Cargando…
Atomically-resolved interlayer charge ordering and its interplay with superconductivity in YBa(2)Cu(3)O(6.81)
High-temperature superconductive (SC) cuprates exhibit not only a SC phase, but also competing orders, suppressing superconductivity. Charge order (CO) has been recognized as an important competing order, but its microscopic spatial interplay with SC phase as well as the interlayer coupling in CO an...
Autores principales: | , , , , , , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2021
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8222377/ https://www.ncbi.nlm.nih.gov/pubmed/34162864 http://dx.doi.org/10.1038/s41467-021-24003-0 |
_version_ | 1783711484011872256 |
---|---|
author | Hsu, Chun-Chih Huang, Bo-Chao Schnedler, Michael Lai, Ming-Yu Wang, Yuh-Lin Dunin-Borkowski, Rafal E. Chang, Chia-Seng Lee, Ting-Kuo Ebert, Philipp Chiu, Ya-Ping |
author_facet | Hsu, Chun-Chih Huang, Bo-Chao Schnedler, Michael Lai, Ming-Yu Wang, Yuh-Lin Dunin-Borkowski, Rafal E. Chang, Chia-Seng Lee, Ting-Kuo Ebert, Philipp Chiu, Ya-Ping |
author_sort | Hsu, Chun-Chih |
collection | PubMed |
description | High-temperature superconductive (SC) cuprates exhibit not only a SC phase, but also competing orders, suppressing superconductivity. Charge order (CO) has been recognized as an important competing order, but its microscopic spatial interplay with SC phase as well as the interlayer coupling in CO and SC phases remain elusive, despite being essential for understanding the physical mechanisms of competing orders and hence superconductivity. Here we report the achievement of direct real-space imaging with atomic-scale resolution of cryogenically cleaved YBa(2)Cu(3)O(6.81) using cross-sectional scanning tunneling microscopy/spectroscopy. CO nanodomains are found embedded in the SC phase with a proximity-like boundary region characterized by mutual suppression of CO and superconductivity. Furthermore, SC coherence as well as CO occur on both CuO chain and plane layers, revealing carrier transport and density of states mixing between layers. The CO antiphase correlation along the c direction suggests a dominance of Coulomb repulsion over Josephson tunneling between adjacent layers. |
format | Online Article Text |
id | pubmed-8222377 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-82223772021-07-09 Atomically-resolved interlayer charge ordering and its interplay with superconductivity in YBa(2)Cu(3)O(6.81) Hsu, Chun-Chih Huang, Bo-Chao Schnedler, Michael Lai, Ming-Yu Wang, Yuh-Lin Dunin-Borkowski, Rafal E. Chang, Chia-Seng Lee, Ting-Kuo Ebert, Philipp Chiu, Ya-Ping Nat Commun Article High-temperature superconductive (SC) cuprates exhibit not only a SC phase, but also competing orders, suppressing superconductivity. Charge order (CO) has been recognized as an important competing order, but its microscopic spatial interplay with SC phase as well as the interlayer coupling in CO and SC phases remain elusive, despite being essential for understanding the physical mechanisms of competing orders and hence superconductivity. Here we report the achievement of direct real-space imaging with atomic-scale resolution of cryogenically cleaved YBa(2)Cu(3)O(6.81) using cross-sectional scanning tunneling microscopy/spectroscopy. CO nanodomains are found embedded in the SC phase with a proximity-like boundary region characterized by mutual suppression of CO and superconductivity. Furthermore, SC coherence as well as CO occur on both CuO chain and plane layers, revealing carrier transport and density of states mixing between layers. The CO antiphase correlation along the c direction suggests a dominance of Coulomb repulsion over Josephson tunneling between adjacent layers. Nature Publishing Group UK 2021-06-23 /pmc/articles/PMC8222377/ /pubmed/34162864 http://dx.doi.org/10.1038/s41467-021-24003-0 Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Hsu, Chun-Chih Huang, Bo-Chao Schnedler, Michael Lai, Ming-Yu Wang, Yuh-Lin Dunin-Borkowski, Rafal E. Chang, Chia-Seng Lee, Ting-Kuo Ebert, Philipp Chiu, Ya-Ping Atomically-resolved interlayer charge ordering and its interplay with superconductivity in YBa(2)Cu(3)O(6.81) |
title | Atomically-resolved interlayer charge ordering and its interplay with superconductivity in YBa(2)Cu(3)O(6.81) |
title_full | Atomically-resolved interlayer charge ordering and its interplay with superconductivity in YBa(2)Cu(3)O(6.81) |
title_fullStr | Atomically-resolved interlayer charge ordering and its interplay with superconductivity in YBa(2)Cu(3)O(6.81) |
title_full_unstemmed | Atomically-resolved interlayer charge ordering and its interplay with superconductivity in YBa(2)Cu(3)O(6.81) |
title_short | Atomically-resolved interlayer charge ordering and its interplay with superconductivity in YBa(2)Cu(3)O(6.81) |
title_sort | atomically-resolved interlayer charge ordering and its interplay with superconductivity in yba(2)cu(3)o(6.81) |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8222377/ https://www.ncbi.nlm.nih.gov/pubmed/34162864 http://dx.doi.org/10.1038/s41467-021-24003-0 |
work_keys_str_mv | AT hsuchunchih atomicallyresolvedinterlayerchargeorderinganditsinterplaywithsuperconductivityinyba2cu3o681 AT huangbochao atomicallyresolvedinterlayerchargeorderinganditsinterplaywithsuperconductivityinyba2cu3o681 AT schnedlermichael atomicallyresolvedinterlayerchargeorderinganditsinterplaywithsuperconductivityinyba2cu3o681 AT laimingyu atomicallyresolvedinterlayerchargeorderinganditsinterplaywithsuperconductivityinyba2cu3o681 AT wangyuhlin atomicallyresolvedinterlayerchargeorderinganditsinterplaywithsuperconductivityinyba2cu3o681 AT duninborkowskirafale atomicallyresolvedinterlayerchargeorderinganditsinterplaywithsuperconductivityinyba2cu3o681 AT changchiaseng atomicallyresolvedinterlayerchargeorderinganditsinterplaywithsuperconductivityinyba2cu3o681 AT leetingkuo atomicallyresolvedinterlayerchargeorderinganditsinterplaywithsuperconductivityinyba2cu3o681 AT ebertphilipp atomicallyresolvedinterlayerchargeorderinganditsinterplaywithsuperconductivityinyba2cu3o681 AT chiuyaping atomicallyresolvedinterlayerchargeorderinganditsinterplaywithsuperconductivityinyba2cu3o681 |