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Mass flow and momentum flux in nanoporous membranes in the transitional flow region

An experimental study of momentum transfer in nanoporous polymeric track-etched membranes with pore diameters ranging from 100 to 1300 nm and nanochannel lengths of 12–20 μm was performed using He, N(2), CO(2), and SF(6) propellants in a wide range of plenum and background pressures. Mass flux throu...

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Autores principales: Podgolin, Stepan K., Petukhov, Dmitrii I., Loimer, Thomas, Eliseev, Andrei A.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society of Chemistry 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8489186/
https://www.ncbi.nlm.nih.gov/pubmed/34369508
http://dx.doi.org/10.1039/d1cp02797b
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author Podgolin, Stepan K.
Petukhov, Dmitrii I.
Loimer, Thomas
Eliseev, Andrei A.
author_facet Podgolin, Stepan K.
Petukhov, Dmitrii I.
Loimer, Thomas
Eliseev, Andrei A.
author_sort Podgolin, Stepan K.
collection PubMed
description An experimental study of momentum transfer in nanoporous polymeric track-etched membranes with pore diameters ranging from 100 to 1300 nm and nanochannel lengths of 12–20 μm was performed using He, N(2), CO(2), and SF(6) propellants in a wide range of plenum and background pressures. Mass flux through the membranes was elaborated as a combination of Knudsen diffusion and viscous flow at Knudsen numbers above 0.1 and become choked at lower Knudsen numbers. The discharge coefficient for the membranes attained was 0.6, making the permeation rate similar to that of thin orifices. The effect is attributed to the mirror reflection of the molecules from the pore walls at low angles of incidence. The exhaust gas velocity is found to be dependent on the plenum to background pressure ratio and channel length-to-diameter ratio, reaching 0.9 of the velocity of the gas expanded to vacuum (up to 2 M). Close to an isothermal expansion occurs in nanochannels of all sizes. A general quantitative description for gas expansion in nanochannels is provided. The highest thrust is generated in the choked flow regime with the SF(6) propellant and a value of 4.5 N cm(−2) is attained at a propellant consumption of 0.165 kg (cm(2) s)(−1) for the membranes with 1300 nm nanochannels. The specific impulse of 138 s is reached for helium. The results show the prospects of the utilization of nanoporous membranes in cold gas propulsion systems.
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spelling pubmed-84891862021-10-25 Mass flow and momentum flux in nanoporous membranes in the transitional flow region Podgolin, Stepan K. Petukhov, Dmitrii I. Loimer, Thomas Eliseev, Andrei A. Phys Chem Chem Phys Chemistry An experimental study of momentum transfer in nanoporous polymeric track-etched membranes with pore diameters ranging from 100 to 1300 nm and nanochannel lengths of 12–20 μm was performed using He, N(2), CO(2), and SF(6) propellants in a wide range of plenum and background pressures. Mass flux through the membranes was elaborated as a combination of Knudsen diffusion and viscous flow at Knudsen numbers above 0.1 and become choked at lower Knudsen numbers. The discharge coefficient for the membranes attained was 0.6, making the permeation rate similar to that of thin orifices. The effect is attributed to the mirror reflection of the molecules from the pore walls at low angles of incidence. The exhaust gas velocity is found to be dependent on the plenum to background pressure ratio and channel length-to-diameter ratio, reaching 0.9 of the velocity of the gas expanded to vacuum (up to 2 M). Close to an isothermal expansion occurs in nanochannels of all sizes. A general quantitative description for gas expansion in nanochannels is provided. The highest thrust is generated in the choked flow regime with the SF(6) propellant and a value of 4.5 N cm(−2) is attained at a propellant consumption of 0.165 kg (cm(2) s)(−1) for the membranes with 1300 nm nanochannels. The specific impulse of 138 s is reached for helium. The results show the prospects of the utilization of nanoporous membranes in cold gas propulsion systems. The Royal Society of Chemistry 2021-07-26 /pmc/articles/PMC8489186/ /pubmed/34369508 http://dx.doi.org/10.1039/d1cp02797b Text en This journal is © the Owner Societies https://creativecommons.org/licenses/by/3.0/
spellingShingle Chemistry
Podgolin, Stepan K.
Petukhov, Dmitrii I.
Loimer, Thomas
Eliseev, Andrei A.
Mass flow and momentum flux in nanoporous membranes in the transitional flow region
title Mass flow and momentum flux in nanoporous membranes in the transitional flow region
title_full Mass flow and momentum flux in nanoporous membranes in the transitional flow region
title_fullStr Mass flow and momentum flux in nanoporous membranes in the transitional flow region
title_full_unstemmed Mass flow and momentum flux in nanoporous membranes in the transitional flow region
title_short Mass flow and momentum flux in nanoporous membranes in the transitional flow region
title_sort mass flow and momentum flux in nanoporous membranes in the transitional flow region
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8489186/
https://www.ncbi.nlm.nih.gov/pubmed/34369508
http://dx.doi.org/10.1039/d1cp02797b
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