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Position-controlled quantum emitters with reproducible emission wavelength in hexagonal boron nitride

Single photon emitters (SPEs) in low-dimensional layered materials have recently gained a large interest owing to the auspicious perspectives of integration and extreme miniaturization offered by this class of materials. However, accurate control of both the spatial location and the emission wavelen...

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Autores principales: Fournier, Clarisse, Plaud, Alexandre, Roux, Sébastien, Pierret, Aurélie, Rosticher, Michael, Watanabe, Kenji, Taniguchi, Takashi, Buil, Stéphanie, Quélin, Xavier, Barjon, Julien, Hermier, Jean-Pierre, Delteil, Aymeric
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8213715/
https://www.ncbi.nlm.nih.gov/pubmed/34145254
http://dx.doi.org/10.1038/s41467-021-24019-6
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author Fournier, Clarisse
Plaud, Alexandre
Roux, Sébastien
Pierret, Aurélie
Rosticher, Michael
Watanabe, Kenji
Taniguchi, Takashi
Buil, Stéphanie
Quélin, Xavier
Barjon, Julien
Hermier, Jean-Pierre
Delteil, Aymeric
author_facet Fournier, Clarisse
Plaud, Alexandre
Roux, Sébastien
Pierret, Aurélie
Rosticher, Michael
Watanabe, Kenji
Taniguchi, Takashi
Buil, Stéphanie
Quélin, Xavier
Barjon, Julien
Hermier, Jean-Pierre
Delteil, Aymeric
author_sort Fournier, Clarisse
collection PubMed
description Single photon emitters (SPEs) in low-dimensional layered materials have recently gained a large interest owing to the auspicious perspectives of integration and extreme miniaturization offered by this class of materials. However, accurate control of both the spatial location and the emission wavelength of the quantum emitters is essentially lacking to date, thus hindering further technological steps towards scalable quantum photonic devices. Here, we evidence SPEs in high purity synthetic hexagonal boron nitride (hBN) that can be activated by an electron beam at chosen locations. SPE ensembles are generated with a spatial accuracy better than the cubed emission wavelength, thus opening the way to integration in optical microstructures. Stable and bright single photon emission is subsequently observed in the visible range up to room temperature upon non-resonant laser excitation. Moreover, the low-temperature emission wavelength is reproducible, with an ensemble distribution of width 3 meV, a statistical dispersion that is more than one order of magnitude lower than the narrowest wavelength spreads obtained in epitaxial hBN samples. Our findings constitute an essential step towards the realization of top-down integrated devices based on identical quantum emitters in 2D materials.
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spelling pubmed-82137152021-07-01 Position-controlled quantum emitters with reproducible emission wavelength in hexagonal boron nitride Fournier, Clarisse Plaud, Alexandre Roux, Sébastien Pierret, Aurélie Rosticher, Michael Watanabe, Kenji Taniguchi, Takashi Buil, Stéphanie Quélin, Xavier Barjon, Julien Hermier, Jean-Pierre Delteil, Aymeric Nat Commun Article Single photon emitters (SPEs) in low-dimensional layered materials have recently gained a large interest owing to the auspicious perspectives of integration and extreme miniaturization offered by this class of materials. However, accurate control of both the spatial location and the emission wavelength of the quantum emitters is essentially lacking to date, thus hindering further technological steps towards scalable quantum photonic devices. Here, we evidence SPEs in high purity synthetic hexagonal boron nitride (hBN) that can be activated by an electron beam at chosen locations. SPE ensembles are generated with a spatial accuracy better than the cubed emission wavelength, thus opening the way to integration in optical microstructures. Stable and bright single photon emission is subsequently observed in the visible range up to room temperature upon non-resonant laser excitation. Moreover, the low-temperature emission wavelength is reproducible, with an ensemble distribution of width 3 meV, a statistical dispersion that is more than one order of magnitude lower than the narrowest wavelength spreads obtained in epitaxial hBN samples. Our findings constitute an essential step towards the realization of top-down integrated devices based on identical quantum emitters in 2D materials. Nature Publishing Group UK 2021-06-18 /pmc/articles/PMC8213715/ /pubmed/34145254 http://dx.doi.org/10.1038/s41467-021-24019-6 Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Fournier, Clarisse
Plaud, Alexandre
Roux, Sébastien
Pierret, Aurélie
Rosticher, Michael
Watanabe, Kenji
Taniguchi, Takashi
Buil, Stéphanie
Quélin, Xavier
Barjon, Julien
Hermier, Jean-Pierre
Delteil, Aymeric
Position-controlled quantum emitters with reproducible emission wavelength in hexagonal boron nitride
title Position-controlled quantum emitters with reproducible emission wavelength in hexagonal boron nitride
title_full Position-controlled quantum emitters with reproducible emission wavelength in hexagonal boron nitride
title_fullStr Position-controlled quantum emitters with reproducible emission wavelength in hexagonal boron nitride
title_full_unstemmed Position-controlled quantum emitters with reproducible emission wavelength in hexagonal boron nitride
title_short Position-controlled quantum emitters with reproducible emission wavelength in hexagonal boron nitride
title_sort position-controlled quantum emitters with reproducible emission wavelength in hexagonal boron nitride
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8213715/
https://www.ncbi.nlm.nih.gov/pubmed/34145254
http://dx.doi.org/10.1038/s41467-021-24019-6
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