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Motional narrowing, ballistic transport, and trapping of room-temperature exciton polaritons in an atomically-thin semiconductor

Monolayer transition metal dichalcogenide crystals (TMDCs) hold great promise for semiconductor optoelectronics because their bound electron-hole pairs (excitons) are stable at room temperature and interact strongly with light. When TMDCs are embedded in an optical microcavity, excitons can hybridis...

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Autores principales: Wurdack, M., Estrecho, E., Todd, S., Yun, T., Pieczarka, M., Earl, S. K., Davis, J. A., Schneider, C., Truscott, A. G., Ostrovskaya, E. A.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8433169/
https://www.ncbi.nlm.nih.gov/pubmed/34508084
http://dx.doi.org/10.1038/s41467-021-25656-7
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author Wurdack, M.
Estrecho, E.
Todd, S.
Yun, T.
Pieczarka, M.
Earl, S. K.
Davis, J. A.
Schneider, C.
Truscott, A. G.
Ostrovskaya, E. A.
author_facet Wurdack, M.
Estrecho, E.
Todd, S.
Yun, T.
Pieczarka, M.
Earl, S. K.
Davis, J. A.
Schneider, C.
Truscott, A. G.
Ostrovskaya, E. A.
author_sort Wurdack, M.
collection PubMed
description Monolayer transition metal dichalcogenide crystals (TMDCs) hold great promise for semiconductor optoelectronics because their bound electron-hole pairs (excitons) are stable at room temperature and interact strongly with light. When TMDCs are embedded in an optical microcavity, excitons can hybridise with cavity photons to form exciton polaritons, which inherit useful properties from their constituents. The ability to manipulate and trap polaritons on a microchip is critical for applications. Here, we create a non-trivial potential landscape for polaritons in monolayer WS(2), and demonstrate their trapping and ballistic propagation across tens of micrometers. We show that the effects of dielectric disorder, which restrict the diffusion of WS(2) excitons and broaden their spectral resonance, are dramatically reduced for polaritons, leading to motional narrowing and preserved partial coherence. Linewidth narrowing and coherence are further enhanced in the trap. Our results demonstrate the possibility of long-range dissipationless transport and efficient trapping of TMDC polaritons in ambient conditions.
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spelling pubmed-84331692021-09-24 Motional narrowing, ballistic transport, and trapping of room-temperature exciton polaritons in an atomically-thin semiconductor Wurdack, M. Estrecho, E. Todd, S. Yun, T. Pieczarka, M. Earl, S. K. Davis, J. A. Schneider, C. Truscott, A. G. Ostrovskaya, E. A. Nat Commun Article Monolayer transition metal dichalcogenide crystals (TMDCs) hold great promise for semiconductor optoelectronics because their bound electron-hole pairs (excitons) are stable at room temperature and interact strongly with light. When TMDCs are embedded in an optical microcavity, excitons can hybridise with cavity photons to form exciton polaritons, which inherit useful properties from their constituents. The ability to manipulate and trap polaritons on a microchip is critical for applications. Here, we create a non-trivial potential landscape for polaritons in monolayer WS(2), and demonstrate their trapping and ballistic propagation across tens of micrometers. We show that the effects of dielectric disorder, which restrict the diffusion of WS(2) excitons and broaden their spectral resonance, are dramatically reduced for polaritons, leading to motional narrowing and preserved partial coherence. Linewidth narrowing and coherence are further enhanced in the trap. Our results demonstrate the possibility of long-range dissipationless transport and efficient trapping of TMDC polaritons in ambient conditions. Nature Publishing Group UK 2021-09-10 /pmc/articles/PMC8433169/ /pubmed/34508084 http://dx.doi.org/10.1038/s41467-021-25656-7 Text en © The Author(s) 2021, corrected publication 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Wurdack, M.
Estrecho, E.
Todd, S.
Yun, T.
Pieczarka, M.
Earl, S. K.
Davis, J. A.
Schneider, C.
Truscott, A. G.
Ostrovskaya, E. A.
Motional narrowing, ballistic transport, and trapping of room-temperature exciton polaritons in an atomically-thin semiconductor
title Motional narrowing, ballistic transport, and trapping of room-temperature exciton polaritons in an atomically-thin semiconductor
title_full Motional narrowing, ballistic transport, and trapping of room-temperature exciton polaritons in an atomically-thin semiconductor
title_fullStr Motional narrowing, ballistic transport, and trapping of room-temperature exciton polaritons in an atomically-thin semiconductor
title_full_unstemmed Motional narrowing, ballistic transport, and trapping of room-temperature exciton polaritons in an atomically-thin semiconductor
title_short Motional narrowing, ballistic transport, and trapping of room-temperature exciton polaritons in an atomically-thin semiconductor
title_sort motional narrowing, ballistic transport, and trapping of room-temperature exciton polaritons in an atomically-thin semiconductor
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8433169/
https://www.ncbi.nlm.nih.gov/pubmed/34508084
http://dx.doi.org/10.1038/s41467-021-25656-7
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