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Imaging antiferromagnetic domain fluctuations and the effect of atomic scale disorder in a doped spin-orbit Mott insulator

Correlated oxides can exhibit complex magnetic patterns. Understanding how magnetic domains form in the presence of disorder and their robustness to temperature variations has been of particular interest, but atomic scale insight has been limited. We use spin-polarized scanning tunneling microscopy...

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Autores principales: Zhao, He, Porter, Zach, Chen, Xiang, Wilson, Stephen D., Wang, Ziqiang, Zeljkovic, Ilija
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8580306/
https://www.ncbi.nlm.nih.gov/pubmed/34757784
http://dx.doi.org/10.1126/sciadv.abi6468
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author Zhao, He
Porter, Zach
Chen, Xiang
Wilson, Stephen D.
Wang, Ziqiang
Zeljkovic, Ilija
author_facet Zhao, He
Porter, Zach
Chen, Xiang
Wilson, Stephen D.
Wang, Ziqiang
Zeljkovic, Ilija
author_sort Zhao, He
collection PubMed
description Correlated oxides can exhibit complex magnetic patterns. Understanding how magnetic domains form in the presence of disorder and their robustness to temperature variations has been of particular interest, but atomic scale insight has been limited. We use spin-polarized scanning tunneling microscopy to image the evolution of spin-resolved modulations originating from antiferromagnetic (AF) ordering in a spin-orbit Mott insulator perovskite iridate Sr(3)Ir(2)O(7) as a function of chemical composition and temperature. We find that replacing only several percent of lanthanum for strontium leaves behind nanometer-scale AF puddles clustering away from lanthanum substitutions preferentially located in the middle strontium oxide layer. Thermal erasure and reentry into the low-temperature ground state leads to a spatial reorganization of the AF puddles, which nevertheless maintain scale-invariant fractal geometry in each configuration. Our experiments reveal multiple stable AF configurations at low temperature and shed light onto spatial fluctuations of the AF order around atomic scale disorder in electron-doped Sr(3)Ir(2)O(7).
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spelling pubmed-85803062021-11-18 Imaging antiferromagnetic domain fluctuations and the effect of atomic scale disorder in a doped spin-orbit Mott insulator Zhao, He Porter, Zach Chen, Xiang Wilson, Stephen D. Wang, Ziqiang Zeljkovic, Ilija Sci Adv Physical and Materials Sciences Correlated oxides can exhibit complex magnetic patterns. Understanding how magnetic domains form in the presence of disorder and their robustness to temperature variations has been of particular interest, but atomic scale insight has been limited. We use spin-polarized scanning tunneling microscopy to image the evolution of spin-resolved modulations originating from antiferromagnetic (AF) ordering in a spin-orbit Mott insulator perovskite iridate Sr(3)Ir(2)O(7) as a function of chemical composition and temperature. We find that replacing only several percent of lanthanum for strontium leaves behind nanometer-scale AF puddles clustering away from lanthanum substitutions preferentially located in the middle strontium oxide layer. Thermal erasure and reentry into the low-temperature ground state leads to a spatial reorganization of the AF puddles, which nevertheless maintain scale-invariant fractal geometry in each configuration. Our experiments reveal multiple stable AF configurations at low temperature and shed light onto spatial fluctuations of the AF order around atomic scale disorder in electron-doped Sr(3)Ir(2)O(7). American Association for the Advancement of Science 2021-11-10 /pmc/articles/PMC8580306/ /pubmed/34757784 http://dx.doi.org/10.1126/sciadv.abi6468 Text en Copyright © 2021 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution License 4.0 (CC BY). https://creativecommons.org/licenses/by/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution license (https://creativecommons.org/licenses/by/4.0/) , which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.
spellingShingle Physical and Materials Sciences
Zhao, He
Porter, Zach
Chen, Xiang
Wilson, Stephen D.
Wang, Ziqiang
Zeljkovic, Ilija
Imaging antiferromagnetic domain fluctuations and the effect of atomic scale disorder in a doped spin-orbit Mott insulator
title Imaging antiferromagnetic domain fluctuations and the effect of atomic scale disorder in a doped spin-orbit Mott insulator
title_full Imaging antiferromagnetic domain fluctuations and the effect of atomic scale disorder in a doped spin-orbit Mott insulator
title_fullStr Imaging antiferromagnetic domain fluctuations and the effect of atomic scale disorder in a doped spin-orbit Mott insulator
title_full_unstemmed Imaging antiferromagnetic domain fluctuations and the effect of atomic scale disorder in a doped spin-orbit Mott insulator
title_short Imaging antiferromagnetic domain fluctuations and the effect of atomic scale disorder in a doped spin-orbit Mott insulator
title_sort imaging antiferromagnetic domain fluctuations and the effect of atomic scale disorder in a doped spin-orbit mott insulator
topic Physical and Materials Sciences
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8580306/
https://www.ncbi.nlm.nih.gov/pubmed/34757784
http://dx.doi.org/10.1126/sciadv.abi6468
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