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Diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids

Spontaneous emergence of organized states in materials driven by non-equilibrium conditions is of notable fundamental and technological interest. In many cases, the states are complex, and their emergence is challenging to predict. Here, we show that an unexpectedly diverse collection of dissipative...

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Detalles Bibliográficos
Autores principales: Raju, Geet, Kyriakopoulos, Nikos, Timonen, Jaakko V. I.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8443174/
https://www.ncbi.nlm.nih.gov/pubmed/34524853
http://dx.doi.org/10.1126/sciadv.abh1642
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author Raju, Geet
Kyriakopoulos, Nikos
Timonen, Jaakko V. I.
author_facet Raju, Geet
Kyriakopoulos, Nikos
Timonen, Jaakko V. I.
author_sort Raju, Geet
collection PubMed
description Spontaneous emergence of organized states in materials driven by non-equilibrium conditions is of notable fundamental and technological interest. In many cases, the states are complex, and their emergence is challenging to predict. Here, we show that an unexpectedly diverse collection of dissipative organized states emerges in a simple system of two liquids under planar confinement when driven by electrohydrodynamic shearing. At low shearing, a symmetry breaking at the liquid-liquid interface leads to a one-dimensional corrugation pattern. At slightly stronger shearing, topological changes give raise to the emergence of Quincke rolling filaments, filament networks, and two-dimensional bicontinuous fluidic lattices. At strong shearing, the system transitions into dissipating polygonal, toroidal, and active droplets that form dilute gas-like states at low densities and complex active emulsions at higher densities. The diversity of the observed dissipative organized states is exceptional, pointing toward non-equilibrium optical devices and new avenues in several fields of research.
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spelling pubmed-84431742021-09-24 Diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids Raju, Geet Kyriakopoulos, Nikos Timonen, Jaakko V. I. Sci Adv Physical and Materials Sciences Spontaneous emergence of organized states in materials driven by non-equilibrium conditions is of notable fundamental and technological interest. In many cases, the states are complex, and their emergence is challenging to predict. Here, we show that an unexpectedly diverse collection of dissipative organized states emerges in a simple system of two liquids under planar confinement when driven by electrohydrodynamic shearing. At low shearing, a symmetry breaking at the liquid-liquid interface leads to a one-dimensional corrugation pattern. At slightly stronger shearing, topological changes give raise to the emergence of Quincke rolling filaments, filament networks, and two-dimensional bicontinuous fluidic lattices. At strong shearing, the system transitions into dissipating polygonal, toroidal, and active droplets that form dilute gas-like states at low densities and complex active emulsions at higher densities. The diversity of the observed dissipative organized states is exceptional, pointing toward non-equilibrium optical devices and new avenues in several fields of research. American Association for the Advancement of Science 2021-09-15 /pmc/articles/PMC8443174/ /pubmed/34524853 http://dx.doi.org/10.1126/sciadv.abh1642 Text en Copyright © 2021 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). https://creativecommons.org/licenses/by-nc/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (https://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.
spellingShingle Physical and Materials Sciences
Raju, Geet
Kyriakopoulos, Nikos
Timonen, Jaakko V. I.
Diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids
title Diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids
title_full Diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids
title_fullStr Diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids
title_full_unstemmed Diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids
title_short Diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids
title_sort diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids
topic Physical and Materials Sciences
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8443174/
https://www.ncbi.nlm.nih.gov/pubmed/34524853
http://dx.doi.org/10.1126/sciadv.abh1642
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