Cargando…

Determination of the electronic transport in type separated carbon nanotubes thin films doped with gold nanocrystals

We report a systematic theoretical and experimental investigation on the electronic transport evolution in metallic and semiconducting carbon nanotubes thin films enriched by gold nanocrystals. We used an ultra-clean production method of both types of single-walled carbon nanotube thin films with/wi...

Descripción completa

Detalles Bibliográficos
Autores principales: Świniarski, M., Dużyńska, A., Gertych, A. P., Czerniak-Łosiewicz, K., Judek, J., Zdrojek, M.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8371105/
https://www.ncbi.nlm.nih.gov/pubmed/34404891
http://dx.doi.org/10.1038/s41598-021-96307-6
_version_ 1783739570508005376
author Świniarski, M.
Dużyńska, A.
Gertych, A. P.
Czerniak-Łosiewicz, K.
Judek, J.
Zdrojek, M.
author_facet Świniarski, M.
Dużyńska, A.
Gertych, A. P.
Czerniak-Łosiewicz, K.
Judek, J.
Zdrojek, M.
author_sort Świniarski, M.
collection PubMed
description We report a systematic theoretical and experimental investigation on the electronic transport evolution in metallic and semiconducting carbon nanotubes thin films enriched by gold nanocrystals. We used an ultra-clean production method of both types of single-walled carbon nanotube thin films with/without gold nanocrystals, which were uniformly dispersed in the whole volume of the thin films, causing a modification of the doping level of the films (verified by Raman spectroscopy). We propose a modification of the electronic transport model with the additional high-temperature features that allow us to interpret the transport within a broader temperature range and that are related to the conductivity type of carbon nanotubes. Moreover, we demonstrate, that the proposed model is also working for thin films with the addition of gold nanocrystals, and only a change of the conductivity level of our samples is observed caused by modification of potential barriers between carbon nanotubes. We also find unusual behavior of doped metallic carbon nanotube thin film, which lowers its conductivity due to doping.
format Online
Article
Text
id pubmed-8371105
institution National Center for Biotechnology Information
language English
publishDate 2021
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-83711052021-08-19 Determination of the electronic transport in type separated carbon nanotubes thin films doped with gold nanocrystals Świniarski, M. Dużyńska, A. Gertych, A. P. Czerniak-Łosiewicz, K. Judek, J. Zdrojek, M. Sci Rep Article We report a systematic theoretical and experimental investigation on the electronic transport evolution in metallic and semiconducting carbon nanotubes thin films enriched by gold nanocrystals. We used an ultra-clean production method of both types of single-walled carbon nanotube thin films with/without gold nanocrystals, which were uniformly dispersed in the whole volume of the thin films, causing a modification of the doping level of the films (verified by Raman spectroscopy). We propose a modification of the electronic transport model with the additional high-temperature features that allow us to interpret the transport within a broader temperature range and that are related to the conductivity type of carbon nanotubes. Moreover, we demonstrate, that the proposed model is also working for thin films with the addition of gold nanocrystals, and only a change of the conductivity level of our samples is observed caused by modification of potential barriers between carbon nanotubes. We also find unusual behavior of doped metallic carbon nanotube thin film, which lowers its conductivity due to doping. Nature Publishing Group UK 2021-08-17 /pmc/articles/PMC8371105/ /pubmed/34404891 http://dx.doi.org/10.1038/s41598-021-96307-6 Text en © The Author(s) 2021, corrected publication 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Świniarski, M.
Dużyńska, A.
Gertych, A. P.
Czerniak-Łosiewicz, K.
Judek, J.
Zdrojek, M.
Determination of the electronic transport in type separated carbon nanotubes thin films doped with gold nanocrystals
title Determination of the electronic transport in type separated carbon nanotubes thin films doped with gold nanocrystals
title_full Determination of the electronic transport in type separated carbon nanotubes thin films doped with gold nanocrystals
title_fullStr Determination of the electronic transport in type separated carbon nanotubes thin films doped with gold nanocrystals
title_full_unstemmed Determination of the electronic transport in type separated carbon nanotubes thin films doped with gold nanocrystals
title_short Determination of the electronic transport in type separated carbon nanotubes thin films doped with gold nanocrystals
title_sort determination of the electronic transport in type separated carbon nanotubes thin films doped with gold nanocrystals
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8371105/
https://www.ncbi.nlm.nih.gov/pubmed/34404891
http://dx.doi.org/10.1038/s41598-021-96307-6
work_keys_str_mv AT swiniarskim determinationoftheelectronictransportintypeseparatedcarbonnanotubesthinfilmsdopedwithgoldnanocrystals
AT duzynskaa determinationoftheelectronictransportintypeseparatedcarbonnanotubesthinfilmsdopedwithgoldnanocrystals
AT gertychap determinationoftheelectronictransportintypeseparatedcarbonnanotubesthinfilmsdopedwithgoldnanocrystals
AT czerniakłosiewiczk determinationoftheelectronictransportintypeseparatedcarbonnanotubesthinfilmsdopedwithgoldnanocrystals
AT judekj determinationoftheelectronictransportintypeseparatedcarbonnanotubesthinfilmsdopedwithgoldnanocrystals
AT zdrojekm determinationoftheelectronictransportintypeseparatedcarbonnanotubesthinfilmsdopedwithgoldnanocrystals