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Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure

Quantum confinement in transition metal dichalcogenides (TMDCs) enables the realization of deterministic single-photon emitters. The position and polarization control of single photons have been achieved via local strain engineering using nanostructures. However, most existing TMDC-based emitters ar...

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Autores principales: So, Jae-Pil, Kim, Ha-Reem, Baek, Hyeonjun, Jeong, Kwang-Yong, Lee, Hoo-Cheol, Huh, Woong, Kim, Yoon Seok, Watanabe, Kenji, Taniguchi, Takashi, Kim, Jungkil, Lee, Chul-Ho, Park, Hong-Gyu
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8528413/
https://www.ncbi.nlm.nih.gov/pubmed/34669464
http://dx.doi.org/10.1126/sciadv.abj3176
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author So, Jae-Pil
Kim, Ha-Reem
Baek, Hyeonjun
Jeong, Kwang-Yong
Lee, Hoo-Cheol
Huh, Woong
Kim, Yoon Seok
Watanabe, Kenji
Taniguchi, Takashi
Kim, Jungkil
Lee, Chul-Ho
Park, Hong-Gyu
author_facet So, Jae-Pil
Kim, Ha-Reem
Baek, Hyeonjun
Jeong, Kwang-Yong
Lee, Hoo-Cheol
Huh, Woong
Kim, Yoon Seok
Watanabe, Kenji
Taniguchi, Takashi
Kim, Jungkil
Lee, Chul-Ho
Park, Hong-Gyu
author_sort So, Jae-Pil
collection PubMed
description Quantum confinement in transition metal dichalcogenides (TMDCs) enables the realization of deterministic single-photon emitters. The position and polarization control of single photons have been achieved via local strain engineering using nanostructures. However, most existing TMDC-based emitters are operated by optical pumping, while the emission sites in electrically pumped emitters are uncontrolled. Here, we demonstrate electrically driven single-photon emitters located at the positions where strains are induced by atomic force microscope indentation on a van der Waals heterostructure consisting of graphene, hexagonal boron nitride, and tungsten diselenide. The optical, electrical, and mechanical properties induced by the local strain gradient were systematically analyzed. The emission at the indentation sites exhibits photon antibunching behavior with a g((2))(0) value of ~0.3, intensity saturation, and a linearly cross-polarized doublet, at 4 kelvin. This robust spatial control of electrically driven single-photon emitters will pave the way for the practical implementation of integrated quantum light sources.
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spelling pubmed-85284132021-10-28 Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure So, Jae-Pil Kim, Ha-Reem Baek, Hyeonjun Jeong, Kwang-Yong Lee, Hoo-Cheol Huh, Woong Kim, Yoon Seok Watanabe, Kenji Taniguchi, Takashi Kim, Jungkil Lee, Chul-Ho Park, Hong-Gyu Sci Adv Physical and Materials Sciences Quantum confinement in transition metal dichalcogenides (TMDCs) enables the realization of deterministic single-photon emitters. The position and polarization control of single photons have been achieved via local strain engineering using nanostructures. However, most existing TMDC-based emitters are operated by optical pumping, while the emission sites in electrically pumped emitters are uncontrolled. Here, we demonstrate electrically driven single-photon emitters located at the positions where strains are induced by atomic force microscope indentation on a van der Waals heterostructure consisting of graphene, hexagonal boron nitride, and tungsten diselenide. The optical, electrical, and mechanical properties induced by the local strain gradient were systematically analyzed. The emission at the indentation sites exhibits photon antibunching behavior with a g((2))(0) value of ~0.3, intensity saturation, and a linearly cross-polarized doublet, at 4 kelvin. This robust spatial control of electrically driven single-photon emitters will pave the way for the practical implementation of integrated quantum light sources. American Association for the Advancement of Science 2021-10-20 /pmc/articles/PMC8528413/ /pubmed/34669464 http://dx.doi.org/10.1126/sciadv.abj3176 Text en Copyright © 2021 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). https://creativecommons.org/licenses/by-nc/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (https://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.
spellingShingle Physical and Materials Sciences
So, Jae-Pil
Kim, Ha-Reem
Baek, Hyeonjun
Jeong, Kwang-Yong
Lee, Hoo-Cheol
Huh, Woong
Kim, Yoon Seok
Watanabe, Kenji
Taniguchi, Takashi
Kim, Jungkil
Lee, Chul-Ho
Park, Hong-Gyu
Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure
title Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure
title_full Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure
title_fullStr Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure
title_full_unstemmed Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure
title_short Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure
title_sort electrically driven strain-induced deterministic single-photon emitters in a van der waals heterostructure
topic Physical and Materials Sciences
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8528413/
https://www.ncbi.nlm.nih.gov/pubmed/34669464
http://dx.doi.org/10.1126/sciadv.abj3176
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