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Determination of the electronic transport in type separated carbon nanotubes thin films doped with gold nanocrystals
We report a systematic theoretical and experimental investigation on the electronic transport evolution in metallic and semiconducting carbon nanotubes thin films enriched by gold nanocrystals. We used an ultra-clean production method of both types of single-walled carbon nanotube thin films with/wi...
Autores principales: | , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2021
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8371105/ https://www.ncbi.nlm.nih.gov/pubmed/34404891 http://dx.doi.org/10.1038/s41598-021-96307-6 |
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author | Świniarski, M. Dużyńska, A. Gertych, A. P. Czerniak-Łosiewicz, K. Judek, J. Zdrojek, M. |
author_facet | Świniarski, M. Dużyńska, A. Gertych, A. P. Czerniak-Łosiewicz, K. Judek, J. Zdrojek, M. |
author_sort | Świniarski, M. |
collection | PubMed |
description | We report a systematic theoretical and experimental investigation on the electronic transport evolution in metallic and semiconducting carbon nanotubes thin films enriched by gold nanocrystals. We used an ultra-clean production method of both types of single-walled carbon nanotube thin films with/without gold nanocrystals, which were uniformly dispersed in the whole volume of the thin films, causing a modification of the doping level of the films (verified by Raman spectroscopy). We propose a modification of the electronic transport model with the additional high-temperature features that allow us to interpret the transport within a broader temperature range and that are related to the conductivity type of carbon nanotubes. Moreover, we demonstrate, that the proposed model is also working for thin films with the addition of gold nanocrystals, and only a change of the conductivity level of our samples is observed caused by modification of potential barriers between carbon nanotubes. We also find unusual behavior of doped metallic carbon nanotube thin film, which lowers its conductivity due to doping. |
format | Online Article Text |
id | pubmed-8371105 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-83711052021-08-19 Determination of the electronic transport in type separated carbon nanotubes thin films doped with gold nanocrystals Świniarski, M. Dużyńska, A. Gertych, A. P. Czerniak-Łosiewicz, K. Judek, J. Zdrojek, M. Sci Rep Article We report a systematic theoretical and experimental investigation on the electronic transport evolution in metallic and semiconducting carbon nanotubes thin films enriched by gold nanocrystals. We used an ultra-clean production method of both types of single-walled carbon nanotube thin films with/without gold nanocrystals, which were uniformly dispersed in the whole volume of the thin films, causing a modification of the doping level of the films (verified by Raman spectroscopy). We propose a modification of the electronic transport model with the additional high-temperature features that allow us to interpret the transport within a broader temperature range and that are related to the conductivity type of carbon nanotubes. Moreover, we demonstrate, that the proposed model is also working for thin films with the addition of gold nanocrystals, and only a change of the conductivity level of our samples is observed caused by modification of potential barriers between carbon nanotubes. We also find unusual behavior of doped metallic carbon nanotube thin film, which lowers its conductivity due to doping. Nature Publishing Group UK 2021-08-17 /pmc/articles/PMC8371105/ /pubmed/34404891 http://dx.doi.org/10.1038/s41598-021-96307-6 Text en © The Author(s) 2021, corrected publication 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Świniarski, M. Dużyńska, A. Gertych, A. P. Czerniak-Łosiewicz, K. Judek, J. Zdrojek, M. Determination of the electronic transport in type separated carbon nanotubes thin films doped with gold nanocrystals |
title | Determination of the electronic transport in type separated carbon nanotubes thin films doped with gold nanocrystals |
title_full | Determination of the electronic transport in type separated carbon nanotubes thin films doped with gold nanocrystals |
title_fullStr | Determination of the electronic transport in type separated carbon nanotubes thin films doped with gold nanocrystals |
title_full_unstemmed | Determination of the electronic transport in type separated carbon nanotubes thin films doped with gold nanocrystals |
title_short | Determination of the electronic transport in type separated carbon nanotubes thin films doped with gold nanocrystals |
title_sort | determination of the electronic transport in type separated carbon nanotubes thin films doped with gold nanocrystals |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8371105/ https://www.ncbi.nlm.nih.gov/pubmed/34404891 http://dx.doi.org/10.1038/s41598-021-96307-6 |
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