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US COVID‐19 Shutdown Demonstrates Importance of Background NO(2) in Inferring NO(x) Emissions From Satellite NO(2) Observations

Satellite nitrogen dioxide (NO(2)) measurements are used extensively to infer nitrogen oxide emissions and their trends, but interpretation can be complicated by background contributions to the NO(2) column sensed from space. We use the step decrease of US anthropogenic emissions from the COVID‐19 s...

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Autores principales: Qu, Zhen, Jacob, Daniel J., Silvern, Rachel F., Shah, Viral, Campbell, Patrick C., Valin, Lukas C., Murray, Lee T.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: John Wiley and Sons Inc. 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8206743/
https://www.ncbi.nlm.nih.gov/pubmed/34149109
http://dx.doi.org/10.1029/2021GL092783
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author Qu, Zhen
Jacob, Daniel J.
Silvern, Rachel F.
Shah, Viral
Campbell, Patrick C.
Valin, Lukas C.
Murray, Lee T.
author_facet Qu, Zhen
Jacob, Daniel J.
Silvern, Rachel F.
Shah, Viral
Campbell, Patrick C.
Valin, Lukas C.
Murray, Lee T.
author_sort Qu, Zhen
collection PubMed
description Satellite nitrogen dioxide (NO(2)) measurements are used extensively to infer nitrogen oxide emissions and their trends, but interpretation can be complicated by background contributions to the NO(2) column sensed from space. We use the step decrease of US anthropogenic emissions from the COVID‐19 shutdown to compare the responses of NO(2) concentrations observed at surface network sites and from satellites (Ozone Monitoring Instrument [OMI], Tropospheric Ozone Monitoring Instrument [TROPOMI]). After correcting for differences in meteorology, surface NO(2) measurements for 2020 show decreases of 20% in March–April and 10% in May–August compared to 2019. The satellites show much weaker responses in March–June and no decrease in July–August, consistent with a large background contribution to the NO(2) column. Inspection of the long‐term OMI trend over remote US regions shows a rising summertime NO(2) background from 2010 to 2019 potentially attributable to wildfires.
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spelling pubmed-82067432021-06-16 US COVID‐19 Shutdown Demonstrates Importance of Background NO(2) in Inferring NO(x) Emissions From Satellite NO(2) Observations Qu, Zhen Jacob, Daniel J. Silvern, Rachel F. Shah, Viral Campbell, Patrick C. Valin, Lukas C. Murray, Lee T. Geophys Res Lett Research Letter Satellite nitrogen dioxide (NO(2)) measurements are used extensively to infer nitrogen oxide emissions and their trends, but interpretation can be complicated by background contributions to the NO(2) column sensed from space. We use the step decrease of US anthropogenic emissions from the COVID‐19 shutdown to compare the responses of NO(2) concentrations observed at surface network sites and from satellites (Ozone Monitoring Instrument [OMI], Tropospheric Ozone Monitoring Instrument [TROPOMI]). After correcting for differences in meteorology, surface NO(2) measurements for 2020 show decreases of 20% in March–April and 10% in May–August compared to 2019. The satellites show much weaker responses in March–June and no decrease in July–August, consistent with a large background contribution to the NO(2) column. Inspection of the long‐term OMI trend over remote US regions shows a rising summertime NO(2) background from 2010 to 2019 potentially attributable to wildfires. John Wiley and Sons Inc. 2021-05-18 2021-05-28 /pmc/articles/PMC8206743/ /pubmed/34149109 http://dx.doi.org/10.1029/2021GL092783 Text en © 2021. The Authors. https://creativecommons.org/licenses/by-nc/4.0/This is an open access article under the terms of the http://creativecommons.org/licenses/by-nc/4.0/ (https://creativecommons.org/licenses/by-nc/4.0/) License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited and is not used for commercial purposes.
spellingShingle Research Letter
Qu, Zhen
Jacob, Daniel J.
Silvern, Rachel F.
Shah, Viral
Campbell, Patrick C.
Valin, Lukas C.
Murray, Lee T.
US COVID‐19 Shutdown Demonstrates Importance of Background NO(2) in Inferring NO(x) Emissions From Satellite NO(2) Observations
title US COVID‐19 Shutdown Demonstrates Importance of Background NO(2) in Inferring NO(x) Emissions From Satellite NO(2) Observations
title_full US COVID‐19 Shutdown Demonstrates Importance of Background NO(2) in Inferring NO(x) Emissions From Satellite NO(2) Observations
title_fullStr US COVID‐19 Shutdown Demonstrates Importance of Background NO(2) in Inferring NO(x) Emissions From Satellite NO(2) Observations
title_full_unstemmed US COVID‐19 Shutdown Demonstrates Importance of Background NO(2) in Inferring NO(x) Emissions From Satellite NO(2) Observations
title_short US COVID‐19 Shutdown Demonstrates Importance of Background NO(2) in Inferring NO(x) Emissions From Satellite NO(2) Observations
title_sort us covid‐19 shutdown demonstrates importance of background no(2) in inferring no(x) emissions from satellite no(2) observations
topic Research Letter
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8206743/
https://www.ncbi.nlm.nih.gov/pubmed/34149109
http://dx.doi.org/10.1029/2021GL092783
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