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Measurements of periodically perturbed dewetting force fields and their consequences on the symmetry of the resulting patterns

We studied the origin of breaking the symmetry for moving circular contact lines of dewetting polymer films suspended on a periodic array of pillars. There, dewetting force fields driving polymer flow were perturbed by elastic micro-pillars arranged in a regular square pattern. Elastic restoring for...

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Autores principales: Roumpos, Konstantinos, Fontaine, Sarah, Pfohl, Thomas, Prucker, Oswald, Rühe, Jürgen, Reiter, Günter
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8222397/
https://www.ncbi.nlm.nih.gov/pubmed/34162940
http://dx.doi.org/10.1038/s41598-021-92544-x
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author Roumpos, Konstantinos
Fontaine, Sarah
Pfohl, Thomas
Prucker, Oswald
Rühe, Jürgen
Reiter, Günter
author_facet Roumpos, Konstantinos
Fontaine, Sarah
Pfohl, Thomas
Prucker, Oswald
Rühe, Jürgen
Reiter, Günter
author_sort Roumpos, Konstantinos
collection PubMed
description We studied the origin of breaking the symmetry for moving circular contact lines of dewetting polymer films suspended on a periodic array of pillars. There, dewetting force fields driving polymer flow were perturbed by elastic micro-pillars arranged in a regular square pattern. Elastic restoring forces of deformed pillars locally balance driving capillary forces and broke the circular symmetry of expanding dewetting holes. The observed envelope of the dewetting holes reflected the symmetry of the underlying pattern, even at sizes much larger than the characteristic period of the pillar array, demonstrating that periodic perturbations in a driving force field can establish a well-defined pattern of lower symmetry. For the presented system, we succeeded in squaring the circle.
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spelling pubmed-82223972021-07-02 Measurements of periodically perturbed dewetting force fields and their consequences on the symmetry of the resulting patterns Roumpos, Konstantinos Fontaine, Sarah Pfohl, Thomas Prucker, Oswald Rühe, Jürgen Reiter, Günter Sci Rep Article We studied the origin of breaking the symmetry for moving circular contact lines of dewetting polymer films suspended on a periodic array of pillars. There, dewetting force fields driving polymer flow were perturbed by elastic micro-pillars arranged in a regular square pattern. Elastic restoring forces of deformed pillars locally balance driving capillary forces and broke the circular symmetry of expanding dewetting holes. The observed envelope of the dewetting holes reflected the symmetry of the underlying pattern, even at sizes much larger than the characteristic period of the pillar array, demonstrating that periodic perturbations in a driving force field can establish a well-defined pattern of lower symmetry. For the presented system, we succeeded in squaring the circle. Nature Publishing Group UK 2021-06-23 /pmc/articles/PMC8222397/ /pubmed/34162940 http://dx.doi.org/10.1038/s41598-021-92544-x Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Roumpos, Konstantinos
Fontaine, Sarah
Pfohl, Thomas
Prucker, Oswald
Rühe, Jürgen
Reiter, Günter
Measurements of periodically perturbed dewetting force fields and their consequences on the symmetry of the resulting patterns
title Measurements of periodically perturbed dewetting force fields and their consequences on the symmetry of the resulting patterns
title_full Measurements of periodically perturbed dewetting force fields and their consequences on the symmetry of the resulting patterns
title_fullStr Measurements of periodically perturbed dewetting force fields and their consequences on the symmetry of the resulting patterns
title_full_unstemmed Measurements of periodically perturbed dewetting force fields and their consequences on the symmetry of the resulting patterns
title_short Measurements of periodically perturbed dewetting force fields and their consequences on the symmetry of the resulting patterns
title_sort measurements of periodically perturbed dewetting force fields and their consequences on the symmetry of the resulting patterns
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8222397/
https://www.ncbi.nlm.nih.gov/pubmed/34162940
http://dx.doi.org/10.1038/s41598-021-92544-x
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