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Lifetime-Associated Two-Dimensional Infrared Spectroscopy Reveals the Hydrogen-Bond Structure of Supercooled Water in Soft Confinement

[Image: see text] We demonstrate a method to address the problem of spectral overlap in multidimensional vibrational spectroscopy and use it to investigate supercooled aqueous sorbitol solutions. The absence of crystallization in these solutions has been attributed to “soft” confinement of water in...

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Detalles Bibliográficos
Autores principales: Caporaletti, Federico, Bonn, Daniel, Woutersen, Sander
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2021
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8256423/
https://www.ncbi.nlm.nih.gov/pubmed/34157231
http://dx.doi.org/10.1021/acs.jpclett.1c01595