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Quasi-1D exciton channels in strain-engineered 2D materials

Strain engineering is a powerful tool in designing artificial platforms for high-temperature excitonic quantum devices. Combining strong light-matter interaction with robust and mobile exciton quasiparticles, two-dimensional transition metal dichalcogenides (2D TMDCs) hold great promise in this ende...

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Autores principales: Dirnberger, Florian, Ziegler, Jonas D., Faria Junior, Paulo E., Bushati, Rezlind, Taniguchi, Takashi, Watanabe, Kenji, Fabian, Jaroslav, Bougeard, Dominique, Chernikov, Alexey, Menon, Vinod M.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8555901/
https://www.ncbi.nlm.nih.gov/pubmed/34714670
http://dx.doi.org/10.1126/sciadv.abj3066
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author Dirnberger, Florian
Ziegler, Jonas D.
Faria Junior, Paulo E.
Bushati, Rezlind
Taniguchi, Takashi
Watanabe, Kenji
Fabian, Jaroslav
Bougeard, Dominique
Chernikov, Alexey
Menon, Vinod M.
author_facet Dirnberger, Florian
Ziegler, Jonas D.
Faria Junior, Paulo E.
Bushati, Rezlind
Taniguchi, Takashi
Watanabe, Kenji
Fabian, Jaroslav
Bougeard, Dominique
Chernikov, Alexey
Menon, Vinod M.
author_sort Dirnberger, Florian
collection PubMed
description Strain engineering is a powerful tool in designing artificial platforms for high-temperature excitonic quantum devices. Combining strong light-matter interaction with robust and mobile exciton quasiparticles, two-dimensional transition metal dichalcogenides (2D TMDCs) hold great promise in this endeavor. However, realizing complex excitonic architectures based on strain-induced electronic potentials alone has proven to be exceptionally difficult so far. Here, we demonstrate deterministic strain engineering of both single-particle electronic bandstructure and excitonic many-particle interactions. We create quasi-1D transport channels to confine excitons and simultaneously enhance their mobility through locally suppressed exciton-phonon scattering. Using ultrafast, all-optical injection and time-resolved readout, we realize highly directional exciton flow with up to 100% anisotropy both at cryogenic and room temperatures. The demonstrated fundamental modification of the exciton transport properties in a deterministically strained 2D material with effectively tunable dimensionality has broad implications for both basic solid-state science and emerging technologies.
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spelling pubmed-85559012021-11-08 Quasi-1D exciton channels in strain-engineered 2D materials Dirnberger, Florian Ziegler, Jonas D. Faria Junior, Paulo E. Bushati, Rezlind Taniguchi, Takashi Watanabe, Kenji Fabian, Jaroslav Bougeard, Dominique Chernikov, Alexey Menon, Vinod M. Sci Adv Physical and Materials Sciences Strain engineering is a powerful tool in designing artificial platforms for high-temperature excitonic quantum devices. Combining strong light-matter interaction with robust and mobile exciton quasiparticles, two-dimensional transition metal dichalcogenides (2D TMDCs) hold great promise in this endeavor. However, realizing complex excitonic architectures based on strain-induced electronic potentials alone has proven to be exceptionally difficult so far. Here, we demonstrate deterministic strain engineering of both single-particle electronic bandstructure and excitonic many-particle interactions. We create quasi-1D transport channels to confine excitons and simultaneously enhance their mobility through locally suppressed exciton-phonon scattering. Using ultrafast, all-optical injection and time-resolved readout, we realize highly directional exciton flow with up to 100% anisotropy both at cryogenic and room temperatures. The demonstrated fundamental modification of the exciton transport properties in a deterministically strained 2D material with effectively tunable dimensionality has broad implications for both basic solid-state science and emerging technologies. American Association for the Advancement of Science 2021-10-29 /pmc/articles/PMC8555901/ /pubmed/34714670 http://dx.doi.org/10.1126/sciadv.abj3066 Text en Copyright © 2021 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). https://creativecommons.org/licenses/by-nc/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (https://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.
spellingShingle Physical and Materials Sciences
Dirnberger, Florian
Ziegler, Jonas D.
Faria Junior, Paulo E.
Bushati, Rezlind
Taniguchi, Takashi
Watanabe, Kenji
Fabian, Jaroslav
Bougeard, Dominique
Chernikov, Alexey
Menon, Vinod M.
Quasi-1D exciton channels in strain-engineered 2D materials
title Quasi-1D exciton channels in strain-engineered 2D materials
title_full Quasi-1D exciton channels in strain-engineered 2D materials
title_fullStr Quasi-1D exciton channels in strain-engineered 2D materials
title_full_unstemmed Quasi-1D exciton channels in strain-engineered 2D materials
title_short Quasi-1D exciton channels in strain-engineered 2D materials
title_sort quasi-1d exciton channels in strain-engineered 2d materials
topic Physical and Materials Sciences
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8555901/
https://www.ncbi.nlm.nih.gov/pubmed/34714670
http://dx.doi.org/10.1126/sciadv.abj3066
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