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One-Step Construction of Multi-Walled CNTs Loaded with Alpha-Fe(2)O(3) Nanoparticles for Efficient Photocatalytic Properties

The aggregation and the rapid restructuring of the photoinduced electron−hole pairs restructuring in the process of photoelectric response remains a great challenge. In this study, a kind of Multi-walled carbon nanotubes loaded Alpha-Fe(2)O(3) (CNTs/α-Fe(2)O(3)) heterostructure composite is successf...

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Detalles Bibliográficos
Autores principales: Xu, Jianle, Wen, Qiang, Zhang, Xiao, Li, Yinhui, Cui, Zeyue, Li, Pengwei, Pan, Chunxu
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8199084/
https://www.ncbi.nlm.nih.gov/pubmed/34070510
http://dx.doi.org/10.3390/ma14112820
Descripción
Sumario:The aggregation and the rapid restructuring of the photoinduced electron−hole pairs restructuring in the process of photoelectric response remains a great challenge. In this study, a kind of Multi-walled carbon nanotubes loaded Alpha-Fe(2)O(3) (CNTs/α-Fe(2)O(3)) heterostructure composite is successfully prepared via the one-step method. Due to the synergistic effect in the as-prepared CNTs/α-Fe(2)O(3), the defect sites and oxygen-containing functional groups of CNTs can dramatically improve the interface charge separation efficiency and prevent the aggregation of α-Fe(2)O(3). The improved photocurrent and enhanced hole–electron separation rate in the CNTs/α-Fe(2)O(3) is obtained, and the narrower band gap is measured to be 2.8 ev with intensive visible-light absorption performance. Thus, the CNTs/α-Fe(2)O(3) composite serves as an excellent visible light photocatalyst and exhibits an outstanding photocatalytic activity for the cationic dye degradation of rhodamine B (RhB). This research supplies a fresh application area forα-Fe(2)O(3) photocatalyst and initiates a new approach for design of high efficiency photocatalytic materials.