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Lattice reconstruction induced multiple ultra-flat bands in twisted bilayer WSe(2)

Moiré superlattices in van der Waals heterostructures provide a tunable platform to study emergent properties that are absent in the natural crystal form. Twisted bilayer transition metal dichalcogenides (TB-TMDs) can host moiré flat bands over a wide range of twist angles. For twist angle close to...

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Autores principales: Li, En, Hu, Jin-Xin, Feng, Xuemeng, Zhou, Zishu, An, Liheng, Law, Kam Tuen, Wang, Ning, Lin, Nian
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8460827/
https://www.ncbi.nlm.nih.gov/pubmed/34556663
http://dx.doi.org/10.1038/s41467-021-25924-6
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author Li, En
Hu, Jin-Xin
Feng, Xuemeng
Zhou, Zishu
An, Liheng
Law, Kam Tuen
Wang, Ning
Lin, Nian
author_facet Li, En
Hu, Jin-Xin
Feng, Xuemeng
Zhou, Zishu
An, Liheng
Law, Kam Tuen
Wang, Ning
Lin, Nian
author_sort Li, En
collection PubMed
description Moiré superlattices in van der Waals heterostructures provide a tunable platform to study emergent properties that are absent in the natural crystal form. Twisted bilayer transition metal dichalcogenides (TB-TMDs) can host moiré flat bands over a wide range of twist angles. For twist angle close to 60°, it was predicted that TB-TMDs undergo a lattice reconstruction which causes the formation of ultra-flat bands. Here, by using scanning tunneling microscopy and spectroscopy, we show the emergence of multiple ultra-flat bands in twisted bilayer WSe(2) when the twist angle is within 3° of 60°. The ultra-flat bands are manifested as narrow tunneling conductance peaks with estimated bandwidth less than 10 meV, which is only a fraction of the estimated on-site Coulomb repulsion energy. The number of these ultra-flat bands and spatial distribution of the wavefunctions match well with the theoretical predictions, strongly evidencing that the observed ultra-flat bands are induced by lattice reconstruction. Our work provides a foundation for further study of the exotic correlated phases in TB-TMDs.
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spelling pubmed-84608272021-10-22 Lattice reconstruction induced multiple ultra-flat bands in twisted bilayer WSe(2) Li, En Hu, Jin-Xin Feng, Xuemeng Zhou, Zishu An, Liheng Law, Kam Tuen Wang, Ning Lin, Nian Nat Commun Article Moiré superlattices in van der Waals heterostructures provide a tunable platform to study emergent properties that are absent in the natural crystal form. Twisted bilayer transition metal dichalcogenides (TB-TMDs) can host moiré flat bands over a wide range of twist angles. For twist angle close to 60°, it was predicted that TB-TMDs undergo a lattice reconstruction which causes the formation of ultra-flat bands. Here, by using scanning tunneling microscopy and spectroscopy, we show the emergence of multiple ultra-flat bands in twisted bilayer WSe(2) when the twist angle is within 3° of 60°. The ultra-flat bands are manifested as narrow tunneling conductance peaks with estimated bandwidth less than 10 meV, which is only a fraction of the estimated on-site Coulomb repulsion energy. The number of these ultra-flat bands and spatial distribution of the wavefunctions match well with the theoretical predictions, strongly evidencing that the observed ultra-flat bands are induced by lattice reconstruction. Our work provides a foundation for further study of the exotic correlated phases in TB-TMDs. Nature Publishing Group UK 2021-09-23 /pmc/articles/PMC8460827/ /pubmed/34556663 http://dx.doi.org/10.1038/s41467-021-25924-6 Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Li, En
Hu, Jin-Xin
Feng, Xuemeng
Zhou, Zishu
An, Liheng
Law, Kam Tuen
Wang, Ning
Lin, Nian
Lattice reconstruction induced multiple ultra-flat bands in twisted bilayer WSe(2)
title Lattice reconstruction induced multiple ultra-flat bands in twisted bilayer WSe(2)
title_full Lattice reconstruction induced multiple ultra-flat bands in twisted bilayer WSe(2)
title_fullStr Lattice reconstruction induced multiple ultra-flat bands in twisted bilayer WSe(2)
title_full_unstemmed Lattice reconstruction induced multiple ultra-flat bands in twisted bilayer WSe(2)
title_short Lattice reconstruction induced multiple ultra-flat bands in twisted bilayer WSe(2)
title_sort lattice reconstruction induced multiple ultra-flat bands in twisted bilayer wse(2)
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8460827/
https://www.ncbi.nlm.nih.gov/pubmed/34556663
http://dx.doi.org/10.1038/s41467-021-25924-6
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