Cargando…
Silver-Doped Cadmium Selenide/Graphene Oxide-Filled Cellulose Acetate Nanocomposites for Photocatalytic Degradation of Malachite Green toward Wastewater Treatment
[Image: see text] Silver-doped cadmium selenide/graphene oxide (GO) (Ag-CdSe/GO) nanocomposites have been synthesized, loaded in cellulose acetate (CA) to form Ag-CdSe/GO@CA heterostructure nanofibers, and characterized in terms of structural, morphological, photocatalytic properties, among others....
Autores principales: | , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2021
|
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8444201/ https://www.ncbi.nlm.nih.gov/pubmed/34549114 http://dx.doi.org/10.1021/acsomega.1c02667 |
_version_ | 1784568441000165376 |
---|---|
author | Ahmed, Mohamed K. Shalan, Ahmed Esmail Afifi, Mohamed El-Desoky, Mohamed M. Lanceros-Méndez, Senentxu |
author_facet | Ahmed, Mohamed K. Shalan, Ahmed Esmail Afifi, Mohamed El-Desoky, Mohamed M. Lanceros-Méndez, Senentxu |
author_sort | Ahmed, Mohamed K. |
collection | PubMed |
description | [Image: see text] Silver-doped cadmium selenide/graphene oxide (GO) (Ag-CdSe/GO) nanocomposites have been synthesized, loaded in cellulose acetate (CA) to form Ag-CdSe/GO@CA heterostructure nanofibers, and characterized in terms of structural, morphological, photocatalytic properties, among others. The photocatalytic degradation of malachite green (MG) was estimated using cadmium selenide-filled CA (CdSe@CA), silver-doped cadmium selenide-filled CA (Ag-CdSe@CA), cadmium selenide/GO-filled CA (CdSe/GO@CA), and silver-doped cadmium selenide/GO-filled CA (Ag-CdSe/GO@CA) nanocomposite materials. The Ag-CdSe/GO@CA nanocomposites exhibit and retain an enhanced photocatalytic activity for the degradation of MG dye. This amended performance is associated with the multifunctional supporting impacts of GO, Ag, and CA on the composite structure and properties. The superior photocatalytic activity is related to the fact that both Ag and GO can act as electron acceptors that boost the separation efficiency of photogenerated carriers and the loading of the combined nanocomposite (Ag-CdSe@GO) on CA nanofibers, which can augment the adsorption of electrons and holes and facilitate the movement of carriers. The stability of Ag-CdSe/GO@CA nanocomposite photocatalysts demonstrates suitable results even after five recycles. This study establishes an advanced semiconductor-based hybrid nanocomposite material for efficient photocatalytic degradation of organic dyes. |
format | Online Article Text |
id | pubmed-8444201 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-84442012021-09-20 Silver-Doped Cadmium Selenide/Graphene Oxide-Filled Cellulose Acetate Nanocomposites for Photocatalytic Degradation of Malachite Green toward Wastewater Treatment Ahmed, Mohamed K. Shalan, Ahmed Esmail Afifi, Mohamed El-Desoky, Mohamed M. Lanceros-Méndez, Senentxu ACS Omega [Image: see text] Silver-doped cadmium selenide/graphene oxide (GO) (Ag-CdSe/GO) nanocomposites have been synthesized, loaded in cellulose acetate (CA) to form Ag-CdSe/GO@CA heterostructure nanofibers, and characterized in terms of structural, morphological, photocatalytic properties, among others. The photocatalytic degradation of malachite green (MG) was estimated using cadmium selenide-filled CA (CdSe@CA), silver-doped cadmium selenide-filled CA (Ag-CdSe@CA), cadmium selenide/GO-filled CA (CdSe/GO@CA), and silver-doped cadmium selenide/GO-filled CA (Ag-CdSe/GO@CA) nanocomposite materials. The Ag-CdSe/GO@CA nanocomposites exhibit and retain an enhanced photocatalytic activity for the degradation of MG dye. This amended performance is associated with the multifunctional supporting impacts of GO, Ag, and CA on the composite structure and properties. The superior photocatalytic activity is related to the fact that both Ag and GO can act as electron acceptors that boost the separation efficiency of photogenerated carriers and the loading of the combined nanocomposite (Ag-CdSe@GO) on CA nanofibers, which can augment the adsorption of electrons and holes and facilitate the movement of carriers. The stability of Ag-CdSe/GO@CA nanocomposite photocatalysts demonstrates suitable results even after five recycles. This study establishes an advanced semiconductor-based hybrid nanocomposite material for efficient photocatalytic degradation of organic dyes. American Chemical Society 2021-08-29 /pmc/articles/PMC8444201/ /pubmed/34549114 http://dx.doi.org/10.1021/acsomega.1c02667 Text en © 2021 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/). |
spellingShingle | Ahmed, Mohamed K. Shalan, Ahmed Esmail Afifi, Mohamed El-Desoky, Mohamed M. Lanceros-Méndez, Senentxu Silver-Doped Cadmium Selenide/Graphene Oxide-Filled Cellulose Acetate Nanocomposites for Photocatalytic Degradation of Malachite Green toward Wastewater Treatment |
title | Silver-Doped Cadmium Selenide/Graphene Oxide-Filled
Cellulose Acetate Nanocomposites for Photocatalytic Degradation of
Malachite Green toward Wastewater Treatment |
title_full | Silver-Doped Cadmium Selenide/Graphene Oxide-Filled
Cellulose Acetate Nanocomposites for Photocatalytic Degradation of
Malachite Green toward Wastewater Treatment |
title_fullStr | Silver-Doped Cadmium Selenide/Graphene Oxide-Filled
Cellulose Acetate Nanocomposites for Photocatalytic Degradation of
Malachite Green toward Wastewater Treatment |
title_full_unstemmed | Silver-Doped Cadmium Selenide/Graphene Oxide-Filled
Cellulose Acetate Nanocomposites for Photocatalytic Degradation of
Malachite Green toward Wastewater Treatment |
title_short | Silver-Doped Cadmium Selenide/Graphene Oxide-Filled
Cellulose Acetate Nanocomposites for Photocatalytic Degradation of
Malachite Green toward Wastewater Treatment |
title_sort | silver-doped cadmium selenide/graphene oxide-filled
cellulose acetate nanocomposites for photocatalytic degradation of
malachite green toward wastewater treatment |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8444201/ https://www.ncbi.nlm.nih.gov/pubmed/34549114 http://dx.doi.org/10.1021/acsomega.1c02667 |
work_keys_str_mv | AT ahmedmohamedk silverdopedcadmiumselenidegrapheneoxidefilledcelluloseacetatenanocompositesforphotocatalyticdegradationofmalachitegreentowardwastewatertreatment AT shalanahmedesmail silverdopedcadmiumselenidegrapheneoxidefilledcelluloseacetatenanocompositesforphotocatalyticdegradationofmalachitegreentowardwastewatertreatment AT afifimohamed silverdopedcadmiumselenidegrapheneoxidefilledcelluloseacetatenanocompositesforphotocatalyticdegradationofmalachitegreentowardwastewatertreatment AT eldesokymohamedm silverdopedcadmiumselenidegrapheneoxidefilledcelluloseacetatenanocompositesforphotocatalyticdegradationofmalachitegreentowardwastewatertreatment AT lancerosmendezsenentxu silverdopedcadmiumselenidegrapheneoxidefilledcelluloseacetatenanocompositesforphotocatalyticdegradationofmalachitegreentowardwastewatertreatment |