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Phonon-assisted relaxation between triplet and singlet states in a self-assembled double quantum dot

We study theoretically phonon-induced spin dynamics of two electrons confined in a self-assembled double quantum dot. We calculate the transition rates and time evolution of occupations for the spin-triplet and spin-singlet states. We characterize the relative importance of various relaxation channe...

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Autores principales: Gawarecki, Krzysztof, Machnikowski, Paweł
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8316559/
https://www.ncbi.nlm.nih.gov/pubmed/34315967
http://dx.doi.org/10.1038/s41598-021-94621-7
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author Gawarecki, Krzysztof
Machnikowski, Paweł
author_facet Gawarecki, Krzysztof
Machnikowski, Paweł
author_sort Gawarecki, Krzysztof
collection PubMed
description We study theoretically phonon-induced spin dynamics of two electrons confined in a self-assembled double quantum dot. We calculate the transition rates and time evolution of occupations for the spin-triplet and spin-singlet states. We characterize the relative importance of various relaxation channels, including two-phonon processes, as a function of the electric and magnetic fields. The simulations are based on a model combining the eight-band [Formula: see text] method and configuration-interaction approach. We show that the electron g-factor mismatch between the Zeeman doublets localized on different dots opens a relatively fast triplet-singlet phonon-assisted relaxation channel. We also demonstrate, that the relaxation near the triplet-singlet anticrossing is slowed down up to several orders of magnitude due to vanishing of some relaxation channels.
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spelling pubmed-83165592021-07-29 Phonon-assisted relaxation between triplet and singlet states in a self-assembled double quantum dot Gawarecki, Krzysztof Machnikowski, Paweł Sci Rep Article We study theoretically phonon-induced spin dynamics of two electrons confined in a self-assembled double quantum dot. We calculate the transition rates and time evolution of occupations for the spin-triplet and spin-singlet states. We characterize the relative importance of various relaxation channels, including two-phonon processes, as a function of the electric and magnetic fields. The simulations are based on a model combining the eight-band [Formula: see text] method and configuration-interaction approach. We show that the electron g-factor mismatch between the Zeeman doublets localized on different dots opens a relatively fast triplet-singlet phonon-assisted relaxation channel. We also demonstrate, that the relaxation near the triplet-singlet anticrossing is slowed down up to several orders of magnitude due to vanishing of some relaxation channels. Nature Publishing Group UK 2021-07-27 /pmc/articles/PMC8316559/ /pubmed/34315967 http://dx.doi.org/10.1038/s41598-021-94621-7 Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open AccessThis article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Gawarecki, Krzysztof
Machnikowski, Paweł
Phonon-assisted relaxation between triplet and singlet states in a self-assembled double quantum dot
title Phonon-assisted relaxation between triplet and singlet states in a self-assembled double quantum dot
title_full Phonon-assisted relaxation between triplet and singlet states in a self-assembled double quantum dot
title_fullStr Phonon-assisted relaxation between triplet and singlet states in a self-assembled double quantum dot
title_full_unstemmed Phonon-assisted relaxation between triplet and singlet states in a self-assembled double quantum dot
title_short Phonon-assisted relaxation between triplet and singlet states in a self-assembled double quantum dot
title_sort phonon-assisted relaxation between triplet and singlet states in a self-assembled double quantum dot
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8316559/
https://www.ncbi.nlm.nih.gov/pubmed/34315967
http://dx.doi.org/10.1038/s41598-021-94621-7
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AT machnikowskipaweł phononassistedrelaxationbetweentripletandsingletstatesinaselfassembleddoublequantumdot