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Global tropospheric ozone responses to reduced NO(x) emissions linked to the COVID-19 worldwide lockdowns

Efforts to stem the transmission of coronavirus disease 2019 (COVID-19) led to rapid, global ancillary reductions in air pollutant emissions. Here, we quantify the impact on tropospheric ozone using a multiconstituent chemical data assimilation system. Anthropogenic NO(x) emissions dropped by at lea...

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Detalles Bibliográficos
Autores principales: Miyazaki, Kazuyuki, Bowman, Kevin, Sekiya, Takashi, Takigawa, Masayuki, Neu, Jessica L., Sudo, Kengo, Osterman, Greg, Eskes, Henk
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8189586/
https://www.ncbi.nlm.nih.gov/pubmed/34108210
http://dx.doi.org/10.1126/sciadv.abf7460
Descripción
Sumario:Efforts to stem the transmission of coronavirus disease 2019 (COVID-19) led to rapid, global ancillary reductions in air pollutant emissions. Here, we quantify the impact on tropospheric ozone using a multiconstituent chemical data assimilation system. Anthropogenic NO(x) emissions dropped by at least 15% globally and 18 to 25% regionally in April and May 2020, which decreased free tropospheric ozone by up to 5 parts per billion, consistent with independent satellite observations. The global total tropospheric ozone burden declined by 6TgO(3) (∼2%) in May and June 2020, largely due to emission reductions in Asia and the Americas that were amplified by regionally high ozone production efficiencies (up to 4 TgO(3)/TgN). Our results show that COVID-19 mitigation left a global atmospheric imprint that altered atmospheric oxidative capacity and climate radiative forcing, providing a test of the efficacy of NO(x) emissions controls for co-benefiting air quality and climate.