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Determination of X-ray detection limit and applications in perovskite X-ray detectors

X-ray detection limit and sensitivity are important figure of merits for perovskite X-ray detectors, but literatures lack a valid mathematic expression for determining the lower limit of detection for a perovskite X-ray detector. In this work, we present a thorough analysis and new method for X-ray...

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Autores principales: Pan, Lei, Shrestha, Shreetu, Taylor, Neil, Nie, Wanyi, Cao, Lei R.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8421435/
https://www.ncbi.nlm.nih.gov/pubmed/34489444
http://dx.doi.org/10.1038/s41467-021-25648-7
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author Pan, Lei
Shrestha, Shreetu
Taylor, Neil
Nie, Wanyi
Cao, Lei R.
author_facet Pan, Lei
Shrestha, Shreetu
Taylor, Neil
Nie, Wanyi
Cao, Lei R.
author_sort Pan, Lei
collection PubMed
description X-ray detection limit and sensitivity are important figure of merits for perovskite X-ray detectors, but literatures lack a valid mathematic expression for determining the lower limit of detection for a perovskite X-ray detector. In this work, we present a thorough analysis and new method for X-ray detection limit determination based on a statistical model that correlates the dark current and the X-ray induced photocurrent with the detection limit. The detection limit can be calculated through the measurement of dark current and sensitivity with an easy-to-follow practice. Alternatively, the detection limit may also be obtained by the measurement of dark current and photocurrent when repeatedly lowering the X-ray dose rate. While the material quality is critical, we show that the device architecture and working mode also have a significant influence on the sensitivity and the detection limit. Our work establishes a fair comparison metrics for material and detector development.
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spelling pubmed-84214352021-09-22 Determination of X-ray detection limit and applications in perovskite X-ray detectors Pan, Lei Shrestha, Shreetu Taylor, Neil Nie, Wanyi Cao, Lei R. Nat Commun Article X-ray detection limit and sensitivity are important figure of merits for perovskite X-ray detectors, but literatures lack a valid mathematic expression for determining the lower limit of detection for a perovskite X-ray detector. In this work, we present a thorough analysis and new method for X-ray detection limit determination based on a statistical model that correlates the dark current and the X-ray induced photocurrent with the detection limit. The detection limit can be calculated through the measurement of dark current and sensitivity with an easy-to-follow practice. Alternatively, the detection limit may also be obtained by the measurement of dark current and photocurrent when repeatedly lowering the X-ray dose rate. While the material quality is critical, we show that the device architecture and working mode also have a significant influence on the sensitivity and the detection limit. Our work establishes a fair comparison metrics for material and detector development. Nature Publishing Group UK 2021-09-06 /pmc/articles/PMC8421435/ /pubmed/34489444 http://dx.doi.org/10.1038/s41467-021-25648-7 Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Pan, Lei
Shrestha, Shreetu
Taylor, Neil
Nie, Wanyi
Cao, Lei R.
Determination of X-ray detection limit and applications in perovskite X-ray detectors
title Determination of X-ray detection limit and applications in perovskite X-ray detectors
title_full Determination of X-ray detection limit and applications in perovskite X-ray detectors
title_fullStr Determination of X-ray detection limit and applications in perovskite X-ray detectors
title_full_unstemmed Determination of X-ray detection limit and applications in perovskite X-ray detectors
title_short Determination of X-ray detection limit and applications in perovskite X-ray detectors
title_sort determination of x-ray detection limit and applications in perovskite x-ray detectors
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8421435/
https://www.ncbi.nlm.nih.gov/pubmed/34489444
http://dx.doi.org/10.1038/s41467-021-25648-7
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