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Electro-Optical Biosensor Based on Embedded Double-Monolayer of Graphene Capacitor in Polymer Technology

In this work, we present an interferometric polymer-based electro-optical device, integrated with an embedded double-monolayer graphene capacitor for biosensing applications. An external voltage across the capacitor applies an electric field to the graphene layers modifying their surface charge dens...

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Autores principales: Portes, Ary V. R., Martins, Ana J. L., Guerrero, Jesus Alvarez, Carvalho, Mauricio M., Amaya-Fernandez, Ferney O., Saito, Lúcia A. M., Ramirez, Jhonattan C.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8537356/
https://www.ncbi.nlm.nih.gov/pubmed/34685322
http://dx.doi.org/10.3390/polym13203564
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author Portes, Ary V. R.
Martins, Ana J. L.
Guerrero, Jesus Alvarez
Carvalho, Mauricio M.
Amaya-Fernandez, Ferney O.
Saito, Lúcia A. M.
Ramirez, Jhonattan C.
author_facet Portes, Ary V. R.
Martins, Ana J. L.
Guerrero, Jesus Alvarez
Carvalho, Mauricio M.
Amaya-Fernandez, Ferney O.
Saito, Lúcia A. M.
Ramirez, Jhonattan C.
author_sort Portes, Ary V. R.
collection PubMed
description In this work, we present an interferometric polymer-based electro-optical device, integrated with an embedded double-monolayer graphene capacitor for biosensing applications. An external voltage across the capacitor applies an electric field to the graphene layers modifying their surface charge density and the Fermi level position in these layers. This in turn changes the electro-optic properties of the graphene layers making absorption in the waveguide tunable with external voltages. Simultaneously, it is possible to appreciate that this phenomenon contributes to the maximization of the light-graphene interaction by evanescent wave in the sensing area. As a result, it is obtained large phase changes at the output of the interferometer, as a function of small variations in the refractive index in the cladding area, which significantly increasing the sensitivity of the device. The optimum interaction length obtained was 1.24 cm considering a cladding refractive index of 1.33. An absorption change of 129 dB/mm was demonstrated. This result combined with the photonic device based on polymer technology may enable a low-cost solution for biosensing applications in Point of Care (PoC) platform.
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spelling pubmed-85373562021-10-24 Electro-Optical Biosensor Based on Embedded Double-Monolayer of Graphene Capacitor in Polymer Technology Portes, Ary V. R. Martins, Ana J. L. Guerrero, Jesus Alvarez Carvalho, Mauricio M. Amaya-Fernandez, Ferney O. Saito, Lúcia A. M. Ramirez, Jhonattan C. Polymers (Basel) Article In this work, we present an interferometric polymer-based electro-optical device, integrated with an embedded double-monolayer graphene capacitor for biosensing applications. An external voltage across the capacitor applies an electric field to the graphene layers modifying their surface charge density and the Fermi level position in these layers. This in turn changes the electro-optic properties of the graphene layers making absorption in the waveguide tunable with external voltages. Simultaneously, it is possible to appreciate that this phenomenon contributes to the maximization of the light-graphene interaction by evanescent wave in the sensing area. As a result, it is obtained large phase changes at the output of the interferometer, as a function of small variations in the refractive index in the cladding area, which significantly increasing the sensitivity of the device. The optimum interaction length obtained was 1.24 cm considering a cladding refractive index of 1.33. An absorption change of 129 dB/mm was demonstrated. This result combined with the photonic device based on polymer technology may enable a low-cost solution for biosensing applications in Point of Care (PoC) platform. MDPI 2021-10-15 /pmc/articles/PMC8537356/ /pubmed/34685322 http://dx.doi.org/10.3390/polym13203564 Text en © 2021 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Portes, Ary V. R.
Martins, Ana J. L.
Guerrero, Jesus Alvarez
Carvalho, Mauricio M.
Amaya-Fernandez, Ferney O.
Saito, Lúcia A. M.
Ramirez, Jhonattan C.
Electro-Optical Biosensor Based on Embedded Double-Monolayer of Graphene Capacitor in Polymer Technology
title Electro-Optical Biosensor Based on Embedded Double-Monolayer of Graphene Capacitor in Polymer Technology
title_full Electro-Optical Biosensor Based on Embedded Double-Monolayer of Graphene Capacitor in Polymer Technology
title_fullStr Electro-Optical Biosensor Based on Embedded Double-Monolayer of Graphene Capacitor in Polymer Technology
title_full_unstemmed Electro-Optical Biosensor Based on Embedded Double-Monolayer of Graphene Capacitor in Polymer Technology
title_short Electro-Optical Biosensor Based on Embedded Double-Monolayer of Graphene Capacitor in Polymer Technology
title_sort electro-optical biosensor based on embedded double-monolayer of graphene capacitor in polymer technology
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8537356/
https://www.ncbi.nlm.nih.gov/pubmed/34685322
http://dx.doi.org/10.3390/polym13203564
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