Strong Crystallographic Influence on Spin Hall Mechanism in PLD-Grown IrO(2) Thin Films

Spin-to-charge conversion is a central process in the emerging field of spintronics. One of its main applications is the electrical detection of spin currents, and for this, the inverse spin Hall effect (ISHE) has become one of the preferred methods. We studied the thickness dependence of the ISHE in iridium oxide (IrO [Formula: see text]) thin films, producing spin currents by means of the spin Seebeck effect in [Formula: see text] Fe [Formula: see text] O [Formula: see text] /IrO [Formula: see text] bilayers prepared by pulsed laser deposition (PLD). The observed ISHE charge current density, which features a maximum as a consequence of the spin diffusion length scale, follows the typical behaviour of spin-Hall-related phenomena. By fitting to the theory developed by Castel et al., we find that the spin Hall angle [Formula: see text] scales proportionally to the thin film resistivity, [Formula: see text] , and obtains a value for the spin diffusion length [Formula: see text] of [Formula: see text] nm. In addition, we observe a negative [Formula: see text] for every studied thickness and temperature, unlike previously reported works, which brings the possibility of tuning the desired functionality of high-resistance spin-Hall-based devices. We attribute this behaviour to the textured growth of the sample in the context of a highly anisotropic value of the spin Hall conductivity in this material.