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Global tropospheric ozone responses to reduced NO(x) emissions linked to the COVID-19 worldwide lockdowns

Efforts to stem the transmission of coronavirus disease 2019 (COVID-19) led to rapid, global ancillary reductions in air pollutant emissions. Here, we quantify the impact on tropospheric ozone using a multiconstituent chemical data assimilation system. Anthropogenic NO(x) emissions dropped by at lea...

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Autores principales: Miyazaki, Kazuyuki, Bowman, Kevin, Sekiya, Takashi, Takigawa, Masayuki, Neu, Jessica L., Sudo, Kengo, Osterman, Greg, Eskes, Henk
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8189586/
https://www.ncbi.nlm.nih.gov/pubmed/34108210
http://dx.doi.org/10.1126/sciadv.abf7460
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author Miyazaki, Kazuyuki
Bowman, Kevin
Sekiya, Takashi
Takigawa, Masayuki
Neu, Jessica L.
Sudo, Kengo
Osterman, Greg
Eskes, Henk
author_facet Miyazaki, Kazuyuki
Bowman, Kevin
Sekiya, Takashi
Takigawa, Masayuki
Neu, Jessica L.
Sudo, Kengo
Osterman, Greg
Eskes, Henk
author_sort Miyazaki, Kazuyuki
collection PubMed
description Efforts to stem the transmission of coronavirus disease 2019 (COVID-19) led to rapid, global ancillary reductions in air pollutant emissions. Here, we quantify the impact on tropospheric ozone using a multiconstituent chemical data assimilation system. Anthropogenic NO(x) emissions dropped by at least 15% globally and 18 to 25% regionally in April and May 2020, which decreased free tropospheric ozone by up to 5 parts per billion, consistent with independent satellite observations. The global total tropospheric ozone burden declined by 6TgO(3) (∼2%) in May and June 2020, largely due to emission reductions in Asia and the Americas that were amplified by regionally high ozone production efficiencies (up to 4 TgO(3)/TgN). Our results show that COVID-19 mitigation left a global atmospheric imprint that altered atmospheric oxidative capacity and climate radiative forcing, providing a test of the efficacy of NO(x) emissions controls for co-benefiting air quality and climate.
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spelling pubmed-81895862021-06-22 Global tropospheric ozone responses to reduced NO(x) emissions linked to the COVID-19 worldwide lockdowns Miyazaki, Kazuyuki Bowman, Kevin Sekiya, Takashi Takigawa, Masayuki Neu, Jessica L. Sudo, Kengo Osterman, Greg Eskes, Henk Sci Adv Research Articles Efforts to stem the transmission of coronavirus disease 2019 (COVID-19) led to rapid, global ancillary reductions in air pollutant emissions. Here, we quantify the impact on tropospheric ozone using a multiconstituent chemical data assimilation system. Anthropogenic NO(x) emissions dropped by at least 15% globally and 18 to 25% regionally in April and May 2020, which decreased free tropospheric ozone by up to 5 parts per billion, consistent with independent satellite observations. The global total tropospheric ozone burden declined by 6TgO(3) (∼2%) in May and June 2020, largely due to emission reductions in Asia and the Americas that were amplified by regionally high ozone production efficiencies (up to 4 TgO(3)/TgN). Our results show that COVID-19 mitigation left a global atmospheric imprint that altered atmospheric oxidative capacity and climate radiative forcing, providing a test of the efficacy of NO(x) emissions controls for co-benefiting air quality and climate. American Association for the Advancement of Science 2021-06-09 /pmc/articles/PMC8189586/ /pubmed/34108210 http://dx.doi.org/10.1126/sciadv.abf7460 Text en Copyright © 2021 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution License 4.0 (CC BY). https://creativecommons.org/licenses/by/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution license (https://creativecommons.org/licenses/by/4.0/) , which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.
spellingShingle Research Articles
Miyazaki, Kazuyuki
Bowman, Kevin
Sekiya, Takashi
Takigawa, Masayuki
Neu, Jessica L.
Sudo, Kengo
Osterman, Greg
Eskes, Henk
Global tropospheric ozone responses to reduced NO(x) emissions linked to the COVID-19 worldwide lockdowns
title Global tropospheric ozone responses to reduced NO(x) emissions linked to the COVID-19 worldwide lockdowns
title_full Global tropospheric ozone responses to reduced NO(x) emissions linked to the COVID-19 worldwide lockdowns
title_fullStr Global tropospheric ozone responses to reduced NO(x) emissions linked to the COVID-19 worldwide lockdowns
title_full_unstemmed Global tropospheric ozone responses to reduced NO(x) emissions linked to the COVID-19 worldwide lockdowns
title_short Global tropospheric ozone responses to reduced NO(x) emissions linked to the COVID-19 worldwide lockdowns
title_sort global tropospheric ozone responses to reduced no(x) emissions linked to the covid-19 worldwide lockdowns
topic Research Articles
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8189586/
https://www.ncbi.nlm.nih.gov/pubmed/34108210
http://dx.doi.org/10.1126/sciadv.abf7460
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