Kinetic arrest of the ferromagnetic state in Mn[Formula: see text] GaC and Ni[Formula: see text] MnGa composite mixtures

The kinetics of the ferromagnetic to antiferromagnetic transition in Mn[Formula: see text] GaC can be arrested and its magnetic properties can be tuned by mixing a small amount ([Formula: see text] 10%) of Heusler Ni[Formula: see text] MnGa to Mn[Formula: see text] GaC. A detailed study of magnetic properties of composite mixtures of Mn[Formula: see text] GaC and Ni[Formula: see text] MnGa with different antiperovskite to Heusler ratio, reveals that the ferromagnetic Ni[Formula: see text] MnGa polarizes magnetic spins of the antiperovskite phase by creating a magnetic strain field in its vicinity. The Heusler phase acts as a defect centre whose influence on the magnetic properties of the majority antiperovskite phase progressively diminishes, creating a distribution of transition temperatures. Such strong interaction between the two phases of the mixture allows for tunability and control over the properties of such magneto-structurally transforming materials.