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One-Step Construction of Multi-Walled CNTs Loaded with Alpha-Fe(2)O(3) Nanoparticles for Efficient Photocatalytic Properties
The aggregation and the rapid restructuring of the photoinduced electron−hole pairs restructuring in the process of photoelectric response remains a great challenge. In this study, a kind of Multi-walled carbon nanotubes loaded Alpha-Fe(2)O(3) (CNTs/α-Fe(2)O(3)) heterostructure composite is successf...
Autores principales: | , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
MDPI
2021
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8199084/ https://www.ncbi.nlm.nih.gov/pubmed/34070510 http://dx.doi.org/10.3390/ma14112820 |
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author | Xu, Jianle Wen, Qiang Zhang, Xiao Li, Yinhui Cui, Zeyue Li, Pengwei Pan, Chunxu |
author_facet | Xu, Jianle Wen, Qiang Zhang, Xiao Li, Yinhui Cui, Zeyue Li, Pengwei Pan, Chunxu |
author_sort | Xu, Jianle |
collection | PubMed |
description | The aggregation and the rapid restructuring of the photoinduced electron−hole pairs restructuring in the process of photoelectric response remains a great challenge. In this study, a kind of Multi-walled carbon nanotubes loaded Alpha-Fe(2)O(3) (CNTs/α-Fe(2)O(3)) heterostructure composite is successfully prepared via the one-step method. Due to the synergistic effect in the as-prepared CNTs/α-Fe(2)O(3), the defect sites and oxygen-containing functional groups of CNTs can dramatically improve the interface charge separation efficiency and prevent the aggregation of α-Fe(2)O(3). The improved photocurrent and enhanced hole–electron separation rate in the CNTs/α-Fe(2)O(3) is obtained, and the narrower band gap is measured to be 2.8 ev with intensive visible-light absorption performance. Thus, the CNTs/α-Fe(2)O(3) composite serves as an excellent visible light photocatalyst and exhibits an outstanding photocatalytic activity for the cationic dye degradation of rhodamine B (RhB). This research supplies a fresh application area forα-Fe(2)O(3) photocatalyst and initiates a new approach for design of high efficiency photocatalytic materials. |
format | Online Article Text |
id | pubmed-8199084 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | MDPI |
record_format | MEDLINE/PubMed |
spelling | pubmed-81990842021-06-14 One-Step Construction of Multi-Walled CNTs Loaded with Alpha-Fe(2)O(3) Nanoparticles for Efficient Photocatalytic Properties Xu, Jianle Wen, Qiang Zhang, Xiao Li, Yinhui Cui, Zeyue Li, Pengwei Pan, Chunxu Materials (Basel) Article The aggregation and the rapid restructuring of the photoinduced electron−hole pairs restructuring in the process of photoelectric response remains a great challenge. In this study, a kind of Multi-walled carbon nanotubes loaded Alpha-Fe(2)O(3) (CNTs/α-Fe(2)O(3)) heterostructure composite is successfully prepared via the one-step method. Due to the synergistic effect in the as-prepared CNTs/α-Fe(2)O(3), the defect sites and oxygen-containing functional groups of CNTs can dramatically improve the interface charge separation efficiency and prevent the aggregation of α-Fe(2)O(3). The improved photocurrent and enhanced hole–electron separation rate in the CNTs/α-Fe(2)O(3) is obtained, and the narrower band gap is measured to be 2.8 ev with intensive visible-light absorption performance. Thus, the CNTs/α-Fe(2)O(3) composite serves as an excellent visible light photocatalyst and exhibits an outstanding photocatalytic activity for the cationic dye degradation of rhodamine B (RhB). This research supplies a fresh application area forα-Fe(2)O(3) photocatalyst and initiates a new approach for design of high efficiency photocatalytic materials. MDPI 2021-05-25 /pmc/articles/PMC8199084/ /pubmed/34070510 http://dx.doi.org/10.3390/ma14112820 Text en © 2021 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Article Xu, Jianle Wen, Qiang Zhang, Xiao Li, Yinhui Cui, Zeyue Li, Pengwei Pan, Chunxu One-Step Construction of Multi-Walled CNTs Loaded with Alpha-Fe(2)O(3) Nanoparticles for Efficient Photocatalytic Properties |
title | One-Step Construction of Multi-Walled CNTs Loaded with Alpha-Fe(2)O(3) Nanoparticles for Efficient Photocatalytic Properties |
title_full | One-Step Construction of Multi-Walled CNTs Loaded with Alpha-Fe(2)O(3) Nanoparticles for Efficient Photocatalytic Properties |
title_fullStr | One-Step Construction of Multi-Walled CNTs Loaded with Alpha-Fe(2)O(3) Nanoparticles for Efficient Photocatalytic Properties |
title_full_unstemmed | One-Step Construction of Multi-Walled CNTs Loaded with Alpha-Fe(2)O(3) Nanoparticles for Efficient Photocatalytic Properties |
title_short | One-Step Construction of Multi-Walled CNTs Loaded with Alpha-Fe(2)O(3) Nanoparticles for Efficient Photocatalytic Properties |
title_sort | one-step construction of multi-walled cnts loaded with alpha-fe(2)o(3) nanoparticles for efficient photocatalytic properties |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8199084/ https://www.ncbi.nlm.nih.gov/pubmed/34070510 http://dx.doi.org/10.3390/ma14112820 |
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