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Bright single photon emitters with enhanced quantum efficiency in a two-dimensional semiconductor coupled with dielectric nano-antennas

Single photon emitters in atomically-thin semiconductors can be deterministically positioned using strain induced by underlying nano-structures. Here, we couple monolayer WSe(2) to high-refractive-index gallium phosphide dielectric nano-antennas providing both optical enhancement and monolayer defor...

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Autores principales: Sortino, Luca, Zotev, Panaiot G., Phillips, Catherine L., Brash, Alistair J., Cambiasso, Javier, Marensi, Elena, Fox, A. Mark, Maier, Stefan A., Sapienza, Riccardo, Tartakovskii, Alexander I.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8523570/
https://www.ncbi.nlm.nih.gov/pubmed/34663795
http://dx.doi.org/10.1038/s41467-021-26262-3
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author Sortino, Luca
Zotev, Panaiot G.
Phillips, Catherine L.
Brash, Alistair J.
Cambiasso, Javier
Marensi, Elena
Fox, A. Mark
Maier, Stefan A.
Sapienza, Riccardo
Tartakovskii, Alexander I.
author_facet Sortino, Luca
Zotev, Panaiot G.
Phillips, Catherine L.
Brash, Alistair J.
Cambiasso, Javier
Marensi, Elena
Fox, A. Mark
Maier, Stefan A.
Sapienza, Riccardo
Tartakovskii, Alexander I.
author_sort Sortino, Luca
collection PubMed
description Single photon emitters in atomically-thin semiconductors can be deterministically positioned using strain induced by underlying nano-structures. Here, we couple monolayer WSe(2) to high-refractive-index gallium phosphide dielectric nano-antennas providing both optical enhancement and monolayer deformation. For single photon emitters formed on such nano-antennas, we find very low (femto-Joule) saturation pulse energies and up to 10(4) times brighter photoluminescence than in WSe(2) placed on low-refractive-index SiO(2) pillars. We show that the key to these observations is the increase on average by a factor of 5 of the quantum efficiency of the emitters coupled to the nano-antennas. This further allows us to gain new insights into their photoluminescence dynamics, revealing the roles of the dark exciton reservoir and Auger processes. We also find that the coherence time of such emitters is limited by intrinsic dephasing processes. Our work establishes dielectric nano-antennas as a platform for high-efficiency quantum light generation in monolayer semiconductors.
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spelling pubmed-85235702021-11-15 Bright single photon emitters with enhanced quantum efficiency in a two-dimensional semiconductor coupled with dielectric nano-antennas Sortino, Luca Zotev, Panaiot G. Phillips, Catherine L. Brash, Alistair J. Cambiasso, Javier Marensi, Elena Fox, A. Mark Maier, Stefan A. Sapienza, Riccardo Tartakovskii, Alexander I. Nat Commun Article Single photon emitters in atomically-thin semiconductors can be deterministically positioned using strain induced by underlying nano-structures. Here, we couple monolayer WSe(2) to high-refractive-index gallium phosphide dielectric nano-antennas providing both optical enhancement and monolayer deformation. For single photon emitters formed on such nano-antennas, we find very low (femto-Joule) saturation pulse energies and up to 10(4) times brighter photoluminescence than in WSe(2) placed on low-refractive-index SiO(2) pillars. We show that the key to these observations is the increase on average by a factor of 5 of the quantum efficiency of the emitters coupled to the nano-antennas. This further allows us to gain new insights into their photoluminescence dynamics, revealing the roles of the dark exciton reservoir and Auger processes. We also find that the coherence time of such emitters is limited by intrinsic dephasing processes. Our work establishes dielectric nano-antennas as a platform for high-efficiency quantum light generation in monolayer semiconductors. Nature Publishing Group UK 2021-10-18 /pmc/articles/PMC8523570/ /pubmed/34663795 http://dx.doi.org/10.1038/s41467-021-26262-3 Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Sortino, Luca
Zotev, Panaiot G.
Phillips, Catherine L.
Brash, Alistair J.
Cambiasso, Javier
Marensi, Elena
Fox, A. Mark
Maier, Stefan A.
Sapienza, Riccardo
Tartakovskii, Alexander I.
Bright single photon emitters with enhanced quantum efficiency in a two-dimensional semiconductor coupled with dielectric nano-antennas
title Bright single photon emitters with enhanced quantum efficiency in a two-dimensional semiconductor coupled with dielectric nano-antennas
title_full Bright single photon emitters with enhanced quantum efficiency in a two-dimensional semiconductor coupled with dielectric nano-antennas
title_fullStr Bright single photon emitters with enhanced quantum efficiency in a two-dimensional semiconductor coupled with dielectric nano-antennas
title_full_unstemmed Bright single photon emitters with enhanced quantum efficiency in a two-dimensional semiconductor coupled with dielectric nano-antennas
title_short Bright single photon emitters with enhanced quantum efficiency in a two-dimensional semiconductor coupled with dielectric nano-antennas
title_sort bright single photon emitters with enhanced quantum efficiency in a two-dimensional semiconductor coupled with dielectric nano-antennas
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8523570/
https://www.ncbi.nlm.nih.gov/pubmed/34663795
http://dx.doi.org/10.1038/s41467-021-26262-3
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