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Charge order lock-in by electron-phonon coupling in La(1.675)Eu(0.2)Sr(0.125)CuO(4)

Charge order is universal to all hole-doped cuprates. Yet, the driving interactions remain an unsolved problem. Electron-electron interaction is widely believed to be essential, whereas the role of electron-phonon interaction is unclear. We report an ultrahigh-resolution resonant inelastic x-ray sca...

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Autores principales: Wang, Qisi, von Arx, Karin, Horio, Masafumi, Mukkattukavil, Deepak John, Küspert, Julia, Sassa, Yasmine, Schmitt, Thorsten, Nag, Abhishek, Pyon, Sunseng, Takayama, Tomohiro, Takagi, Hidenori, Garcia-Fernandez, Mirian, Zhou, Ke-Jin, Chang, Johan
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8245032/
https://www.ncbi.nlm.nih.gov/pubmed/34193430
http://dx.doi.org/10.1126/sciadv.abg7394
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author Wang, Qisi
von Arx, Karin
Horio, Masafumi
Mukkattukavil, Deepak John
Küspert, Julia
Sassa, Yasmine
Schmitt, Thorsten
Nag, Abhishek
Pyon, Sunseng
Takayama, Tomohiro
Takagi, Hidenori
Garcia-Fernandez, Mirian
Zhou, Ke-Jin
Chang, Johan
author_facet Wang, Qisi
von Arx, Karin
Horio, Masafumi
Mukkattukavil, Deepak John
Küspert, Julia
Sassa, Yasmine
Schmitt, Thorsten
Nag, Abhishek
Pyon, Sunseng
Takayama, Tomohiro
Takagi, Hidenori
Garcia-Fernandez, Mirian
Zhou, Ke-Jin
Chang, Johan
author_sort Wang, Qisi
collection PubMed
description Charge order is universal to all hole-doped cuprates. Yet, the driving interactions remain an unsolved problem. Electron-electron interaction is widely believed to be essential, whereas the role of electron-phonon interaction is unclear. We report an ultrahigh-resolution resonant inelastic x-ray scattering (RIXS) study of the in-plane bond-stretching phonon mode in stripe-ordered cuprate La(1.675)Eu(0.2)Sr(0.125)CuO(4). Phonon softening and lifetime shortening are found around the charge ordering wave vector. In addition to these self-energy effects, the electron-phonon coupling is probed by its proportionality to the RIXS cross section. We find an enhancement of the electron-phonon coupling around the charge-stripe ordering wave vector upon cooling into the low-temperature tetragonal structure phase. These results suggest that, in addition to electronic correlations, electron-phonon coupling contributes substantially to the emergence of long-range charge-stripe order in cuprates.
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spelling pubmed-82450322021-07-13 Charge order lock-in by electron-phonon coupling in La(1.675)Eu(0.2)Sr(0.125)CuO(4) Wang, Qisi von Arx, Karin Horio, Masafumi Mukkattukavil, Deepak John Küspert, Julia Sassa, Yasmine Schmitt, Thorsten Nag, Abhishek Pyon, Sunseng Takayama, Tomohiro Takagi, Hidenori Garcia-Fernandez, Mirian Zhou, Ke-Jin Chang, Johan Sci Adv Research Articles Charge order is universal to all hole-doped cuprates. Yet, the driving interactions remain an unsolved problem. Electron-electron interaction is widely believed to be essential, whereas the role of electron-phonon interaction is unclear. We report an ultrahigh-resolution resonant inelastic x-ray scattering (RIXS) study of the in-plane bond-stretching phonon mode in stripe-ordered cuprate La(1.675)Eu(0.2)Sr(0.125)CuO(4). Phonon softening and lifetime shortening are found around the charge ordering wave vector. In addition to these self-energy effects, the electron-phonon coupling is probed by its proportionality to the RIXS cross section. We find an enhancement of the electron-phonon coupling around the charge-stripe ordering wave vector upon cooling into the low-temperature tetragonal structure phase. These results suggest that, in addition to electronic correlations, electron-phonon coupling contributes substantially to the emergence of long-range charge-stripe order in cuprates. American Association for the Advancement of Science 2021-06-30 /pmc/articles/PMC8245032/ /pubmed/34193430 http://dx.doi.org/10.1126/sciadv.abg7394 Text en Copyright © 2021 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). https://creativecommons.org/licenses/by-nc/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (https://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.
spellingShingle Research Articles
Wang, Qisi
von Arx, Karin
Horio, Masafumi
Mukkattukavil, Deepak John
Küspert, Julia
Sassa, Yasmine
Schmitt, Thorsten
Nag, Abhishek
Pyon, Sunseng
Takayama, Tomohiro
Takagi, Hidenori
Garcia-Fernandez, Mirian
Zhou, Ke-Jin
Chang, Johan
Charge order lock-in by electron-phonon coupling in La(1.675)Eu(0.2)Sr(0.125)CuO(4)
title Charge order lock-in by electron-phonon coupling in La(1.675)Eu(0.2)Sr(0.125)CuO(4)
title_full Charge order lock-in by electron-phonon coupling in La(1.675)Eu(0.2)Sr(0.125)CuO(4)
title_fullStr Charge order lock-in by electron-phonon coupling in La(1.675)Eu(0.2)Sr(0.125)CuO(4)
title_full_unstemmed Charge order lock-in by electron-phonon coupling in La(1.675)Eu(0.2)Sr(0.125)CuO(4)
title_short Charge order lock-in by electron-phonon coupling in La(1.675)Eu(0.2)Sr(0.125)CuO(4)
title_sort charge order lock-in by electron-phonon coupling in la(1.675)eu(0.2)sr(0.125)cuo(4)
topic Research Articles
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8245032/
https://www.ncbi.nlm.nih.gov/pubmed/34193430
http://dx.doi.org/10.1126/sciadv.abg7394
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