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Fano Lineshapes and Rabi Splittings: Can They Be Artificially Generated or Obscured by the Numerical Aperture?

[Image: see text] Fano resonances and Rabi splittings are routinely reported in the scientific literature. Asymmetric resonance lineshapes are usually associated with Fano resonances, and two split peaks in the spectrum are often attributed to a Rabi splitting. True Fano resonances and Rabi splittin...

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Autores principales: Geng, Zhoumuyan, Theenhaus, Johanna, Patra, Biplab K., Zheng, Jian-Yao, Busink, Joris, Garnett, Erik C., Rodriguez, Said R. K.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2021
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8155561/
https://www.ncbi.nlm.nih.gov/pubmed/34056036
http://dx.doi.org/10.1021/acsphotonics.1c00128
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author Geng, Zhoumuyan
Theenhaus, Johanna
Patra, Biplab K.
Zheng, Jian-Yao
Busink, Joris
Garnett, Erik C.
Rodriguez, Said R. K.
author_facet Geng, Zhoumuyan
Theenhaus, Johanna
Patra, Biplab K.
Zheng, Jian-Yao
Busink, Joris
Garnett, Erik C.
Rodriguez, Said R. K.
author_sort Geng, Zhoumuyan
collection PubMed
description [Image: see text] Fano resonances and Rabi splittings are routinely reported in the scientific literature. Asymmetric resonance lineshapes are usually associated with Fano resonances, and two split peaks in the spectrum are often attributed to a Rabi splitting. True Fano resonances and Rabi splittings are unequivocal signatures of coherent coupling between subsystems. However, can the same spectral lineshapes characterizing Fano resonances and Rabi splittings arise from a purely incoherent sum of intensities? Here we answer this question through experiments with a tunable Fabry-Pérot cavity containing a CsPbBr(3) perovskite crystal. By measuring the transmission and photoluminescence of this system using microscope objectives with different numerical aperture (NA), we find that even a modest NA = 0.4 can artificially generate Fano resonances and Rabi splittings. We furthermore show that this modest NA can obscure the anticrossing of a bona fide strongly coupled light–matter system. Through transfer matrix calculations we confirm that these spectral artifacts are due to the incoherent sum of transmitted intensities at different angles captured by the NA. Our results are relevant to the wide nanophotonics community, characterizing dispersive optical systems with high numerical aperture microscope objectives. We conclude with general guidelines to avoid pitfalls in the characterization of such optical systems.
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spelling pubmed-81555612021-05-28 Fano Lineshapes and Rabi Splittings: Can They Be Artificially Generated or Obscured by the Numerical Aperture? Geng, Zhoumuyan Theenhaus, Johanna Patra, Biplab K. Zheng, Jian-Yao Busink, Joris Garnett, Erik C. Rodriguez, Said R. K. ACS Photonics [Image: see text] Fano resonances and Rabi splittings are routinely reported in the scientific literature. Asymmetric resonance lineshapes are usually associated with Fano resonances, and two split peaks in the spectrum are often attributed to a Rabi splitting. True Fano resonances and Rabi splittings are unequivocal signatures of coherent coupling between subsystems. However, can the same spectral lineshapes characterizing Fano resonances and Rabi splittings arise from a purely incoherent sum of intensities? Here we answer this question through experiments with a tunable Fabry-Pérot cavity containing a CsPbBr(3) perovskite crystal. By measuring the transmission and photoluminescence of this system using microscope objectives with different numerical aperture (NA), we find that even a modest NA = 0.4 can artificially generate Fano resonances and Rabi splittings. We furthermore show that this modest NA can obscure the anticrossing of a bona fide strongly coupled light–matter system. Through transfer matrix calculations we confirm that these spectral artifacts are due to the incoherent sum of transmitted intensities at different angles captured by the NA. Our results are relevant to the wide nanophotonics community, characterizing dispersive optical systems with high numerical aperture microscope objectives. We conclude with general guidelines to avoid pitfalls in the characterization of such optical systems. American Chemical Society 2021-05-04 2021-05-19 /pmc/articles/PMC8155561/ /pubmed/34056036 http://dx.doi.org/10.1021/acsphotonics.1c00128 Text en © 2021 The Authors. Published by American Chemical Society Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Geng, Zhoumuyan
Theenhaus, Johanna
Patra, Biplab K.
Zheng, Jian-Yao
Busink, Joris
Garnett, Erik C.
Rodriguez, Said R. K.
Fano Lineshapes and Rabi Splittings: Can They Be Artificially Generated or Obscured by the Numerical Aperture?
title Fano Lineshapes and Rabi Splittings: Can They Be Artificially Generated or Obscured by the Numerical Aperture?
title_full Fano Lineshapes and Rabi Splittings: Can They Be Artificially Generated or Obscured by the Numerical Aperture?
title_fullStr Fano Lineshapes and Rabi Splittings: Can They Be Artificially Generated or Obscured by the Numerical Aperture?
title_full_unstemmed Fano Lineshapes and Rabi Splittings: Can They Be Artificially Generated or Obscured by the Numerical Aperture?
title_short Fano Lineshapes and Rabi Splittings: Can They Be Artificially Generated or Obscured by the Numerical Aperture?
title_sort fano lineshapes and rabi splittings: can they be artificially generated or obscured by the numerical aperture?
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8155561/
https://www.ncbi.nlm.nih.gov/pubmed/34056036
http://dx.doi.org/10.1021/acsphotonics.1c00128
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