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One-Step Fabrication of a Functionally Integrated Device Based on Polydimethylsiloxane-Coated SiO(2) NPs for Efficient and Continuous Oil Absorption

The construction of superhydrophobic surfaces necessitates the rational design of topographic surface structure and the reduction of surface energy. To date, the reported strategies are usually complex with multi-steps and costly. Thus, the simultaneous achievement of the two indispensable factors i...

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Autores principales: Ju, Guannan, Zhou, Lei, Jiao, Chang, Shen, Jiafeng, Luan, Yihao, Zhao, Xinyu
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8537208/
https://www.ncbi.nlm.nih.gov/pubmed/34683592
http://dx.doi.org/10.3390/ma14205998
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author Ju, Guannan
Zhou, Lei
Jiao, Chang
Shen, Jiafeng
Luan, Yihao
Zhao, Xinyu
author_facet Ju, Guannan
Zhou, Lei
Jiao, Chang
Shen, Jiafeng
Luan, Yihao
Zhao, Xinyu
author_sort Ju, Guannan
collection PubMed
description The construction of superhydrophobic surfaces necessitates the rational design of topographic surface structure and the reduction of surface energy. To date, the reported strategies are usually complex with multi-steps and costly. Thus, the simultaneous achievement of the two indispensable factors is highly desired, yet rather challenging. Herein, we develop a novel structure engineering strategy of realizing the fabrication of a functionally integrated device (FID) with a superhydrophobic surface via a one-step spraying method. Specifically, silica nanoparticles are used to control the surface roughness of the device, while polydimethylsiloxane is employed as the hydrophobic coating. Benefitting from the adopted superhydrophobicity, the as-fabricated FID exhibits a continuous, excellent oil-water separating performance (e.g., 92.5% separating efficiency) when coupled with a peristaltic pump. Notably, a smart design of incorporating a gas switch is adopted in this device, thereby effectively preventing water from entering the FID, realizing thorough oil collection, and avoiding secondary pollution. This work opens up an avenue for the design and development of the FID, accessible for rapid preparation and large-scale practical application.
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spelling pubmed-85372082021-10-24 One-Step Fabrication of a Functionally Integrated Device Based on Polydimethylsiloxane-Coated SiO(2) NPs for Efficient and Continuous Oil Absorption Ju, Guannan Zhou, Lei Jiao, Chang Shen, Jiafeng Luan, Yihao Zhao, Xinyu Materials (Basel) Article The construction of superhydrophobic surfaces necessitates the rational design of topographic surface structure and the reduction of surface energy. To date, the reported strategies are usually complex with multi-steps and costly. Thus, the simultaneous achievement of the two indispensable factors is highly desired, yet rather challenging. Herein, we develop a novel structure engineering strategy of realizing the fabrication of a functionally integrated device (FID) with a superhydrophobic surface via a one-step spraying method. Specifically, silica nanoparticles are used to control the surface roughness of the device, while polydimethylsiloxane is employed as the hydrophobic coating. Benefitting from the adopted superhydrophobicity, the as-fabricated FID exhibits a continuous, excellent oil-water separating performance (e.g., 92.5% separating efficiency) when coupled with a peristaltic pump. Notably, a smart design of incorporating a gas switch is adopted in this device, thereby effectively preventing water from entering the FID, realizing thorough oil collection, and avoiding secondary pollution. This work opens up an avenue for the design and development of the FID, accessible for rapid preparation and large-scale practical application. MDPI 2021-10-12 /pmc/articles/PMC8537208/ /pubmed/34683592 http://dx.doi.org/10.3390/ma14205998 Text en © 2021 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Ju, Guannan
Zhou, Lei
Jiao, Chang
Shen, Jiafeng
Luan, Yihao
Zhao, Xinyu
One-Step Fabrication of a Functionally Integrated Device Based on Polydimethylsiloxane-Coated SiO(2) NPs for Efficient and Continuous Oil Absorption
title One-Step Fabrication of a Functionally Integrated Device Based on Polydimethylsiloxane-Coated SiO(2) NPs for Efficient and Continuous Oil Absorption
title_full One-Step Fabrication of a Functionally Integrated Device Based on Polydimethylsiloxane-Coated SiO(2) NPs for Efficient and Continuous Oil Absorption
title_fullStr One-Step Fabrication of a Functionally Integrated Device Based on Polydimethylsiloxane-Coated SiO(2) NPs for Efficient and Continuous Oil Absorption
title_full_unstemmed One-Step Fabrication of a Functionally Integrated Device Based on Polydimethylsiloxane-Coated SiO(2) NPs for Efficient and Continuous Oil Absorption
title_short One-Step Fabrication of a Functionally Integrated Device Based on Polydimethylsiloxane-Coated SiO(2) NPs for Efficient and Continuous Oil Absorption
title_sort one-step fabrication of a functionally integrated device based on polydimethylsiloxane-coated sio(2) nps for efficient and continuous oil absorption
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8537208/
https://www.ncbi.nlm.nih.gov/pubmed/34683592
http://dx.doi.org/10.3390/ma14205998
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