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A General and Predictive Understanding of Thermal Transport from 1D- and 2D-Confined Nanostructures: Theory and Experiment

[Image: see text] Heat management is crucial in the design of nanoscale devices as the operating temperature determines their efficiency and lifetime. Past experimental and theoretical works exploring nanoscale heat transport in semiconductors addressed known deviations from Fourier’s law modeling b...

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Autores principales: Beardo, Albert, Knobloch, Joshua L., Sendra, Lluc, Bafaluy, Javier, Frazer, Travis D., Chao, Weilun, Hernandez-Charpak, Jorge N., Kapteyn, Henry C., Abad, Begoña, Murnane, Margaret M., Alvarez, F. Xavier, Camacho, Juan
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2021
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8483436/
https://www.ncbi.nlm.nih.gov/pubmed/34328719
http://dx.doi.org/10.1021/acsnano.1c01946
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author Beardo, Albert
Knobloch, Joshua L.
Sendra, Lluc
Bafaluy, Javier
Frazer, Travis D.
Chao, Weilun
Hernandez-Charpak, Jorge N.
Kapteyn, Henry C.
Abad, Begoña
Murnane, Margaret M.
Alvarez, F. Xavier
Camacho, Juan
author_facet Beardo, Albert
Knobloch, Joshua L.
Sendra, Lluc
Bafaluy, Javier
Frazer, Travis D.
Chao, Weilun
Hernandez-Charpak, Jorge N.
Kapteyn, Henry C.
Abad, Begoña
Murnane, Margaret M.
Alvarez, F. Xavier
Camacho, Juan
author_sort Beardo, Albert
collection PubMed
description [Image: see text] Heat management is crucial in the design of nanoscale devices as the operating temperature determines their efficiency and lifetime. Past experimental and theoretical works exploring nanoscale heat transport in semiconductors addressed known deviations from Fourier’s law modeling by including effective parameters, such as a size-dependent thermal conductivity. However, recent experiments have qualitatively shown behavior that cannot be modeled in this way. Here, we combine advanced experiment and theory to show that the cooling of 1D- and 2D-confined nanoscale hot spots on silicon can be described using a general hydrodynamic heat transport model, contrary to previous understanding of heat flow in bulk silicon. We use a comprehensive set of extreme ultraviolet scatterometry measurements of nondiffusive transport from transiently heated nanolines and nanodots to validate and generalize our ab initio model, that does not need any geometry-dependent fitting parameters. This allows us to uncover the existence of two distinct time scales and heat transport mechanisms: an interface resistance regime that dominates on short time scales and a hydrodynamic-like phonon transport regime that dominates on longer time scales. Moreover, our model can predict the full thermomechanical response on nanometer length scales and picosecond time scales for arbitrary geometries, providing an advanced practical tool for thermal management of nanoscale technologies. Furthermore, we derive analytical expressions for the transport time scales, valid for a subset of geometries, supplying a route for optimizing heat dissipation.
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spelling pubmed-84834362021-10-01 A General and Predictive Understanding of Thermal Transport from 1D- and 2D-Confined Nanostructures: Theory and Experiment Beardo, Albert Knobloch, Joshua L. Sendra, Lluc Bafaluy, Javier Frazer, Travis D. Chao, Weilun Hernandez-Charpak, Jorge N. Kapteyn, Henry C. Abad, Begoña Murnane, Margaret M. Alvarez, F. Xavier Camacho, Juan ACS Nano [Image: see text] Heat management is crucial in the design of nanoscale devices as the operating temperature determines their efficiency and lifetime. Past experimental and theoretical works exploring nanoscale heat transport in semiconductors addressed known deviations from Fourier’s law modeling by including effective parameters, such as a size-dependent thermal conductivity. However, recent experiments have qualitatively shown behavior that cannot be modeled in this way. Here, we combine advanced experiment and theory to show that the cooling of 1D- and 2D-confined nanoscale hot spots on silicon can be described using a general hydrodynamic heat transport model, contrary to previous understanding of heat flow in bulk silicon. We use a comprehensive set of extreme ultraviolet scatterometry measurements of nondiffusive transport from transiently heated nanolines and nanodots to validate and generalize our ab initio model, that does not need any geometry-dependent fitting parameters. This allows us to uncover the existence of two distinct time scales and heat transport mechanisms: an interface resistance regime that dominates on short time scales and a hydrodynamic-like phonon transport regime that dominates on longer time scales. Moreover, our model can predict the full thermomechanical response on nanometer length scales and picosecond time scales for arbitrary geometries, providing an advanced practical tool for thermal management of nanoscale technologies. Furthermore, we derive analytical expressions for the transport time scales, valid for a subset of geometries, supplying a route for optimizing heat dissipation. American Chemical Society 2021-07-30 2021-08-24 /pmc/articles/PMC8483436/ /pubmed/34328719 http://dx.doi.org/10.1021/acsnano.1c01946 Text en © 2021 American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Beardo, Albert
Knobloch, Joshua L.
Sendra, Lluc
Bafaluy, Javier
Frazer, Travis D.
Chao, Weilun
Hernandez-Charpak, Jorge N.
Kapteyn, Henry C.
Abad, Begoña
Murnane, Margaret M.
Alvarez, F. Xavier
Camacho, Juan
A General and Predictive Understanding of Thermal Transport from 1D- and 2D-Confined Nanostructures: Theory and Experiment
title A General and Predictive Understanding of Thermal Transport from 1D- and 2D-Confined Nanostructures: Theory and Experiment
title_full A General and Predictive Understanding of Thermal Transport from 1D- and 2D-Confined Nanostructures: Theory and Experiment
title_fullStr A General and Predictive Understanding of Thermal Transport from 1D- and 2D-Confined Nanostructures: Theory and Experiment
title_full_unstemmed A General and Predictive Understanding of Thermal Transport from 1D- and 2D-Confined Nanostructures: Theory and Experiment
title_short A General and Predictive Understanding of Thermal Transport from 1D- and 2D-Confined Nanostructures: Theory and Experiment
title_sort a general and predictive understanding of thermal transport from 1d- and 2d-confined nanostructures: theory and experiment
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8483436/
https://www.ncbi.nlm.nih.gov/pubmed/34328719
http://dx.doi.org/10.1021/acsnano.1c01946
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