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Alkynyl triazenes enable divergent syntheses of 2-pyrones
The 2-pyrone motif occurs frequently in bioactive natural products and is appreciated as synthetic intermediates. However, only few methods allow for diversifying functional group modifications on this relevant heterocycle. The distinct properties of 1-alkynyl triazenes promote a smooth addition of...
Autores principales: | , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
The Royal Society of Chemistry
2021
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8261734/ https://www.ncbi.nlm.nih.gov/pubmed/34276943 http://dx.doi.org/10.1039/d1sc02583j |
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author | Tan, Jin-Fay Bormann, Carl Thomas Severin, Kay Cramer, Nicolai |
author_facet | Tan, Jin-Fay Bormann, Carl Thomas Severin, Kay Cramer, Nicolai |
author_sort | Tan, Jin-Fay |
collection | PubMed |
description | The 2-pyrone motif occurs frequently in bioactive natural products and is appreciated as synthetic intermediates. However, only few methods allow for diversifying functional group modifications on this relevant heterocycle. The distinct properties of 1-alkynyl triazenes promote a smooth addition of propiolic acids across the triple bond. Addition of catalytic amounts of silver salt induces cyclization to 2-pyrones. Depending on the reaction temperature, either 6-triazenyl or 5-triazenyl 2-pyrones are selectively formed. The triazenyl unit is subsequently replaced by a variety of valuable groups in a one-pot process yielding for instance 2-fluoro pyrones. The substitution occurs with an intriguing 1,5-carbonyl transposition. Moreover, the triazenyl group serves as traceless activating group for subsequent Diels–Alder cycloadditions and as a constituting unit for rare fused aminopyrazole pyrone heterocycles. |
format | Online Article Text |
id | pubmed-8261734 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | The Royal Society of Chemistry |
record_format | MEDLINE/PubMed |
spelling | pubmed-82617342021-07-16 Alkynyl triazenes enable divergent syntheses of 2-pyrones Tan, Jin-Fay Bormann, Carl Thomas Severin, Kay Cramer, Nicolai Chem Sci Chemistry The 2-pyrone motif occurs frequently in bioactive natural products and is appreciated as synthetic intermediates. However, only few methods allow for diversifying functional group modifications on this relevant heterocycle. The distinct properties of 1-alkynyl triazenes promote a smooth addition of propiolic acids across the triple bond. Addition of catalytic amounts of silver salt induces cyclization to 2-pyrones. Depending on the reaction temperature, either 6-triazenyl or 5-triazenyl 2-pyrones are selectively formed. The triazenyl unit is subsequently replaced by a variety of valuable groups in a one-pot process yielding for instance 2-fluoro pyrones. The substitution occurs with an intriguing 1,5-carbonyl transposition. Moreover, the triazenyl group serves as traceless activating group for subsequent Diels–Alder cycloadditions and as a constituting unit for rare fused aminopyrazole pyrone heterocycles. The Royal Society of Chemistry 2021-06-04 /pmc/articles/PMC8261734/ /pubmed/34276943 http://dx.doi.org/10.1039/d1sc02583j Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/ |
spellingShingle | Chemistry Tan, Jin-Fay Bormann, Carl Thomas Severin, Kay Cramer, Nicolai Alkynyl triazenes enable divergent syntheses of 2-pyrones |
title | Alkynyl triazenes enable divergent syntheses of 2-pyrones |
title_full | Alkynyl triazenes enable divergent syntheses of 2-pyrones |
title_fullStr | Alkynyl triazenes enable divergent syntheses of 2-pyrones |
title_full_unstemmed | Alkynyl triazenes enable divergent syntheses of 2-pyrones |
title_short | Alkynyl triazenes enable divergent syntheses of 2-pyrones |
title_sort | alkynyl triazenes enable divergent syntheses of 2-pyrones |
topic | Chemistry |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8261734/ https://www.ncbi.nlm.nih.gov/pubmed/34276943 http://dx.doi.org/10.1039/d1sc02583j |
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