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Current-Induced One-Dimensional Diffusion of Co Adatoms on Graphene Nanoribbons

[Image: see text] One-dimensional diffusion of Co adatoms on graphene nanoribbons has been induced and investigated by means of scanning tunnelling microscopy (STM). To this end, the nanoribbons and the Co adatoms have been imaged before and after injecting current pulses into the nanoribbons, with...

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Autores principales: Preis, Tobias, Vrbica, Sasha, Eroms, Jonathan, Repp, Jascha, van Ruitenbeek, Jan M.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2021
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8554795/
https://www.ncbi.nlm.nih.gov/pubmed/34652923
http://dx.doi.org/10.1021/acs.nanolett.1c03073
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author Preis, Tobias
Vrbica, Sasha
Eroms, Jonathan
Repp, Jascha
van Ruitenbeek, Jan M.
author_facet Preis, Tobias
Vrbica, Sasha
Eroms, Jonathan
Repp, Jascha
van Ruitenbeek, Jan M.
author_sort Preis, Tobias
collection PubMed
description [Image: see text] One-dimensional diffusion of Co adatoms on graphene nanoribbons has been induced and investigated by means of scanning tunnelling microscopy (STM). To this end, the nanoribbons and the Co adatoms have been imaged before and after injecting current pulses into the nanoribbons, with the STM tip in direct contact with the ribbon. We observe current-induced motion of the Co atoms along the nanoribbons, which is approximately described by a distribution expected for a thermally activated one-dimensional random walk. This indicates that the nanoribbons reach temperatures far beyond 100 K, which is well above the temperature of the underlying Au substrate. This model system can be developed further for the study of electromigration at the single-atom level.
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spelling pubmed-85547952021-11-01 Current-Induced One-Dimensional Diffusion of Co Adatoms on Graphene Nanoribbons Preis, Tobias Vrbica, Sasha Eroms, Jonathan Repp, Jascha van Ruitenbeek, Jan M. Nano Lett [Image: see text] One-dimensional diffusion of Co adatoms on graphene nanoribbons has been induced and investigated by means of scanning tunnelling microscopy (STM). To this end, the nanoribbons and the Co adatoms have been imaged before and after injecting current pulses into the nanoribbons, with the STM tip in direct contact with the ribbon. We observe current-induced motion of the Co atoms along the nanoribbons, which is approximately described by a distribution expected for a thermally activated one-dimensional random walk. This indicates that the nanoribbons reach temperatures far beyond 100 K, which is well above the temperature of the underlying Au substrate. This model system can be developed further for the study of electromigration at the single-atom level. American Chemical Society 2021-10-15 2021-10-27 /pmc/articles/PMC8554795/ /pubmed/34652923 http://dx.doi.org/10.1021/acs.nanolett.1c03073 Text en © 2021 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Preis, Tobias
Vrbica, Sasha
Eroms, Jonathan
Repp, Jascha
van Ruitenbeek, Jan M.
Current-Induced One-Dimensional Diffusion of Co Adatoms on Graphene Nanoribbons
title Current-Induced One-Dimensional Diffusion of Co Adatoms on Graphene Nanoribbons
title_full Current-Induced One-Dimensional Diffusion of Co Adatoms on Graphene Nanoribbons
title_fullStr Current-Induced One-Dimensional Diffusion of Co Adatoms on Graphene Nanoribbons
title_full_unstemmed Current-Induced One-Dimensional Diffusion of Co Adatoms on Graphene Nanoribbons
title_short Current-Induced One-Dimensional Diffusion of Co Adatoms on Graphene Nanoribbons
title_sort current-induced one-dimensional diffusion of co adatoms on graphene nanoribbons
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8554795/
https://www.ncbi.nlm.nih.gov/pubmed/34652923
http://dx.doi.org/10.1021/acs.nanolett.1c03073
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