Sub- and Supercritical Water Gasification of Rice Husk: Parametric Optimization Using the I-Optimality Criterion
title_sort sub- and supercritical water gasification of rice husk: parametric optimization using the i-optimality criterion
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8154174/
https://www.ncbi.nlm.nih.gov/pubmed/34056398
http://dx.doi.org/10.1021/acsomega.0c06318
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