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Femtosecond Single Cycle Pulses Enhanced the Efficiency of High Order Harmonic Generation

High-order harmonic generation is a nonlinear process that converts the gained energy during light-matter interaction into high-frequency radiation, thus resulting in the generation of coherent attosecond pulses in the XUV and soft x-ray regions. Here, we propose a control scheme for enhancing the e...

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Autores principales: Taoutioui, Abdelmalek, Agueny, Hicham
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8227859/
https://www.ncbi.nlm.nih.gov/pubmed/34073368
http://dx.doi.org/10.3390/mi12060610
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author Taoutioui, Abdelmalek
Agueny, Hicham
author_facet Taoutioui, Abdelmalek
Agueny, Hicham
author_sort Taoutioui, Abdelmalek
collection PubMed
description High-order harmonic generation is a nonlinear process that converts the gained energy during light-matter interaction into high-frequency radiation, thus resulting in the generation of coherent attosecond pulses in the XUV and soft x-ray regions. Here, we propose a control scheme for enhancing the efficiency of HHG process induced by an intense near-infrared (NIR) multi-cycle laser pulse. The scheme is based on introducing an infrared (IR) single-cycle pulse and exploiting its characteristic feature that manifests by a non-zero displacement effect to generate high-photon energy. The proposed scenario is numerically implemented on the basis of the time-dependent Schrödinger equation. In particular, we show that the combined pulses allow one to produce high-energy plateaus and that the harmonic cutoff is extended by a factor of 3 compared to the case with the NIR pulse alone. The emerged high-energy plateaus is understood as a result of a vast momentum transfer from the single-cycle field to the ionized electrons while travelling in the NIR field, thus leading to high-momentum electron recollisions. We also identify the role of the IR single-cycle field for controlling the directionality of the emitted electrons via the IR-field induced electron displacement effect. We further show that the emerged plateaus can be controlled by varying the relative carrier-envelope phase between the two pulses as well as the wavelengths. Our findings pave the way for an efficient control of light-matter interaction with the use of assisting femtosecond single-cycle fields.
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spelling pubmed-82278592021-06-26 Femtosecond Single Cycle Pulses Enhanced the Efficiency of High Order Harmonic Generation Taoutioui, Abdelmalek Agueny, Hicham Micromachines (Basel) Article High-order harmonic generation is a nonlinear process that converts the gained energy during light-matter interaction into high-frequency radiation, thus resulting in the generation of coherent attosecond pulses in the XUV and soft x-ray regions. Here, we propose a control scheme for enhancing the efficiency of HHG process induced by an intense near-infrared (NIR) multi-cycle laser pulse. The scheme is based on introducing an infrared (IR) single-cycle pulse and exploiting its characteristic feature that manifests by a non-zero displacement effect to generate high-photon energy. The proposed scenario is numerically implemented on the basis of the time-dependent Schrödinger equation. In particular, we show that the combined pulses allow one to produce high-energy plateaus and that the harmonic cutoff is extended by a factor of 3 compared to the case with the NIR pulse alone. The emerged high-energy plateaus is understood as a result of a vast momentum transfer from the single-cycle field to the ionized electrons while travelling in the NIR field, thus leading to high-momentum electron recollisions. We also identify the role of the IR single-cycle field for controlling the directionality of the emitted electrons via the IR-field induced electron displacement effect. We further show that the emerged plateaus can be controlled by varying the relative carrier-envelope phase between the two pulses as well as the wavelengths. Our findings pave the way for an efficient control of light-matter interaction with the use of assisting femtosecond single-cycle fields. MDPI 2021-05-26 /pmc/articles/PMC8227859/ /pubmed/34073368 http://dx.doi.org/10.3390/mi12060610 Text en © 2021 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Taoutioui, Abdelmalek
Agueny, Hicham
Femtosecond Single Cycle Pulses Enhanced the Efficiency of High Order Harmonic Generation
title Femtosecond Single Cycle Pulses Enhanced the Efficiency of High Order Harmonic Generation
title_full Femtosecond Single Cycle Pulses Enhanced the Efficiency of High Order Harmonic Generation
title_fullStr Femtosecond Single Cycle Pulses Enhanced the Efficiency of High Order Harmonic Generation
title_full_unstemmed Femtosecond Single Cycle Pulses Enhanced the Efficiency of High Order Harmonic Generation
title_short Femtosecond Single Cycle Pulses Enhanced the Efficiency of High Order Harmonic Generation
title_sort femtosecond single cycle pulses enhanced the efficiency of high order harmonic generation
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8227859/
https://www.ncbi.nlm.nih.gov/pubmed/34073368
http://dx.doi.org/10.3390/mi12060610
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