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Study on Soot Emission Characteristics of Methane/Oxygen Inverse Diffusion Flame

[Image: see text] Inverse diffusion flame (IDF) is an effective and widely used reaction form in the process of noncatalytic partial oxidation (NC-POX) of gaseous hydrocarbons (such as natural gas and coke oven gas). However, soot is generated in the combustion chamber in the case of unreasonable fe...

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Autores principales: Wu, Runmin, Xie, Fei, Wei, Juntao, Song, Xudong, Yang, Huijun, Lv, Peng, Yu, Guangsuo
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2021
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8444205/
https://www.ncbi.nlm.nih.gov/pubmed/34549120
http://dx.doi.org/10.1021/acsomega.1c02789
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author Wu, Runmin
Xie, Fei
Wei, Juntao
Song, Xudong
Yang, Huijun
Lv, Peng
Yu, Guangsuo
author_facet Wu, Runmin
Xie, Fei
Wei, Juntao
Song, Xudong
Yang, Huijun
Lv, Peng
Yu, Guangsuo
author_sort Wu, Runmin
collection PubMed
description [Image: see text] Inverse diffusion flame (IDF) is an effective and widely used reaction form in the process of noncatalytic partial oxidation (NC-POX) of gaseous hydrocarbons (such as natural gas and coke oven gas). However, soot is generated in the combustion chamber in the case of unreasonable feeding conditions, and thus causes serious damage to the wall and nozzle. In this study, the effects of the equivalence ratio ([O/C](e)), the oxygen flow rate, and the Reynolds number on the soot and CH* emission characteristics of CH(4)/O(2) inverse diffusion flame were comprehensively analyzed based on a hyperspectral imaging system. In addition, the relationship between CH* and soot is explored using Ansys Fluent simulation. The experimental results show that the soot radiation core generation area is located in the outer ring of the flame, and the radial distribution of the radiation intensity is bimodal. With the increase in [O/C](e), the initial position for soot radiation and the overall radiation intensity of soot decrease. In addition, the CH* radiation intensity decreases as [O/C](e) increases, and CH* exists in the whole flame. The simulation results clearly show that the existence of CH* is conducive to soot production. The emission intensity and the core area of soot formation increase with the increase in the oxygen velocity. Additionally, the soot emission region increases and the flame tip changes from a round blunt to symmetrical tip with the increase in the Reynolds number.
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spelling pubmed-84442052021-09-20 Study on Soot Emission Characteristics of Methane/Oxygen Inverse Diffusion Flame Wu, Runmin Xie, Fei Wei, Juntao Song, Xudong Yang, Huijun Lv, Peng Yu, Guangsuo ACS Omega [Image: see text] Inverse diffusion flame (IDF) is an effective and widely used reaction form in the process of noncatalytic partial oxidation (NC-POX) of gaseous hydrocarbons (such as natural gas and coke oven gas). However, soot is generated in the combustion chamber in the case of unreasonable feeding conditions, and thus causes serious damage to the wall and nozzle. In this study, the effects of the equivalence ratio ([O/C](e)), the oxygen flow rate, and the Reynolds number on the soot and CH* emission characteristics of CH(4)/O(2) inverse diffusion flame were comprehensively analyzed based on a hyperspectral imaging system. In addition, the relationship between CH* and soot is explored using Ansys Fluent simulation. The experimental results show that the soot radiation core generation area is located in the outer ring of the flame, and the radial distribution of the radiation intensity is bimodal. With the increase in [O/C](e), the initial position for soot radiation and the overall radiation intensity of soot decrease. In addition, the CH* radiation intensity decreases as [O/C](e) increases, and CH* exists in the whole flame. The simulation results clearly show that the existence of CH* is conducive to soot production. The emission intensity and the core area of soot formation increase with the increase in the oxygen velocity. Additionally, the soot emission region increases and the flame tip changes from a round blunt to symmetrical tip with the increase in the Reynolds number. American Chemical Society 2021-08-31 /pmc/articles/PMC8444205/ /pubmed/34549120 http://dx.doi.org/10.1021/acsomega.1c02789 Text en © 2021 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Wu, Runmin
Xie, Fei
Wei, Juntao
Song, Xudong
Yang, Huijun
Lv, Peng
Yu, Guangsuo
Study on Soot Emission Characteristics of Methane/Oxygen Inverse Diffusion Flame
title Study on Soot Emission Characteristics of Methane/Oxygen Inverse Diffusion Flame
title_full Study on Soot Emission Characteristics of Methane/Oxygen Inverse Diffusion Flame
title_fullStr Study on Soot Emission Characteristics of Methane/Oxygen Inverse Diffusion Flame
title_full_unstemmed Study on Soot Emission Characteristics of Methane/Oxygen Inverse Diffusion Flame
title_short Study on Soot Emission Characteristics of Methane/Oxygen Inverse Diffusion Flame
title_sort study on soot emission characteristics of methane/oxygen inverse diffusion flame
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8444205/
https://www.ncbi.nlm.nih.gov/pubmed/34549120
http://dx.doi.org/10.1021/acsomega.1c02789
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