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Atomically-resolved interlayer charge ordering and its interplay with superconductivity in YBa(2)Cu(3)O(6.81)

High-temperature superconductive (SC) cuprates exhibit not only a SC phase, but also competing orders, suppressing superconductivity. Charge order (CO) has been recognized as an important competing order, but its microscopic spatial interplay with SC phase as well as the interlayer coupling in CO an...

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Autores principales: Hsu, Chun-Chih, Huang, Bo-Chao, Schnedler, Michael, Lai, Ming-Yu, Wang, Yuh-Lin, Dunin-Borkowski, Rafal E., Chang, Chia-Seng, Lee, Ting-Kuo, Ebert, Philipp, Chiu, Ya-Ping
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8222377/
https://www.ncbi.nlm.nih.gov/pubmed/34162864
http://dx.doi.org/10.1038/s41467-021-24003-0
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author Hsu, Chun-Chih
Huang, Bo-Chao
Schnedler, Michael
Lai, Ming-Yu
Wang, Yuh-Lin
Dunin-Borkowski, Rafal E.
Chang, Chia-Seng
Lee, Ting-Kuo
Ebert, Philipp
Chiu, Ya-Ping
author_facet Hsu, Chun-Chih
Huang, Bo-Chao
Schnedler, Michael
Lai, Ming-Yu
Wang, Yuh-Lin
Dunin-Borkowski, Rafal E.
Chang, Chia-Seng
Lee, Ting-Kuo
Ebert, Philipp
Chiu, Ya-Ping
author_sort Hsu, Chun-Chih
collection PubMed
description High-temperature superconductive (SC) cuprates exhibit not only a SC phase, but also competing orders, suppressing superconductivity. Charge order (CO) has been recognized as an important competing order, but its microscopic spatial interplay with SC phase as well as the interlayer coupling in CO and SC phases remain elusive, despite being essential for understanding the physical mechanisms of competing orders and hence superconductivity. Here we report the achievement of direct real-space imaging with atomic-scale resolution of cryogenically cleaved YBa(2)Cu(3)O(6.81) using cross-sectional scanning tunneling microscopy/spectroscopy. CO nanodomains are found embedded in the SC phase with a proximity-like boundary region characterized by mutual suppression of CO and superconductivity. Furthermore, SC coherence as well as CO occur on both CuO chain and plane layers, revealing carrier transport and density of states mixing between layers. The CO antiphase correlation along the c direction suggests a dominance of Coulomb repulsion over Josephson tunneling between adjacent layers.
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spelling pubmed-82223772021-07-09 Atomically-resolved interlayer charge ordering and its interplay with superconductivity in YBa(2)Cu(3)O(6.81) Hsu, Chun-Chih Huang, Bo-Chao Schnedler, Michael Lai, Ming-Yu Wang, Yuh-Lin Dunin-Borkowski, Rafal E. Chang, Chia-Seng Lee, Ting-Kuo Ebert, Philipp Chiu, Ya-Ping Nat Commun Article High-temperature superconductive (SC) cuprates exhibit not only a SC phase, but also competing orders, suppressing superconductivity. Charge order (CO) has been recognized as an important competing order, but its microscopic spatial interplay with SC phase as well as the interlayer coupling in CO and SC phases remain elusive, despite being essential for understanding the physical mechanisms of competing orders and hence superconductivity. Here we report the achievement of direct real-space imaging with atomic-scale resolution of cryogenically cleaved YBa(2)Cu(3)O(6.81) using cross-sectional scanning tunneling microscopy/spectroscopy. CO nanodomains are found embedded in the SC phase with a proximity-like boundary region characterized by mutual suppression of CO and superconductivity. Furthermore, SC coherence as well as CO occur on both CuO chain and plane layers, revealing carrier transport and density of states mixing between layers. The CO antiphase correlation along the c direction suggests a dominance of Coulomb repulsion over Josephson tunneling between adjacent layers. Nature Publishing Group UK 2021-06-23 /pmc/articles/PMC8222377/ /pubmed/34162864 http://dx.doi.org/10.1038/s41467-021-24003-0 Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Hsu, Chun-Chih
Huang, Bo-Chao
Schnedler, Michael
Lai, Ming-Yu
Wang, Yuh-Lin
Dunin-Borkowski, Rafal E.
Chang, Chia-Seng
Lee, Ting-Kuo
Ebert, Philipp
Chiu, Ya-Ping
Atomically-resolved interlayer charge ordering and its interplay with superconductivity in YBa(2)Cu(3)O(6.81)
title Atomically-resolved interlayer charge ordering and its interplay with superconductivity in YBa(2)Cu(3)O(6.81)
title_full Atomically-resolved interlayer charge ordering and its interplay with superconductivity in YBa(2)Cu(3)O(6.81)
title_fullStr Atomically-resolved interlayer charge ordering and its interplay with superconductivity in YBa(2)Cu(3)O(6.81)
title_full_unstemmed Atomically-resolved interlayer charge ordering and its interplay with superconductivity in YBa(2)Cu(3)O(6.81)
title_short Atomically-resolved interlayer charge ordering and its interplay with superconductivity in YBa(2)Cu(3)O(6.81)
title_sort atomically-resolved interlayer charge ordering and its interplay with superconductivity in yba(2)cu(3)o(6.81)
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8222377/
https://www.ncbi.nlm.nih.gov/pubmed/34162864
http://dx.doi.org/10.1038/s41467-021-24003-0
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