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Lifetime-Associated Two-Dimensional Infrared Spectroscopy Reveals the Hydrogen-Bond Structure of Supercooled Water in Soft Confinement
[Image: see text] We demonstrate a method to address the problem of spectral overlap in multidimensional vibrational spectroscopy and use it to investigate supercooled aqueous sorbitol solutions. The absence of crystallization in these solutions has been attributed to “soft” confinement of water in...
Autores principales: | Caporaletti, Federico, Bonn, Daniel, Woutersen, Sander |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical
Society
2021
|
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8256423/ https://www.ncbi.nlm.nih.gov/pubmed/34157231 http://dx.doi.org/10.1021/acs.jpclett.1c01595 |
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