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Extraordinary phase coherence length in epitaxial halide perovskites

Inorganic halide perovskites have emerged as a promising platform in a wide range of applications from solar energy harvesting to computing and light emission. The recent advent of epitaxial thin film growth of halide perovskites has made it possible to investigate low-dimensional quantum electronic...

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Autores principales: Nasyedkin, Kostyantyn, King, Isaac, Zhang, Liangji, Chen, Pei, Wang, Lili, Staples, Richard J., Lunt, Richard R., Pollanen, Johannes
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Elsevier 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8358163/
https://www.ncbi.nlm.nih.gov/pubmed/34401682
http://dx.doi.org/10.1016/j.isci.2021.102912
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author Nasyedkin, Kostyantyn
King, Isaac
Zhang, Liangji
Chen, Pei
Wang, Lili
Staples, Richard J.
Lunt, Richard R.
Pollanen, Johannes
author_facet Nasyedkin, Kostyantyn
King, Isaac
Zhang, Liangji
Chen, Pei
Wang, Lili
Staples, Richard J.
Lunt, Richard R.
Pollanen, Johannes
author_sort Nasyedkin, Kostyantyn
collection PubMed
description Inorganic halide perovskites have emerged as a promising platform in a wide range of applications from solar energy harvesting to computing and light emission. The recent advent of epitaxial thin film growth of halide perovskites has made it possible to investigate low-dimensional quantum electronic devices based on this class of materials. This study leverages advances in vapor-phase epitaxy of halide perovskites to perform low-temperature magnetotransport measurements on single-domain cesium tin iodide (CsSnI(3)) epitaxial thin films. The low-field magnetoresistance carries signatures of coherent quantum interference effects and spin-orbit coupling. These weak anti-localization measurements reveal a micron-scale low-temperature phase coherence length for charge carriers in this system. The results indicate that epitaxial halide perovskite heterostructures are a promising platform for investigating long coherent quantum electronic effects and potential applications in spintronics and spin-orbitronics.
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spelling pubmed-83581632021-08-15 Extraordinary phase coherence length in epitaxial halide perovskites Nasyedkin, Kostyantyn King, Isaac Zhang, Liangji Chen, Pei Wang, Lili Staples, Richard J. Lunt, Richard R. Pollanen, Johannes iScience Article Inorganic halide perovskites have emerged as a promising platform in a wide range of applications from solar energy harvesting to computing and light emission. The recent advent of epitaxial thin film growth of halide perovskites has made it possible to investigate low-dimensional quantum electronic devices based on this class of materials. This study leverages advances in vapor-phase epitaxy of halide perovskites to perform low-temperature magnetotransport measurements on single-domain cesium tin iodide (CsSnI(3)) epitaxial thin films. The low-field magnetoresistance carries signatures of coherent quantum interference effects and spin-orbit coupling. These weak anti-localization measurements reveal a micron-scale low-temperature phase coherence length for charge carriers in this system. The results indicate that epitaxial halide perovskite heterostructures are a promising platform for investigating long coherent quantum electronic effects and potential applications in spintronics and spin-orbitronics. Elsevier 2021-07-28 /pmc/articles/PMC8358163/ /pubmed/34401682 http://dx.doi.org/10.1016/j.isci.2021.102912 Text en © 2021 The Author(s) https://creativecommons.org/licenses/by-nc-nd/4.0/This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Article
Nasyedkin, Kostyantyn
King, Isaac
Zhang, Liangji
Chen, Pei
Wang, Lili
Staples, Richard J.
Lunt, Richard R.
Pollanen, Johannes
Extraordinary phase coherence length in epitaxial halide perovskites
title Extraordinary phase coherence length in epitaxial halide perovskites
title_full Extraordinary phase coherence length in epitaxial halide perovskites
title_fullStr Extraordinary phase coherence length in epitaxial halide perovskites
title_full_unstemmed Extraordinary phase coherence length in epitaxial halide perovskites
title_short Extraordinary phase coherence length in epitaxial halide perovskites
title_sort extraordinary phase coherence length in epitaxial halide perovskites
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8358163/
https://www.ncbi.nlm.nih.gov/pubmed/34401682
http://dx.doi.org/10.1016/j.isci.2021.102912
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