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Influence of Different Thermal Aging Conditions on Soot Combustion with Catalyst by Thermogravimetric Analysis

Diesel particulates are deposited in the diesel particulate filter and removed by the regeneration process. The Printex-U (PU) particles are simulated as the diesel soot to investigate the influence of thermal aging conditions on soot combustion performance with the addition of catalysts. The compre...

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Autores principales: Yang, Yi, Fang, Jia, Huang, Junfeng, Qin, Zihan, Zhang, Qian, Pu, Ping, Pan, Suozhu
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8269735/
https://www.ncbi.nlm.nih.gov/pubmed/34208891
http://dx.doi.org/10.3390/ma14133647
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author Yang, Yi
Fang, Jia
Huang, Junfeng
Qin, Zihan
Zhang, Qian
Pu, Ping
Pan, Suozhu
author_facet Yang, Yi
Fang, Jia
Huang, Junfeng
Qin, Zihan
Zhang, Qian
Pu, Ping
Pan, Suozhu
author_sort Yang, Yi
collection PubMed
description Diesel particulates are deposited in the diesel particulate filter and removed by the regeneration process. The Printex-U (PU) particles are simulated as the diesel soot to investigate the influence of thermal aging conditions on soot combustion performance with the addition of catalysts. The comprehensive combustion index S, combustion stability index R(w) and peak temperature T(p) are obtained to evaluate the combustion performance. Compared with the PU/Pt mixtures of different Pt contents (2 g/ft(3), 3.5 g/ft(3), and 5 g/ft(3)), the 10 g/ft(3) Pt contents improve soot combustion with the outstanding oxygen absorption ability. When the weight ratio of PU/Pt mixture is 1:1, the promoted effect achieves the maximum degree. The S and R(w) increase to 8.90 × 10(−8) %(2)min(−2)°C(−3) and 39.11 × 10(5), respectively, compared with pure PU. After the thermal aging process, the PU/Pt mixture with a 350 °C aging temperature for 10 h promotes the soot combustion the best when compared to pure PU particles. It is not good as the PU/Pt mixture without aging, because the inner properties of soot and Pt/Al(2)O(3) catalyst may have been changed. The S and R(w) are 9.07 × 10(−8) %(2)min(−2)°C(−3) and 38.39 × 10(5), respectively, which are close to the no aging mixture. This work plays a crucial role in understanding the mechanism of the comprehensive effect of soot and catalyst on soot combustion after the thermal aging process.
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spelling pubmed-82697352021-07-10 Influence of Different Thermal Aging Conditions on Soot Combustion with Catalyst by Thermogravimetric Analysis Yang, Yi Fang, Jia Huang, Junfeng Qin, Zihan Zhang, Qian Pu, Ping Pan, Suozhu Materials (Basel) Article Diesel particulates are deposited in the diesel particulate filter and removed by the regeneration process. The Printex-U (PU) particles are simulated as the diesel soot to investigate the influence of thermal aging conditions on soot combustion performance with the addition of catalysts. The comprehensive combustion index S, combustion stability index R(w) and peak temperature T(p) are obtained to evaluate the combustion performance. Compared with the PU/Pt mixtures of different Pt contents (2 g/ft(3), 3.5 g/ft(3), and 5 g/ft(3)), the 10 g/ft(3) Pt contents improve soot combustion with the outstanding oxygen absorption ability. When the weight ratio of PU/Pt mixture is 1:1, the promoted effect achieves the maximum degree. The S and R(w) increase to 8.90 × 10(−8) %(2)min(−2)°C(−3) and 39.11 × 10(5), respectively, compared with pure PU. After the thermal aging process, the PU/Pt mixture with a 350 °C aging temperature for 10 h promotes the soot combustion the best when compared to pure PU particles. It is not good as the PU/Pt mixture without aging, because the inner properties of soot and Pt/Al(2)O(3) catalyst may have been changed. The S and R(w) are 9.07 × 10(−8) %(2)min(−2)°C(−3) and 38.39 × 10(5), respectively, which are close to the no aging mixture. This work plays a crucial role in understanding the mechanism of the comprehensive effect of soot and catalyst on soot combustion after the thermal aging process. MDPI 2021-06-30 /pmc/articles/PMC8269735/ /pubmed/34208891 http://dx.doi.org/10.3390/ma14133647 Text en © 2021 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Yang, Yi
Fang, Jia
Huang, Junfeng
Qin, Zihan
Zhang, Qian
Pu, Ping
Pan, Suozhu
Influence of Different Thermal Aging Conditions on Soot Combustion with Catalyst by Thermogravimetric Analysis
title Influence of Different Thermal Aging Conditions on Soot Combustion with Catalyst by Thermogravimetric Analysis
title_full Influence of Different Thermal Aging Conditions on Soot Combustion with Catalyst by Thermogravimetric Analysis
title_fullStr Influence of Different Thermal Aging Conditions on Soot Combustion with Catalyst by Thermogravimetric Analysis
title_full_unstemmed Influence of Different Thermal Aging Conditions on Soot Combustion with Catalyst by Thermogravimetric Analysis
title_short Influence of Different Thermal Aging Conditions on Soot Combustion with Catalyst by Thermogravimetric Analysis
title_sort influence of different thermal aging conditions on soot combustion with catalyst by thermogravimetric analysis
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8269735/
https://www.ncbi.nlm.nih.gov/pubmed/34208891
http://dx.doi.org/10.3390/ma14133647
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