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Polariton condensation in an organic microcavity utilising a hybrid metal-DBR mirror

We have developed a simplified approach to fabricate high-reflectivity mirrors suitable for applications in a strongly-coupled organic-semiconductor microcavity. Such mirrors are based on a small number of quarter-wave dielectric pairs deposited on top of a thick silver film that combine high reflec...

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Detalles Bibliográficos
Autores principales: McGhee, Kirsty E., Putintsev, Anton, Jayaprakash, Rahul, Georgiou, Kyriacos, O’Kane, Mary E., Kilbride, Rachel C., Cassella, Elena J., Cavazzini, Marco, Sannikov, Denis A., Lagoudakis, Pavlos G., Lidzey, David G.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8536762/
https://www.ncbi.nlm.nih.gov/pubmed/34686707
http://dx.doi.org/10.1038/s41598-021-00203-y
Descripción
Sumario:We have developed a simplified approach to fabricate high-reflectivity mirrors suitable for applications in a strongly-coupled organic-semiconductor microcavity. Such mirrors are based on a small number of quarter-wave dielectric pairs deposited on top of a thick silver film that combine high reflectivity and broad reflectivity bandwidth. Using this approach, we construct a microcavity containing the molecular dye BODIPY-Br in which the bottom cavity mirror is composed of a silver layer coated by a SiO(2) and a Nb(2)O(5) film, and show that this cavity undergoes polariton condensation at a similar threshold to that of a control cavity whose bottom mirror consists of ten quarter-wave dielectric pairs. We observe, however, that the roughness of the hybrid mirror—caused by limited adhesion between the silver and the dielectric pair—apparently prevents complete collapse of the population to the ground polariton state above the condensation threshold.