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Magic Numbers in Boson (4)He Clusters: The Auger Evaporation Mechanism

The absence of magic numbers in bosonic (4)He clusters predicted by all theories since 1984 has been challenged by high-resolution matter-wave diffraction experiments. The observed magic numbers were explained in terms of enhanced growth rates of specific cluster sizes for which an additional excita...

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Detalles Bibliográficos
Autores principales: Spreafico, Elena, Benedek, Giorgio, Kornilov, Oleg, Toennies, Jan Peter
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8537914/
https://www.ncbi.nlm.nih.gov/pubmed/34684825
http://dx.doi.org/10.3390/molecules26206244
Descripción
Sumario:The absence of magic numbers in bosonic (4)He clusters predicted by all theories since 1984 has been challenged by high-resolution matter-wave diffraction experiments. The observed magic numbers were explained in terms of enhanced growth rates of specific cluster sizes for which an additional excitation level calculated by diffusion Monte Carlo is stabilized. The present theoretical study provides an alternative explanation based on a simple independent particle model of the He clusters. Collisions between cluster atoms in excited states within the cluster lead to selective evaporation via an Auger process. The calculated magic numbers as well as the shape of the number distributions are in quite reasonable agreement with the experiments.