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Quasi-Guided Modes in Titanium Dioxide Arrays Fabricated via Soft Nanoimprint Lithography

[Image: see text] Reversible quasi-guided modes (QGMs) are observed in titanium dioxide (TiO(2)) metasurface arrays fabricated via soft nanoimprint lithography. A TiO(2) layer between the nanopillar array and the substrate can facilitate the propagation of QGMs. This layer is porous, allowing for th...

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Autores principales: Garcia, Jorge A., Hrelescu, Calin, Zhang, Xia, Grosso, David, Abbarchi, Marco, Bradley, A. Louise
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2021
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8517955/
https://www.ncbi.nlm.nih.gov/pubmed/34591453
http://dx.doi.org/10.1021/acsami.1c11456
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author Garcia, Jorge A.
Hrelescu, Calin
Zhang, Xia
Grosso, David
Abbarchi, Marco
Bradley, A. Louise
author_facet Garcia, Jorge A.
Hrelescu, Calin
Zhang, Xia
Grosso, David
Abbarchi, Marco
Bradley, A. Louise
author_sort Garcia, Jorge A.
collection PubMed
description [Image: see text] Reversible quasi-guided modes (QGMs) are observed in titanium dioxide (TiO(2)) metasurface arrays fabricated via soft nanoimprint lithography. A TiO(2) layer between the nanopillar array and the substrate can facilitate the propagation of QGMs. This layer is porous, allowing for the tuning of the layer properties by incorporating another material. The presence of the QGMs is strongly dependent on the refractive index of the TiO(2) layer. QGMs are not supported if the refractive index of the porous TiO(2) is too low. It is demonstrated that after depositing R6G on the array QGMs can be observed as very strong and narrow reflectance peaks and transmittance dips. Furthermore, as the second material can penetrate through the pores into the layer it can experience the regions of high field enhancement associated with the QGMs. These results are of interest for a wide range of applications including but not limited to sensing, nonlinear optics, and emission control.
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spelling pubmed-85179552021-10-15 Quasi-Guided Modes in Titanium Dioxide Arrays Fabricated via Soft Nanoimprint Lithography Garcia, Jorge A. Hrelescu, Calin Zhang, Xia Grosso, David Abbarchi, Marco Bradley, A. Louise ACS Appl Mater Interfaces [Image: see text] Reversible quasi-guided modes (QGMs) are observed in titanium dioxide (TiO(2)) metasurface arrays fabricated via soft nanoimprint lithography. A TiO(2) layer between the nanopillar array and the substrate can facilitate the propagation of QGMs. This layer is porous, allowing for the tuning of the layer properties by incorporating another material. The presence of the QGMs is strongly dependent on the refractive index of the TiO(2) layer. QGMs are not supported if the refractive index of the porous TiO(2) is too low. It is demonstrated that after depositing R6G on the array QGMs can be observed as very strong and narrow reflectance peaks and transmittance dips. Furthermore, as the second material can penetrate through the pores into the layer it can experience the regions of high field enhancement associated with the QGMs. These results are of interest for a wide range of applications including but not limited to sensing, nonlinear optics, and emission control. American Chemical Society 2021-09-30 2021-10-13 /pmc/articles/PMC8517955/ /pubmed/34591453 http://dx.doi.org/10.1021/acsami.1c11456 Text en © 2021 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Garcia, Jorge A.
Hrelescu, Calin
Zhang, Xia
Grosso, David
Abbarchi, Marco
Bradley, A. Louise
Quasi-Guided Modes in Titanium Dioxide Arrays Fabricated via Soft Nanoimprint Lithography
title Quasi-Guided Modes in Titanium Dioxide Arrays Fabricated via Soft Nanoimprint Lithography
title_full Quasi-Guided Modes in Titanium Dioxide Arrays Fabricated via Soft Nanoimprint Lithography
title_fullStr Quasi-Guided Modes in Titanium Dioxide Arrays Fabricated via Soft Nanoimprint Lithography
title_full_unstemmed Quasi-Guided Modes in Titanium Dioxide Arrays Fabricated via Soft Nanoimprint Lithography
title_short Quasi-Guided Modes in Titanium Dioxide Arrays Fabricated via Soft Nanoimprint Lithography
title_sort quasi-guided modes in titanium dioxide arrays fabricated via soft nanoimprint lithography
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8517955/
https://www.ncbi.nlm.nih.gov/pubmed/34591453
http://dx.doi.org/10.1021/acsami.1c11456
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