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The influence of Coulomb interaction screening on the excitons in disordered two-dimensional insulators

We study the joint effect of disorder and Coulomb interaction screening on the exciton spectra in two-dimensional (2D) structures. These can be van der Waals structures or heterostructures of organic (polymeric) semiconductors as well as inorganic substances like transition metal dichalcogenides. We...

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Autores principales: Kirichenko, E. V., Stephanovich, V. A.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8184999/
https://www.ncbi.nlm.nih.gov/pubmed/34099801
http://dx.doi.org/10.1038/s41598-021-91414-w
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author Kirichenko, E. V.
Stephanovich, V. A.
author_facet Kirichenko, E. V.
Stephanovich, V. A.
author_sort Kirichenko, E. V.
collection PubMed
description We study the joint effect of disorder and Coulomb interaction screening on the exciton spectra in two-dimensional (2D) structures. These can be van der Waals structures or heterostructures of organic (polymeric) semiconductors as well as inorganic substances like transition metal dichalcogenides. We consider 2D screened hydrogenic problem with Rytova–Keldysh interaction by means of so-called fractional Scrödinger equation. Our main finding is that above synergy between screening and disorder either destroys the exciton (strong screening) or promote the creation of a bound state, leading to its collapse in the extreme case. Our second finding is energy levels crossing, i.e. the degeneracy (with respect to index [Formula: see text] ) of the exciton eigenenergies at certain discrete value of screening radius. Latter effects may also be related to the quantum manifestations of chaotic exciton behavior in above 2D semiconductor structures. Hence, they should be considered in device applications, where the interplay between dielectric screening and disorder is important.
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spelling pubmed-81849992021-06-08 The influence of Coulomb interaction screening on the excitons in disordered two-dimensional insulators Kirichenko, E. V. Stephanovich, V. A. Sci Rep Article We study the joint effect of disorder and Coulomb interaction screening on the exciton spectra in two-dimensional (2D) structures. These can be van der Waals structures or heterostructures of organic (polymeric) semiconductors as well as inorganic substances like transition metal dichalcogenides. We consider 2D screened hydrogenic problem with Rytova–Keldysh interaction by means of so-called fractional Scrödinger equation. Our main finding is that above synergy between screening and disorder either destroys the exciton (strong screening) or promote the creation of a bound state, leading to its collapse in the extreme case. Our second finding is energy levels crossing, i.e. the degeneracy (with respect to index [Formula: see text] ) of the exciton eigenenergies at certain discrete value of screening radius. Latter effects may also be related to the quantum manifestations of chaotic exciton behavior in above 2D semiconductor structures. Hence, they should be considered in device applications, where the interplay between dielectric screening and disorder is important. Nature Publishing Group UK 2021-06-07 /pmc/articles/PMC8184999/ /pubmed/34099801 http://dx.doi.org/10.1038/s41598-021-91414-w Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open AccessThis article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Kirichenko, E. V.
Stephanovich, V. A.
The influence of Coulomb interaction screening on the excitons in disordered two-dimensional insulators
title The influence of Coulomb interaction screening on the excitons in disordered two-dimensional insulators
title_full The influence of Coulomb interaction screening on the excitons in disordered two-dimensional insulators
title_fullStr The influence of Coulomb interaction screening on the excitons in disordered two-dimensional insulators
title_full_unstemmed The influence of Coulomb interaction screening on the excitons in disordered two-dimensional insulators
title_short The influence of Coulomb interaction screening on the excitons in disordered two-dimensional insulators
title_sort influence of coulomb interaction screening on the excitons in disordered two-dimensional insulators
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8184999/
https://www.ncbi.nlm.nih.gov/pubmed/34099801
http://dx.doi.org/10.1038/s41598-021-91414-w
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