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One-Step Construction of Multi-Walled CNTs Loaded with Alpha-Fe(2)O(3) Nanoparticles for Efficient Photocatalytic Properties

The aggregation and the rapid restructuring of the photoinduced electron−hole pairs restructuring in the process of photoelectric response remains a great challenge. In this study, a kind of Multi-walled carbon nanotubes loaded Alpha-Fe(2)O(3) (CNTs/α-Fe(2)O(3)) heterostructure composite is successf...

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Autores principales: Xu, Jianle, Wen, Qiang, Zhang, Xiao, Li, Yinhui, Cui, Zeyue, Li, Pengwei, Pan, Chunxu
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8199084/
https://www.ncbi.nlm.nih.gov/pubmed/34070510
http://dx.doi.org/10.3390/ma14112820
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author Xu, Jianle
Wen, Qiang
Zhang, Xiao
Li, Yinhui
Cui, Zeyue
Li, Pengwei
Pan, Chunxu
author_facet Xu, Jianle
Wen, Qiang
Zhang, Xiao
Li, Yinhui
Cui, Zeyue
Li, Pengwei
Pan, Chunxu
author_sort Xu, Jianle
collection PubMed
description The aggregation and the rapid restructuring of the photoinduced electron−hole pairs restructuring in the process of photoelectric response remains a great challenge. In this study, a kind of Multi-walled carbon nanotubes loaded Alpha-Fe(2)O(3) (CNTs/α-Fe(2)O(3)) heterostructure composite is successfully prepared via the one-step method. Due to the synergistic effect in the as-prepared CNTs/α-Fe(2)O(3), the defect sites and oxygen-containing functional groups of CNTs can dramatically improve the interface charge separation efficiency and prevent the aggregation of α-Fe(2)O(3). The improved photocurrent and enhanced hole–electron separation rate in the CNTs/α-Fe(2)O(3) is obtained, and the narrower band gap is measured to be 2.8 ev with intensive visible-light absorption performance. Thus, the CNTs/α-Fe(2)O(3) composite serves as an excellent visible light photocatalyst and exhibits an outstanding photocatalytic activity for the cationic dye degradation of rhodamine B (RhB). This research supplies a fresh application area forα-Fe(2)O(3) photocatalyst and initiates a new approach for design of high efficiency photocatalytic materials.
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spelling pubmed-81990842021-06-14 One-Step Construction of Multi-Walled CNTs Loaded with Alpha-Fe(2)O(3) Nanoparticles for Efficient Photocatalytic Properties Xu, Jianle Wen, Qiang Zhang, Xiao Li, Yinhui Cui, Zeyue Li, Pengwei Pan, Chunxu Materials (Basel) Article The aggregation and the rapid restructuring of the photoinduced electron−hole pairs restructuring in the process of photoelectric response remains a great challenge. In this study, a kind of Multi-walled carbon nanotubes loaded Alpha-Fe(2)O(3) (CNTs/α-Fe(2)O(3)) heterostructure composite is successfully prepared via the one-step method. Due to the synergistic effect in the as-prepared CNTs/α-Fe(2)O(3), the defect sites and oxygen-containing functional groups of CNTs can dramatically improve the interface charge separation efficiency and prevent the aggregation of α-Fe(2)O(3). The improved photocurrent and enhanced hole–electron separation rate in the CNTs/α-Fe(2)O(3) is obtained, and the narrower band gap is measured to be 2.8 ev with intensive visible-light absorption performance. Thus, the CNTs/α-Fe(2)O(3) composite serves as an excellent visible light photocatalyst and exhibits an outstanding photocatalytic activity for the cationic dye degradation of rhodamine B (RhB). This research supplies a fresh application area forα-Fe(2)O(3) photocatalyst and initiates a new approach for design of high efficiency photocatalytic materials. MDPI 2021-05-25 /pmc/articles/PMC8199084/ /pubmed/34070510 http://dx.doi.org/10.3390/ma14112820 Text en © 2021 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Xu, Jianle
Wen, Qiang
Zhang, Xiao
Li, Yinhui
Cui, Zeyue
Li, Pengwei
Pan, Chunxu
One-Step Construction of Multi-Walled CNTs Loaded with Alpha-Fe(2)O(3) Nanoparticles for Efficient Photocatalytic Properties
title One-Step Construction of Multi-Walled CNTs Loaded with Alpha-Fe(2)O(3) Nanoparticles for Efficient Photocatalytic Properties
title_full One-Step Construction of Multi-Walled CNTs Loaded with Alpha-Fe(2)O(3) Nanoparticles for Efficient Photocatalytic Properties
title_fullStr One-Step Construction of Multi-Walled CNTs Loaded with Alpha-Fe(2)O(3) Nanoparticles for Efficient Photocatalytic Properties
title_full_unstemmed One-Step Construction of Multi-Walled CNTs Loaded with Alpha-Fe(2)O(3) Nanoparticles for Efficient Photocatalytic Properties
title_short One-Step Construction of Multi-Walled CNTs Loaded with Alpha-Fe(2)O(3) Nanoparticles for Efficient Photocatalytic Properties
title_sort one-step construction of multi-walled cnts loaded with alpha-fe(2)o(3) nanoparticles for efficient photocatalytic properties
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8199084/
https://www.ncbi.nlm.nih.gov/pubmed/34070510
http://dx.doi.org/10.3390/ma14112820
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