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Highly Resolved and Robust Dynamic X‐Ray Imaging Using Perovskite Glass‐Ceramic Scintillator with Reduced Light Scattering
All‐inorganic perovskite quantum dots (QDs) CsPbX(3) (X = Cl, Br, and I) have recently emerged as a new promising class of X‐ray scintillators. However, the instability of perovskite QDs and the strong optical scattering of the thick opaque QD scintillator film imped it to realize high‐quality and r...
Autores principales: | , , , , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
John Wiley and Sons Inc.
2021
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8336613/ https://www.ncbi.nlm.nih.gov/pubmed/34075729 http://dx.doi.org/10.1002/advs.202003728 |
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author | Ma, Wenbo Jiang, Tingming Yang, Ze Zhang, Hao Su, Yirong Chen, Zeng Chen, Xinya Ma, Yaoguang Zhu, Wenjuan Yu, Xue Zhu, Haiming Qiu, Jianbei Liu, Xu Xu, Xuhui Yang, Yang (Michael) |
author_facet | Ma, Wenbo Jiang, Tingming Yang, Ze Zhang, Hao Su, Yirong Chen, Zeng Chen, Xinya Ma, Yaoguang Zhu, Wenjuan Yu, Xue Zhu, Haiming Qiu, Jianbei Liu, Xu Xu, Xuhui Yang, Yang (Michael) |
author_sort | Ma, Wenbo |
collection | PubMed |
description | All‐inorganic perovskite quantum dots (QDs) CsPbX(3) (X = Cl, Br, and I) have recently emerged as a new promising class of X‐ray scintillators. However, the instability of perovskite QDs and the strong optical scattering of the thick opaque QD scintillator film imped it to realize high‐quality and robust X‐ray image. Herein, the europium (Eu) doped CsPbBr(3) QDs are in situ grown inside transparent amorphous matrix to form glass‐ceramic (GC) scintillator with glass phase serving as both matrix and encapsulation for the perovskite QD scintillators. The small amount of Eu dopant optimizes the crystallization of CsPbBr(3) QDs and makes their distribution more uniform in the glass matrix, which can significantly reduce the light scattering and also enhance the photoluminescence emission of CsPbBr(3) QDs. As a result, a remarkably high spatial resolution of 15.0 lp mm(−1) is realized thanks to the reduced light scattering, which is so far a record resolution for perovskite scintillator based X‐ray imaging, and the scintillation stability is also significantly improved compared to the bare perovskite QD scintillators. Those results provide an effective platform particularly for the emerging perovskite nanocrystal scintillators to reduce light scattering and improve radiation hardness. |
format | Online Article Text |
id | pubmed-8336613 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | John Wiley and Sons Inc. |
record_format | MEDLINE/PubMed |
spelling | pubmed-83366132021-08-11 Highly Resolved and Robust Dynamic X‐Ray Imaging Using Perovskite Glass‐Ceramic Scintillator with Reduced Light Scattering Ma, Wenbo Jiang, Tingming Yang, Ze Zhang, Hao Su, Yirong Chen, Zeng Chen, Xinya Ma, Yaoguang Zhu, Wenjuan Yu, Xue Zhu, Haiming Qiu, Jianbei Liu, Xu Xu, Xuhui Yang, Yang (Michael) Adv Sci (Weinh) Communications All‐inorganic perovskite quantum dots (QDs) CsPbX(3) (X = Cl, Br, and I) have recently emerged as a new promising class of X‐ray scintillators. However, the instability of perovskite QDs and the strong optical scattering of the thick opaque QD scintillator film imped it to realize high‐quality and robust X‐ray image. Herein, the europium (Eu) doped CsPbBr(3) QDs are in situ grown inside transparent amorphous matrix to form glass‐ceramic (GC) scintillator with glass phase serving as both matrix and encapsulation for the perovskite QD scintillators. The small amount of Eu dopant optimizes the crystallization of CsPbBr(3) QDs and makes their distribution more uniform in the glass matrix, which can significantly reduce the light scattering and also enhance the photoluminescence emission of CsPbBr(3) QDs. As a result, a remarkably high spatial resolution of 15.0 lp mm(−1) is realized thanks to the reduced light scattering, which is so far a record resolution for perovskite scintillator based X‐ray imaging, and the scintillation stability is also significantly improved compared to the bare perovskite QD scintillators. Those results provide an effective platform particularly for the emerging perovskite nanocrystal scintillators to reduce light scattering and improve radiation hardness. John Wiley and Sons Inc. 2021-06-02 /pmc/articles/PMC8336613/ /pubmed/34075729 http://dx.doi.org/10.1002/advs.202003728 Text en © 2021 The Authors. Advanced Science published by Wiley‐VCH GmbH https://creativecommons.org/licenses/by/4.0/This is an open access article under the terms of the http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited. |
spellingShingle | Communications Ma, Wenbo Jiang, Tingming Yang, Ze Zhang, Hao Su, Yirong Chen, Zeng Chen, Xinya Ma, Yaoguang Zhu, Wenjuan Yu, Xue Zhu, Haiming Qiu, Jianbei Liu, Xu Xu, Xuhui Yang, Yang (Michael) Highly Resolved and Robust Dynamic X‐Ray Imaging Using Perovskite Glass‐Ceramic Scintillator with Reduced Light Scattering |
title | Highly Resolved and Robust Dynamic X‐Ray Imaging Using Perovskite Glass‐Ceramic Scintillator with Reduced Light Scattering |
title_full | Highly Resolved and Robust Dynamic X‐Ray Imaging Using Perovskite Glass‐Ceramic Scintillator with Reduced Light Scattering |
title_fullStr | Highly Resolved and Robust Dynamic X‐Ray Imaging Using Perovskite Glass‐Ceramic Scintillator with Reduced Light Scattering |
title_full_unstemmed | Highly Resolved and Robust Dynamic X‐Ray Imaging Using Perovskite Glass‐Ceramic Scintillator with Reduced Light Scattering |
title_short | Highly Resolved and Robust Dynamic X‐Ray Imaging Using Perovskite Glass‐Ceramic Scintillator with Reduced Light Scattering |
title_sort | highly resolved and robust dynamic x‐ray imaging using perovskite glass‐ceramic scintillator with reduced light scattering |
topic | Communications |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8336613/ https://www.ncbi.nlm.nih.gov/pubmed/34075729 http://dx.doi.org/10.1002/advs.202003728 |
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