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Charge order lock-in by electron-phonon coupling in La(1.675)Eu(0.2)Sr(0.125)CuO(4)

Charge order is universal to all hole-doped cuprates. Yet, the driving interactions remain an unsolved problem. Electron-electron interaction is widely believed to be essential, whereas the role of electron-phonon interaction is unclear. We report an ultrahigh-resolution resonant inelastic x-ray sca...

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Detalles Bibliográficos
Autores principales: Wang, Qisi, von Arx, Karin, Horio, Masafumi, Mukkattukavil, Deepak John, Küspert, Julia, Sassa, Yasmine, Schmitt, Thorsten, Nag, Abhishek, Pyon, Sunseng, Takayama, Tomohiro, Takagi, Hidenori, Garcia-Fernandez, Mirian, Zhou, Ke-Jin, Chang, Johan
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8245032/
https://www.ncbi.nlm.nih.gov/pubmed/34193430
http://dx.doi.org/10.1126/sciadv.abg7394
Descripción
Sumario:Charge order is universal to all hole-doped cuprates. Yet, the driving interactions remain an unsolved problem. Electron-electron interaction is widely believed to be essential, whereas the role of electron-phonon interaction is unclear. We report an ultrahigh-resolution resonant inelastic x-ray scattering (RIXS) study of the in-plane bond-stretching phonon mode in stripe-ordered cuprate La(1.675)Eu(0.2)Sr(0.125)CuO(4). Phonon softening and lifetime shortening are found around the charge ordering wave vector. In addition to these self-energy effects, the electron-phonon coupling is probed by its proportionality to the RIXS cross section. We find an enhancement of the electron-phonon coupling around the charge-stripe ordering wave vector upon cooling into the low-temperature tetragonal structure phase. These results suggest that, in addition to electronic correlations, electron-phonon coupling contributes substantially to the emergence of long-range charge-stripe order in cuprates.