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Optimization Based on the Surface Plasmon Optical Properties of Adjustable Metal Nano-Microcavity System for Biosensing

This paper mainly studies the plasma optical properties of the silver nanorod and gold film system with gap structure. During the experiment, the finite element analysis method and COMSOL Multiphysics are used for modeling and simulation. The study changes the thickness of the PE spacer layer betwee...

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Autores principales: Zhu, Jin, Yang, Yiye, Yin, Yanping, Yuan, Huining
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Frontiers Media S.A. 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8554147/
https://www.ncbi.nlm.nih.gov/pubmed/34722464
http://dx.doi.org/10.3389/fchem.2021.762638
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author Zhu, Jin
Yang, Yiye
Yin, Yanping
Yuan, Huining
author_facet Zhu, Jin
Yang, Yiye
Yin, Yanping
Yuan, Huining
author_sort Zhu, Jin
collection PubMed
description This paper mainly studies the plasma optical properties of the silver nanorod and gold film system with gap structure. During the experiment, the finite element analysis method and COMSOL Multiphysics are used for modeling and simulation. The study changes the thickness of the PE spacer layer between the silver nanorod and the gold film, the conditions of the incident light and the surrounding environment medium. Due to the anisotropic characteristics of silver nanorod, the microcavity system is extremely sensitive to the changes of internal and external conditions, and the system exhibits strong performance along the long axis of the nanorod. By analyzing the extinction spectrum of the nanoparticle and the electric field section diagrams at resonance peak, it is found that the plasma optical properties of the system greatly depend on the gap distance, and the surrounding electric field of the silver nanorod is confined in the gap. Both ends of the nanorod and the gap are distributed with high concentrations of hot spots, which reflects the strong hybridization of multiple resonance modes. Under certain excitation conditions, the plasma hybridization behavior will produce a multi-pole mode, and the surface electric field distribution of the nanorod reflects the spatial directionality. In addition, the system is also highly sensitive to the environmental media, which will cause significant changes in its optical properties. The plasma microcavity system with silver nanorod and gold film studied in this paper can be used to develop high-sensitivity biosensors, which has great value in the field of biomedical detection.
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spelling pubmed-85541472021-10-30 Optimization Based on the Surface Plasmon Optical Properties of Adjustable Metal Nano-Microcavity System for Biosensing Zhu, Jin Yang, Yiye Yin, Yanping Yuan, Huining Front Chem Chemistry This paper mainly studies the plasma optical properties of the silver nanorod and gold film system with gap structure. During the experiment, the finite element analysis method and COMSOL Multiphysics are used for modeling and simulation. The study changes the thickness of the PE spacer layer between the silver nanorod and the gold film, the conditions of the incident light and the surrounding environment medium. Due to the anisotropic characteristics of silver nanorod, the microcavity system is extremely sensitive to the changes of internal and external conditions, and the system exhibits strong performance along the long axis of the nanorod. By analyzing the extinction spectrum of the nanoparticle and the electric field section diagrams at resonance peak, it is found that the plasma optical properties of the system greatly depend on the gap distance, and the surrounding electric field of the silver nanorod is confined in the gap. Both ends of the nanorod and the gap are distributed with high concentrations of hot spots, which reflects the strong hybridization of multiple resonance modes. Under certain excitation conditions, the plasma hybridization behavior will produce a multi-pole mode, and the surface electric field distribution of the nanorod reflects the spatial directionality. In addition, the system is also highly sensitive to the environmental media, which will cause significant changes in its optical properties. The plasma microcavity system with silver nanorod and gold film studied in this paper can be used to develop high-sensitivity biosensors, which has great value in the field of biomedical detection. Frontiers Media S.A. 2021-10-15 /pmc/articles/PMC8554147/ /pubmed/34722464 http://dx.doi.org/10.3389/fchem.2021.762638 Text en Copyright © 2021 Zhu, Yang, Yin and Yuan. https://creativecommons.org/licenses/by/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) and the copyright owner(s) are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms.
spellingShingle Chemistry
Zhu, Jin
Yang, Yiye
Yin, Yanping
Yuan, Huining
Optimization Based on the Surface Plasmon Optical Properties of Adjustable Metal Nano-Microcavity System for Biosensing
title Optimization Based on the Surface Plasmon Optical Properties of Adjustable Metal Nano-Microcavity System for Biosensing
title_full Optimization Based on the Surface Plasmon Optical Properties of Adjustable Metal Nano-Microcavity System for Biosensing
title_fullStr Optimization Based on the Surface Plasmon Optical Properties of Adjustable Metal Nano-Microcavity System for Biosensing
title_full_unstemmed Optimization Based on the Surface Plasmon Optical Properties of Adjustable Metal Nano-Microcavity System for Biosensing
title_short Optimization Based on the Surface Plasmon Optical Properties of Adjustable Metal Nano-Microcavity System for Biosensing
title_sort optimization based on the surface plasmon optical properties of adjustable metal nano-microcavity system for biosensing
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8554147/
https://www.ncbi.nlm.nih.gov/pubmed/34722464
http://dx.doi.org/10.3389/fchem.2021.762638
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