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Charge order lock-in by electron-phonon coupling in La(1.675)Eu(0.2)Sr(0.125)CuO(4)
Charge order is universal to all hole-doped cuprates. Yet, the driving interactions remain an unsolved problem. Electron-electron interaction is widely believed to be essential, whereas the role of electron-phonon interaction is unclear. We report an ultrahigh-resolution resonant inelastic x-ray sca...
Autores principales: | , , , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Association for the Advancement of Science
2021
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8245032/ https://www.ncbi.nlm.nih.gov/pubmed/34193430 http://dx.doi.org/10.1126/sciadv.abg7394 |
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author | Wang, Qisi von Arx, Karin Horio, Masafumi Mukkattukavil, Deepak John Küspert, Julia Sassa, Yasmine Schmitt, Thorsten Nag, Abhishek Pyon, Sunseng Takayama, Tomohiro Takagi, Hidenori Garcia-Fernandez, Mirian Zhou, Ke-Jin Chang, Johan |
author_facet | Wang, Qisi von Arx, Karin Horio, Masafumi Mukkattukavil, Deepak John Küspert, Julia Sassa, Yasmine Schmitt, Thorsten Nag, Abhishek Pyon, Sunseng Takayama, Tomohiro Takagi, Hidenori Garcia-Fernandez, Mirian Zhou, Ke-Jin Chang, Johan |
author_sort | Wang, Qisi |
collection | PubMed |
description | Charge order is universal to all hole-doped cuprates. Yet, the driving interactions remain an unsolved problem. Electron-electron interaction is widely believed to be essential, whereas the role of electron-phonon interaction is unclear. We report an ultrahigh-resolution resonant inelastic x-ray scattering (RIXS) study of the in-plane bond-stretching phonon mode in stripe-ordered cuprate La(1.675)Eu(0.2)Sr(0.125)CuO(4). Phonon softening and lifetime shortening are found around the charge ordering wave vector. In addition to these self-energy effects, the electron-phonon coupling is probed by its proportionality to the RIXS cross section. We find an enhancement of the electron-phonon coupling around the charge-stripe ordering wave vector upon cooling into the low-temperature tetragonal structure phase. These results suggest that, in addition to electronic correlations, electron-phonon coupling contributes substantially to the emergence of long-range charge-stripe order in cuprates. |
format | Online Article Text |
id | pubmed-8245032 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | American Association for the Advancement of Science |
record_format | MEDLINE/PubMed |
spelling | pubmed-82450322021-07-13 Charge order lock-in by electron-phonon coupling in La(1.675)Eu(0.2)Sr(0.125)CuO(4) Wang, Qisi von Arx, Karin Horio, Masafumi Mukkattukavil, Deepak John Küspert, Julia Sassa, Yasmine Schmitt, Thorsten Nag, Abhishek Pyon, Sunseng Takayama, Tomohiro Takagi, Hidenori Garcia-Fernandez, Mirian Zhou, Ke-Jin Chang, Johan Sci Adv Research Articles Charge order is universal to all hole-doped cuprates. Yet, the driving interactions remain an unsolved problem. Electron-electron interaction is widely believed to be essential, whereas the role of electron-phonon interaction is unclear. We report an ultrahigh-resolution resonant inelastic x-ray scattering (RIXS) study of the in-plane bond-stretching phonon mode in stripe-ordered cuprate La(1.675)Eu(0.2)Sr(0.125)CuO(4). Phonon softening and lifetime shortening are found around the charge ordering wave vector. In addition to these self-energy effects, the electron-phonon coupling is probed by its proportionality to the RIXS cross section. We find an enhancement of the electron-phonon coupling around the charge-stripe ordering wave vector upon cooling into the low-temperature tetragonal structure phase. These results suggest that, in addition to electronic correlations, electron-phonon coupling contributes substantially to the emergence of long-range charge-stripe order in cuprates. American Association for the Advancement of Science 2021-06-30 /pmc/articles/PMC8245032/ /pubmed/34193430 http://dx.doi.org/10.1126/sciadv.abg7394 Text en Copyright © 2021 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). https://creativecommons.org/licenses/by-nc/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (https://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited. |
spellingShingle | Research Articles Wang, Qisi von Arx, Karin Horio, Masafumi Mukkattukavil, Deepak John Küspert, Julia Sassa, Yasmine Schmitt, Thorsten Nag, Abhishek Pyon, Sunseng Takayama, Tomohiro Takagi, Hidenori Garcia-Fernandez, Mirian Zhou, Ke-Jin Chang, Johan Charge order lock-in by electron-phonon coupling in La(1.675)Eu(0.2)Sr(0.125)CuO(4) |
title | Charge order lock-in by electron-phonon coupling in La(1.675)Eu(0.2)Sr(0.125)CuO(4) |
title_full | Charge order lock-in by electron-phonon coupling in La(1.675)Eu(0.2)Sr(0.125)CuO(4) |
title_fullStr | Charge order lock-in by electron-phonon coupling in La(1.675)Eu(0.2)Sr(0.125)CuO(4) |
title_full_unstemmed | Charge order lock-in by electron-phonon coupling in La(1.675)Eu(0.2)Sr(0.125)CuO(4) |
title_short | Charge order lock-in by electron-phonon coupling in La(1.675)Eu(0.2)Sr(0.125)CuO(4) |
title_sort | charge order lock-in by electron-phonon coupling in la(1.675)eu(0.2)sr(0.125)cuo(4) |
topic | Research Articles |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8245032/ https://www.ncbi.nlm.nih.gov/pubmed/34193430 http://dx.doi.org/10.1126/sciadv.abg7394 |
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