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Methodological and Conceptual Progresses in Studies on the Latent Tracks in PADC

Modified structure along latent tracks and track formation process have been investigated in poly (allyl diglycol carbonate), PADC, which is well recognized as a sensitive etched track detector. This knowledge is essential to develop novel detectors with improved track registration property. The tra...

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Autores principales: Yamauchi, Tomoya, Kanasaki, Masato, Barillon, Rémi
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8398540/
https://www.ncbi.nlm.nih.gov/pubmed/34451202
http://dx.doi.org/10.3390/polym13162665
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author Yamauchi, Tomoya
Kanasaki, Masato
Barillon, Rémi
author_facet Yamauchi, Tomoya
Kanasaki, Masato
Barillon, Rémi
author_sort Yamauchi, Tomoya
collection PubMed
description Modified structure along latent tracks and track formation process have been investigated in poly (allyl diglycol carbonate), PADC, which is well recognized as a sensitive etched track detector. This knowledge is essential to develop novel detectors with improved track registration property. The track structures of protons and heavy ions (He, C, Ne, Ar, Fe, Kr and Xe) have been examined by means of FT-IR spectrometry, covering the stopping power region between 1.2 to 12,000 eV/nm. Through a set of experiments on low-LET radiations—such as gamma ray-, multi-step damage process by electron hits was confirmed in the radiation-sensitive parts of the PADC repeat-unit. From this result, we unveiled for the first-time the layered structure in tracks, in relation with the number of secondary electrons. We also proved that the etch pit was formed when at least two repeat-units were destroyed along the track radial direction. To evaluate the number of secondary electrons around the tracks, a series of numerical simulations were performed with Geant4-DNA. Therefore, we are proposing new physical criterions to describe the detection thresholds. Furthermore, we propose a present issue of the definition of detection threshold for semi-relativistic C ions. Additionally, as a possible chemical criterion, formation density of hydroxyl group is suggested to express the response of PADC.
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spelling pubmed-83985402021-08-29 Methodological and Conceptual Progresses in Studies on the Latent Tracks in PADC Yamauchi, Tomoya Kanasaki, Masato Barillon, Rémi Polymers (Basel) Article Modified structure along latent tracks and track formation process have been investigated in poly (allyl diglycol carbonate), PADC, which is well recognized as a sensitive etched track detector. This knowledge is essential to develop novel detectors with improved track registration property. The track structures of protons and heavy ions (He, C, Ne, Ar, Fe, Kr and Xe) have been examined by means of FT-IR spectrometry, covering the stopping power region between 1.2 to 12,000 eV/nm. Through a set of experiments on low-LET radiations—such as gamma ray-, multi-step damage process by electron hits was confirmed in the radiation-sensitive parts of the PADC repeat-unit. From this result, we unveiled for the first-time the layered structure in tracks, in relation with the number of secondary electrons. We also proved that the etch pit was formed when at least two repeat-units were destroyed along the track radial direction. To evaluate the number of secondary electrons around the tracks, a series of numerical simulations were performed with Geant4-DNA. Therefore, we are proposing new physical criterions to describe the detection thresholds. Furthermore, we propose a present issue of the definition of detection threshold for semi-relativistic C ions. Additionally, as a possible chemical criterion, formation density of hydroxyl group is suggested to express the response of PADC. MDPI 2021-08-10 /pmc/articles/PMC8398540/ /pubmed/34451202 http://dx.doi.org/10.3390/polym13162665 Text en © 2021 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Yamauchi, Tomoya
Kanasaki, Masato
Barillon, Rémi
Methodological and Conceptual Progresses in Studies on the Latent Tracks in PADC
title Methodological and Conceptual Progresses in Studies on the Latent Tracks in PADC
title_full Methodological and Conceptual Progresses in Studies on the Latent Tracks in PADC
title_fullStr Methodological and Conceptual Progresses in Studies on the Latent Tracks in PADC
title_full_unstemmed Methodological and Conceptual Progresses in Studies on the Latent Tracks in PADC
title_short Methodological and Conceptual Progresses in Studies on the Latent Tracks in PADC
title_sort methodological and conceptual progresses in studies on the latent tracks in padc
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8398540/
https://www.ncbi.nlm.nih.gov/pubmed/34451202
http://dx.doi.org/10.3390/polym13162665
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