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Diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids
Spontaneous emergence of organized states in materials driven by non-equilibrium conditions is of notable fundamental and technological interest. In many cases, the states are complex, and their emergence is challenging to predict. Here, we show that an unexpectedly diverse collection of dissipative...
Autores principales: | , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
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American Association for the Advancement of Science
2021
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8443174/ https://www.ncbi.nlm.nih.gov/pubmed/34524853 http://dx.doi.org/10.1126/sciadv.abh1642 |
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author | Raju, Geet Kyriakopoulos, Nikos Timonen, Jaakko V. I. |
author_facet | Raju, Geet Kyriakopoulos, Nikos Timonen, Jaakko V. I. |
author_sort | Raju, Geet |
collection | PubMed |
description | Spontaneous emergence of organized states in materials driven by non-equilibrium conditions is of notable fundamental and technological interest. In many cases, the states are complex, and their emergence is challenging to predict. Here, we show that an unexpectedly diverse collection of dissipative organized states emerges in a simple system of two liquids under planar confinement when driven by electrohydrodynamic shearing. At low shearing, a symmetry breaking at the liquid-liquid interface leads to a one-dimensional corrugation pattern. At slightly stronger shearing, topological changes give raise to the emergence of Quincke rolling filaments, filament networks, and two-dimensional bicontinuous fluidic lattices. At strong shearing, the system transitions into dissipating polygonal, toroidal, and active droplets that form dilute gas-like states at low densities and complex active emulsions at higher densities. The diversity of the observed dissipative organized states is exceptional, pointing toward non-equilibrium optical devices and new avenues in several fields of research. |
format | Online Article Text |
id | pubmed-8443174 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | American Association for the Advancement of Science |
record_format | MEDLINE/PubMed |
spelling | pubmed-84431742021-09-24 Diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids Raju, Geet Kyriakopoulos, Nikos Timonen, Jaakko V. I. Sci Adv Physical and Materials Sciences Spontaneous emergence of organized states in materials driven by non-equilibrium conditions is of notable fundamental and technological interest. In many cases, the states are complex, and their emergence is challenging to predict. Here, we show that an unexpectedly diverse collection of dissipative organized states emerges in a simple system of two liquids under planar confinement when driven by electrohydrodynamic shearing. At low shearing, a symmetry breaking at the liquid-liquid interface leads to a one-dimensional corrugation pattern. At slightly stronger shearing, topological changes give raise to the emergence of Quincke rolling filaments, filament networks, and two-dimensional bicontinuous fluidic lattices. At strong shearing, the system transitions into dissipating polygonal, toroidal, and active droplets that form dilute gas-like states at low densities and complex active emulsions at higher densities. The diversity of the observed dissipative organized states is exceptional, pointing toward non-equilibrium optical devices and new avenues in several fields of research. American Association for the Advancement of Science 2021-09-15 /pmc/articles/PMC8443174/ /pubmed/34524853 http://dx.doi.org/10.1126/sciadv.abh1642 Text en Copyright © 2021 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). https://creativecommons.org/licenses/by-nc/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (https://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited. |
spellingShingle | Physical and Materials Sciences Raju, Geet Kyriakopoulos, Nikos Timonen, Jaakko V. I. Diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids |
title | Diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids |
title_full | Diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids |
title_fullStr | Diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids |
title_full_unstemmed | Diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids |
title_short | Diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids |
title_sort | diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids |
topic | Physical and Materials Sciences |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8443174/ https://www.ncbi.nlm.nih.gov/pubmed/34524853 http://dx.doi.org/10.1126/sciadv.abh1642 |
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