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Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure
Quantum confinement in transition metal dichalcogenides (TMDCs) enables the realization of deterministic single-photon emitters. The position and polarization control of single photons have been achieved via local strain engineering using nanostructures. However, most existing TMDC-based emitters ar...
Autores principales: | , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Association for the Advancement of Science
2021
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8528413/ https://www.ncbi.nlm.nih.gov/pubmed/34669464 http://dx.doi.org/10.1126/sciadv.abj3176 |
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author | So, Jae-Pil Kim, Ha-Reem Baek, Hyeonjun Jeong, Kwang-Yong Lee, Hoo-Cheol Huh, Woong Kim, Yoon Seok Watanabe, Kenji Taniguchi, Takashi Kim, Jungkil Lee, Chul-Ho Park, Hong-Gyu |
author_facet | So, Jae-Pil Kim, Ha-Reem Baek, Hyeonjun Jeong, Kwang-Yong Lee, Hoo-Cheol Huh, Woong Kim, Yoon Seok Watanabe, Kenji Taniguchi, Takashi Kim, Jungkil Lee, Chul-Ho Park, Hong-Gyu |
author_sort | So, Jae-Pil |
collection | PubMed |
description | Quantum confinement in transition metal dichalcogenides (TMDCs) enables the realization of deterministic single-photon emitters. The position and polarization control of single photons have been achieved via local strain engineering using nanostructures. However, most existing TMDC-based emitters are operated by optical pumping, while the emission sites in electrically pumped emitters are uncontrolled. Here, we demonstrate electrically driven single-photon emitters located at the positions where strains are induced by atomic force microscope indentation on a van der Waals heterostructure consisting of graphene, hexagonal boron nitride, and tungsten diselenide. The optical, electrical, and mechanical properties induced by the local strain gradient were systematically analyzed. The emission at the indentation sites exhibits photon antibunching behavior with a g((2))(0) value of ~0.3, intensity saturation, and a linearly cross-polarized doublet, at 4 kelvin. This robust spatial control of electrically driven single-photon emitters will pave the way for the practical implementation of integrated quantum light sources. |
format | Online Article Text |
id | pubmed-8528413 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | American Association for the Advancement of Science |
record_format | MEDLINE/PubMed |
spelling | pubmed-85284132021-10-28 Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure So, Jae-Pil Kim, Ha-Reem Baek, Hyeonjun Jeong, Kwang-Yong Lee, Hoo-Cheol Huh, Woong Kim, Yoon Seok Watanabe, Kenji Taniguchi, Takashi Kim, Jungkil Lee, Chul-Ho Park, Hong-Gyu Sci Adv Physical and Materials Sciences Quantum confinement in transition metal dichalcogenides (TMDCs) enables the realization of deterministic single-photon emitters. The position and polarization control of single photons have been achieved via local strain engineering using nanostructures. However, most existing TMDC-based emitters are operated by optical pumping, while the emission sites in electrically pumped emitters are uncontrolled. Here, we demonstrate electrically driven single-photon emitters located at the positions where strains are induced by atomic force microscope indentation on a van der Waals heterostructure consisting of graphene, hexagonal boron nitride, and tungsten diselenide. The optical, electrical, and mechanical properties induced by the local strain gradient were systematically analyzed. The emission at the indentation sites exhibits photon antibunching behavior with a g((2))(0) value of ~0.3, intensity saturation, and a linearly cross-polarized doublet, at 4 kelvin. This robust spatial control of electrically driven single-photon emitters will pave the way for the practical implementation of integrated quantum light sources. American Association for the Advancement of Science 2021-10-20 /pmc/articles/PMC8528413/ /pubmed/34669464 http://dx.doi.org/10.1126/sciadv.abj3176 Text en Copyright © 2021 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). https://creativecommons.org/licenses/by-nc/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (https://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited. |
spellingShingle | Physical and Materials Sciences So, Jae-Pil Kim, Ha-Reem Baek, Hyeonjun Jeong, Kwang-Yong Lee, Hoo-Cheol Huh, Woong Kim, Yoon Seok Watanabe, Kenji Taniguchi, Takashi Kim, Jungkil Lee, Chul-Ho Park, Hong-Gyu Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure |
title | Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure |
title_full | Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure |
title_fullStr | Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure |
title_full_unstemmed | Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure |
title_short | Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure |
title_sort | electrically driven strain-induced deterministic single-photon emitters in a van der waals heterostructure |
topic | Physical and Materials Sciences |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8528413/ https://www.ncbi.nlm.nih.gov/pubmed/34669464 http://dx.doi.org/10.1126/sciadv.abj3176 |
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