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Magic Numbers in Boson (4)He Clusters: The Auger Evaporation Mechanism

The absence of magic numbers in bosonic (4)He clusters predicted by all theories since 1984 has been challenged by high-resolution matter-wave diffraction experiments. The observed magic numbers were explained in terms of enhanced growth rates of specific cluster sizes for which an additional excita...

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Autores principales: Spreafico, Elena, Benedek, Giorgio, Kornilov, Oleg, Toennies, Jan Peter
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8537914/
https://www.ncbi.nlm.nih.gov/pubmed/34684825
http://dx.doi.org/10.3390/molecules26206244
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author Spreafico, Elena
Benedek, Giorgio
Kornilov, Oleg
Toennies, Jan Peter
author_facet Spreafico, Elena
Benedek, Giorgio
Kornilov, Oleg
Toennies, Jan Peter
author_sort Spreafico, Elena
collection PubMed
description The absence of magic numbers in bosonic (4)He clusters predicted by all theories since 1984 has been challenged by high-resolution matter-wave diffraction experiments. The observed magic numbers were explained in terms of enhanced growth rates of specific cluster sizes for which an additional excitation level calculated by diffusion Monte Carlo is stabilized. The present theoretical study provides an alternative explanation based on a simple independent particle model of the He clusters. Collisions between cluster atoms in excited states within the cluster lead to selective evaporation via an Auger process. The calculated magic numbers as well as the shape of the number distributions are in quite reasonable agreement with the experiments.
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spelling pubmed-85379142021-10-24 Magic Numbers in Boson (4)He Clusters: The Auger Evaporation Mechanism Spreafico, Elena Benedek, Giorgio Kornilov, Oleg Toennies, Jan Peter Molecules Article The absence of magic numbers in bosonic (4)He clusters predicted by all theories since 1984 has been challenged by high-resolution matter-wave diffraction experiments. The observed magic numbers were explained in terms of enhanced growth rates of specific cluster sizes for which an additional excitation level calculated by diffusion Monte Carlo is stabilized. The present theoretical study provides an alternative explanation based on a simple independent particle model of the He clusters. Collisions between cluster atoms in excited states within the cluster lead to selective evaporation via an Auger process. The calculated magic numbers as well as the shape of the number distributions are in quite reasonable agreement with the experiments. MDPI 2021-10-15 /pmc/articles/PMC8537914/ /pubmed/34684825 http://dx.doi.org/10.3390/molecules26206244 Text en © 2021 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Spreafico, Elena
Benedek, Giorgio
Kornilov, Oleg
Toennies, Jan Peter
Magic Numbers in Boson (4)He Clusters: The Auger Evaporation Mechanism
title Magic Numbers in Boson (4)He Clusters: The Auger Evaporation Mechanism
title_full Magic Numbers in Boson (4)He Clusters: The Auger Evaporation Mechanism
title_fullStr Magic Numbers in Boson (4)He Clusters: The Auger Evaporation Mechanism
title_full_unstemmed Magic Numbers in Boson (4)He Clusters: The Auger Evaporation Mechanism
title_short Magic Numbers in Boson (4)He Clusters: The Auger Evaporation Mechanism
title_sort magic numbers in boson (4)he clusters: the auger evaporation mechanism
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8537914/
https://www.ncbi.nlm.nih.gov/pubmed/34684825
http://dx.doi.org/10.3390/molecules26206244
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