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Carbon Nanotube Far Infrared Detectors with High Responsivity and Superior Polarization Selectivity Based on Engineered Optical Antennas

Single-wall carbon nanotube (SWCNT) thin films are promising for sensitive uncooled infrared detection based on the photothermoelectric effect. The SWCNT film is usually shaped into a belt and diversely doped to form a p-n junction at the center. Under the illumination of a focused incident light, t...

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Autores principales: Ren, Xiansong, Ji, Zhaoyu, Chen, Binkai, Zhou, Jing, Chu, Zeshi, Chen, Xiaoshuang
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8347452/
https://www.ncbi.nlm.nih.gov/pubmed/34372458
http://dx.doi.org/10.3390/s21155221
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author Ren, Xiansong
Ji, Zhaoyu
Chen, Binkai
Zhou, Jing
Chu, Zeshi
Chen, Xiaoshuang
author_facet Ren, Xiansong
Ji, Zhaoyu
Chen, Binkai
Zhou, Jing
Chu, Zeshi
Chen, Xiaoshuang
author_sort Ren, Xiansong
collection PubMed
description Single-wall carbon nanotube (SWCNT) thin films are promising for sensitive uncooled infrared detection based on the photothermoelectric effect. The SWCNT film is usually shaped into a belt and diversely doped to form a p-n junction at the center. Under the illumination of a focused incident light, the temperature gradient from the junction to the contacts leads to photoresponse. When the SWCNTs are aligned in one direction, the photoresponse becomes polarization selective. Although a typical bowtie antenna can improve the responsivity and polarization extinction ratio by deep-subwavelength light focusing, the absolute absorptance of the junction region is only 0.6%. In this work, the antenna was engineered for a higher light coupling efficiency. By integrating a bottom metal plane at a specific distance from the SWCNT film and optimizing the antenna geometries, we achieved ultra-efficient impedance matching between the antenna and the SWCNTs, thus the absorptance of the junction region was further enhanced by 21.3 times and reached 13.5%, which is more than 3 orders of magnitude higher than that of the device without the engineered antenna. The peak responsivity was further enhanced by 19.9 times and responsivity reached 1500 V/W at 1 THz. The resonant frequency can be tuned by changing the size of the antenna. Over the frequency range of 0.5 THz to 1.5 THz, the peak responsivity was further enhanced by 8.1 to 19.9 times, and the polarization extinction ratio was enhanced by 2.7 to 22.3 times. The highest polarization extinction ratio reached 3.04 × 10(5) at 0.5 THz. The results are based on the numerical simulations of the light and the thermal fields.
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spelling pubmed-83474522021-08-08 Carbon Nanotube Far Infrared Detectors with High Responsivity and Superior Polarization Selectivity Based on Engineered Optical Antennas Ren, Xiansong Ji, Zhaoyu Chen, Binkai Zhou, Jing Chu, Zeshi Chen, Xiaoshuang Sensors (Basel) Communication Single-wall carbon nanotube (SWCNT) thin films are promising for sensitive uncooled infrared detection based on the photothermoelectric effect. The SWCNT film is usually shaped into a belt and diversely doped to form a p-n junction at the center. Under the illumination of a focused incident light, the temperature gradient from the junction to the contacts leads to photoresponse. When the SWCNTs are aligned in one direction, the photoresponse becomes polarization selective. Although a typical bowtie antenna can improve the responsivity and polarization extinction ratio by deep-subwavelength light focusing, the absolute absorptance of the junction region is only 0.6%. In this work, the antenna was engineered for a higher light coupling efficiency. By integrating a bottom metal plane at a specific distance from the SWCNT film and optimizing the antenna geometries, we achieved ultra-efficient impedance matching between the antenna and the SWCNTs, thus the absorptance of the junction region was further enhanced by 21.3 times and reached 13.5%, which is more than 3 orders of magnitude higher than that of the device without the engineered antenna. The peak responsivity was further enhanced by 19.9 times and responsivity reached 1500 V/W at 1 THz. The resonant frequency can be tuned by changing the size of the antenna. Over the frequency range of 0.5 THz to 1.5 THz, the peak responsivity was further enhanced by 8.1 to 19.9 times, and the polarization extinction ratio was enhanced by 2.7 to 22.3 times. The highest polarization extinction ratio reached 3.04 × 10(5) at 0.5 THz. The results are based on the numerical simulations of the light and the thermal fields. MDPI 2021-07-31 /pmc/articles/PMC8347452/ /pubmed/34372458 http://dx.doi.org/10.3390/s21155221 Text en © 2021 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Communication
Ren, Xiansong
Ji, Zhaoyu
Chen, Binkai
Zhou, Jing
Chu, Zeshi
Chen, Xiaoshuang
Carbon Nanotube Far Infrared Detectors with High Responsivity and Superior Polarization Selectivity Based on Engineered Optical Antennas
title Carbon Nanotube Far Infrared Detectors with High Responsivity and Superior Polarization Selectivity Based on Engineered Optical Antennas
title_full Carbon Nanotube Far Infrared Detectors with High Responsivity and Superior Polarization Selectivity Based on Engineered Optical Antennas
title_fullStr Carbon Nanotube Far Infrared Detectors with High Responsivity and Superior Polarization Selectivity Based on Engineered Optical Antennas
title_full_unstemmed Carbon Nanotube Far Infrared Detectors with High Responsivity and Superior Polarization Selectivity Based on Engineered Optical Antennas
title_short Carbon Nanotube Far Infrared Detectors with High Responsivity and Superior Polarization Selectivity Based on Engineered Optical Antennas
title_sort carbon nanotube far infrared detectors with high responsivity and superior polarization selectivity based on engineered optical antennas
topic Communication
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8347452/
https://www.ncbi.nlm.nih.gov/pubmed/34372458
http://dx.doi.org/10.3390/s21155221
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